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671.
Désirée Sauter Martin Schröter Christoph Frey Cornelia Weber Ulrike Mersdorf Jan-Willi Janiesch Ilia Platzman Joachim P. Spatz 《Macromolecular bioscience》2023,23(8):2200437
Imitation of cellular processes in cell-like compartments is a current research focus in synthetic biology. Here, a method is introduced for assembling an artificial cytoskeleton in a synthetic cell model system based on a poly(N-isopropyl acrylamide) (PNIPAM) composite material. Toward this end, a PNIPAM-based composite material inside water-in-oil droplets that are stabilized with PNIPAM-functionalized and commercial fluorosurfactants is introduced. The temperature-mediated contraction/release behavior of the PNIPAM-based cytoskeleton is investigated. The reversibility of the PNIPAM transition is further examined in bulk and in droplets and it could be shown that hydrogel induced deformation could be used to controllably manipulate droplet-based synthetic cell motility upon temperature changes. It is envisioned that a combination of the presented artificial cytoskeleton with naturally occurring components might expand the bandwidth of the bottom-up synthetic biology. 相似文献
672.
The structure changes proceeding in AlCu 2.1 at.% Mg(x) alloys with magnesium concentration form 0 to 1.2 at.% at room temperature and 100 °C are followed by small-angle neutron investigation. The results are fitted on different models. The most important result is that with increase of the Mg contents clearly a growth of the thickness opposite to the growth of the growth of the diameter to discern. The results give a good idea of the formation of GPZI(Mg) with the adequate portion of magnesium in the AlCuMg(x)-alloys and their transition to GPZII(Mg) respectively θ″ (Mg). 相似文献
673.
A new morphology of ternary ABC triblock copolymers is presented which results from the asymmetric interaction between a centre block (poly(ethylene-co-butene)) to different end blocks (polystyrene and poly(methyl methacrylate)). This morphology with the appearance of a “knitting pattern” can be described as an intermediate of a morphology of A, B and C lamellae and a morphology of A and C lamellae with B cylinders at the A/C interface. 相似文献
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Dieter Wöhrle Maria Shopova Jörg G. Moser Holger Kliesch Ulrike Michelsen Silke Müller Andrea Weitemeyer 《Macromolecular Symposia》1996,105(1):127-138
Different possibilities of macromolecular metal complexes as photosensitizers (PS) for their potential use in the photodynamic therapy of cancer are described. The prepared metal porphyrazin derivatives (metals: Zn(II), Si(IV)(X)2) exhibit long wavelength absorption and high singlet oxygen quantum yields under irradiation. One possibility is the incorporation of the PSs in liposomal vesicles giving hydrophobic conjugates with low densitiy proteins in the serum after injection. Good tumor accumulation and photodynamic activities are observed. Increased tumor uptake is also known for Pcs covalently connected via the ligand to poly(ethylene glycol monomethyl ether). New compounds contain the hydrophilic polymer at axial substituents of Si(X)2Pc and Si(X)2Nc. Some newly synthesized compounds with only one functional group exhibit the possibility of coupling to macromolecules like e.g. monoclonal antibodies. 相似文献
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