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881.
The periodic precipitation pattern formation in gelatinous media is interpreted as a moving boundary problem. The time law,
spacing law and width law are revisited on the basis of the new scenario. The explicit dependence of the geometric structure
on the initial concentrations of the reactants is derived. Matalon—Packter law, which relates the spacing coefficient with
the initial concentrations is reformulated removing many ambiguities and impractical parameters. Experimental results are
discussed to establish the significance of moving boundary concept in the diffusion controlled pattern forming systems 相似文献
882.
A.D. Bykov V.N. Saveliev C. Camy-Peyret A. Valentin 《Journal of Molecular Spectroscopy》2004,224(2):164-175
Forty-seven N2 broadened water vapor line-widths have been measured in the 1845-2140 cm−1 spectral range with a Fourier Transform spectrometer in the 258-330 K temperature range at a spectral resolution of 0.005 cm−1 for the lines with upper state rotational quantum number up to 16. The measured exponents of the temperature dependence of the width exhibit a large range of values from 1.60 to −0.86. Theoretical calculations were made using a semi-empirical technique based on the Anderson theory. The calculated broadening coefficients as well as the temperature exponents for the half-width agree satisfactory with measured values. 相似文献
883.
We obtain Dirac’s classic monopole charge quantization from the point of view of geometric quantization and demonstrate how this leads to the conclusion that the electromagnetic field is a U(1)-gauge field. 相似文献
884.
The results of optical study and quantum-chemical simulation of a conjugated organic system, 2-cyclooctylamino-5-nitropyridine (COANP)-fullerene, performed to determine its potential for application as a limiter of visible and near-IR laser radiation and as a material for diffraction elements in systems for reversible recording of optical information, are presented. Complexation between a COANP molecule and fullerene is considered as one of the main mechanisms responsible for the corresponding properties of this system. For the first time, nonlinear optical characteristics of COANP-C60 and COANP-C70 systems are comparatively studied and the intermolecular interaction between a COANP molecule and fullerene is analyzed on the quantum-chemical level. 相似文献
885.
A. V. Burenin 《Optics and Spectroscopy》2004,97(6):867-875
A noninvariant geometrical group characterizing the internal dynamics of the tetrahydrofuran molecule C4H8O with allowance for the clearly pronounced pseudorotation effect is constructed. On this basis, some qualitative features of the energy spectrum of the molecule following from the analysis of high-resolution spectroscopic data are explained. 相似文献
886.
The phenomenon of plasmon resonance in a nanosphere and a nanospheroid is considered. As is known, this phenomenon does not depend explicitly on the size of these nanoparticles. However, it is shown that, actually, the resonance conditions are determined by the diameter of the nanosphere and by the length of the major axis of the nanospheroid. 相似文献
887.
Experimental dependences of the doubly charged ion yield N 2+ on the laser radiation intensity F are analyzed for the case of ion formation by the two-electron mechanism. It is shown that the region where the dependence N 2+(F) is characterized by the degree of nonlinearity K≈2.5 corresponds to the saturation of the process of doubly charged ion formation. This region is described well by theoretical calculations performed for Gaussian laser beams. 相似文献
888.
The diffraction of a plane wave incident on a thick hologram at the first and second Bragg angles in the process of nonlinear recording is analyzed using the coupled-wave equations. It is shown that, in this case, the two-wave approximation with the use of effective modulation amplitudes of the refractive index, n 1ef and n 2ef, can be applied. Analytical dependences of n 1ef and n 2ef on the modulation amplitudes of the refractive index n 1 and n 2 at the fundamental and doubled spatial frequencies are obtained and the criteria of their applicability are determined. The dependences found are used to calculate the parameters of gratings recorded in a photopolymeric material. 相似文献
889.
The cross section of absorption of electromagnetic radiation by an inhomogeneous spherical particle is calculated. The general case of an arbitrary value of the ratio of the particle radius to the radius of the dielectric core is considered. The condition of diffuse reflection of electrons from the inner and outer surfaces of the metal layer of the particle is taken as the boundary condition of the problem. The limiting cases are considered and the results obtained are discussed. 相似文献
890.
Computer processing of electronic absorption spectra of rare-earth elements in inorganic laser media
Algorithms and program modules are developed for calculation of the Judd-Ofelt parameters on modern computers. These programs can be used to perform numerical analysis of the energy absorption by rareearth ions in laser media. 相似文献