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11.
A Mukherjee M Dasgupta DJ Hinde CR Morton AC Berriman RD Butt JO Newton H Timmers 《Pramana》2001,57(1):195-198
Fusion cross-sections for the 7Li + 12C reaction have been measured at energies above the Coulomb barrier by the direct detection of evaporation residues. The heavy
evaporation residues with energies below 3 MeV could not be separated out from the α-particles in the spectrum and hence their
contribution was estimated using statistical model calculations. The present work indicates that suppression of fusion cross-sections
due to the breakup of 7Li may not be significant for 7Li + 12C reaction at energies around the barrier. 相似文献
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Usher AJ Lucas NT Dalton GT Randles MD Viau L Humphrey MG Petrie S Stranger R Willis AC Rae AD 《Inorganic chemistry》2006,45(26):10859-10872
Reactions of the tetrahedral clusters MoIr3(mu-CO)3(CO)8(eta-L) (L = C5HMe4, C5Me5) with the carbonylmetalate anions [Mo(CO)3(eta-L)]- afford the trigonal bipyramidal clusters Mo2Ir3(mu3-H)(mu-CO)2(CO)9(eta-L)2 (L = C5HMe4 (3c), 74%; L = C5Me5 (3d), 55%) in which the group 6 metal atoms occupy the apexes; reaction of the cyclopentadienylmolybdenum-containing analogues or their cyclopentadienyltungsten-containing homologues failed to afford analogous products. Reactions of MIr3(mu-CO)3(CO)8(eta-C5H5) (M = Mo, W) with [M(CO)3(eta-L)]- (L = C5HMe4, C5Me5) afford the core-expanded heteroapex clusters M2Ir3(mu3-H)(mu-CO)2(CO)9(eta-C5H5)(eta-L) (M = Mo, L = C5HMe4 (5c), 9%, L = C5Me5 (5d), 4%; M = W, L = C5Me5 (6d), 5%) in low yield, together with the homoapex clusters M2Ir3(mu3-H)(mu-CO)2(CO)9(eta-L)2 (M = Mo, L = C5HMe4 (3c), 81%, L = C5Me5 (3d), 60%; M = W, L = C5Me5 (4d), 5%) in much higher yield for the Mo-containing examples. The identities of clusters 3c,d, 4d, and 5c,d have been confirmed by single-crystal X-ray diffraction studies, with the same disposition of ligands about the trigonal bipyramidal cluster cores being observed in each case, a ligand arrangement that has been examined by complementary density functional theory studies. While cluster 5d is accessible as above, no reaction is observed from MoIr3(mu-CO)3(CO)8(eta-C5Me5) and [M(CO)3(eta-C5H5)]-. Treating MoIr3(mu-CO)3(CO)8(eta-C5H5) with 1 equiv of [M(CO)3(eta-C5Me5)]- affords 5d as the major product, a further 1 equiv affording some MoIr3(mu-CO)3(CO)8(eta-C5Me5) and a third 1 equiv giving a good yield of 3d. This is consistent with reaction proceeding by apex fragment addition, followed by apex fragment elimination, and finally a further apex fragment addition, the homometallic incoming apexes being distinguished from the departing vertices by their highly methylated cyclopentadienyl ligands. Spectroscopic data suggest that the electron density at these disparate-metal-containing cluster cores is tunable by progressive (conceptual) cyclopentadienyl alkylation. 相似文献
16.
C. R. Whitehouse G. Lacey A. G. Cullis S. J. Barnett A. M. Keir A. D. Johnson J. H. Jefferson G. W. Smith T. Martin B. F. Usher B. Lunn J. C. H. Hogg W. E. Hagston P. Ashu B. K. Tanner W. Spirkl G. F. Clark 《Journal of Crystal Growth》1995,150(1-4):85-91
The important value of the X-ray topography (XRT) technique for the investigation of III-V strained-layer relaxation processes is described. In addition to post-growth ex-situ XRT studies, a unique combined XRT/MBE growth facility has been constructed which allows the generation, motion and interaction of misfit dislocations to be monitored in-situ during epilayer growth, for the first time. The in-situ data already obtained for (100) InGaAs strained-layer growth on both Czochralski- and vertical-gradient freeze-grown GaAs substrates indicates technologically important differences in the initial relaxation process, including, in the latter case, the observation of a previously unreported secondary relaxation phase. Initial results relating to the influence of both post-growth annealing and the subsequent cool-down process are also described. 相似文献
17.
C. M. Townsley A. Usher B. L. Gallagher M. Henini G. Hill 《Physica E: Low-dimensional Systems and Nanostructures》1998,1(1-4)
We report a spectroscopic investigation of the densities of both occupied and unoccupied states of a high-quality two-dimensional hole system, in the regime of the quantum Hall effects (QHEs). Photoluminescence and photoluminescence excitation spectroscopies are used to elucidate the complicated valence band structure of the holes, and to establish their optical response to the QHEs. 相似文献
18.
Petravic M Deenapanray PN Comtet G Hellner L Dujardin G Usher BF 《Physical review letters》2000,84(10):2255-2258
Photon-stimulated desorption of H(+) from hydrogenated GaAs (110) and (100) surfaces was studied as a function of photon energy. Distinct peaks, observed around As 3d core-level binding energy for desorption from the GaAs (100) surface and in the As 3d and Ga 3p region for desorption from the GaAs (110) surface, show a striking similarity with the fine structure (spin-orbit splitting) measured in the photoemission from As 3d and Ga 3p levels. These results provide clear evidence for direct desorption processes and represent a basis for selective modification of hydrogenated GaAs surfaces. 相似文献
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E. Eisenhandler W.R. Gibson C. Hojvat P.I.P. Kalmus L.C.Y.Lee Chi Kwong T.W. Pritchard E.C. Usher D.T. Williams M. Harrison W.H. Range M.A.R. Kemp A.D. Rush J.N. Woulds G.T.J. Arnison A. Astbury D.P. Jones A.S.L. Parsons 《Physics letters. [Part B]》1973,47(6):536-540
The differential cross-sections for p → π?π+ in the momentum range 0.8 to 2.4 GeV/c (centre-of-mass energy 2.02 to 2.57 GeV) are analysed in terms of the possible existence of s-channel resonances. The systematics of the dip structures and the s-dependence of dσ/dt are presented. 相似文献