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141.
Ab initio materials design for transparent-conducting-oxide-based new-functional materials 总被引:1,自引:0,他引:1
H. Katayama-Yoshida K. Sato H. Kizaki H. Funashima I. Hamada T. Fukushima V.A. Dinh M. Toyoda 《Applied Physics A: Materials Science & Processing》2007,89(1):19-27
Based upon ab initio electronic structure calculations for delafossite CuAlO2 and ZnO, we report on the design of new-functional materials for transparent conducting oxides (TCO), such as (i) low-resistive
p-type ZnO and CuAlO2 by co-doping, (ii) high-efficiency thermoelectric power in CuAlO2 (ZT>3) by p-type doping, (iii) half-metallic ferromagnetism in transition-metal-impurity doped CuAlO2 and ZnO-based diluted magnetic semiconductors, and (iv) CaO, MgO, SrO and BaO based DMS without transition metal impurities.
We also discuss the implementation of the self-interaction correction to our materials design method.
PACS 61.72.Bb; 61.72.Jj; 71.15.Mb; 72.15.Jf; 82.75.-d 相似文献
142.
We report a direct observation of the temperature field on a steel specimen during ablation by multiple femtosecond laser pulses using an infrared thermography technique. From the experimental results and simulation study of the temperature field, we quantified the deposited thermal power into the specimen during the ablation process. We found that more than two thirds of the incident laser power was deposited in the steel specimen when ablated by multiple femtosecond laser pulses. This result provides further understanding of the heating effect in materials processing by ultrashort laser pulses. 相似文献
143.
H. Tran V. Dana X. Thomas 《Journal of Quantitative Spectroscopy & Radiative Transfer》2007,108(3):342-362
Line intensities are measured for 546 transitions belonging to 13 bands of the main isotopologue 12C2H2 of the acetylene molecule, in the 1.5-μm spectral domain. A multispectrum fitting procedure is used to retrieve line parameters from Fourier transform spectra. Prior to this work, line intensities were known for only 4 bands in this spectral region, from the work of El Hachtouki and Vander Auwera [Absolute line intensities in acetylene: the 1.5 μm region. J Mol Spectrosc 2002;216:355-62]. An excellent agreement is found with the results of these authors, showing that the accuracy of both results is likely better than 1% for the strong bands. However, the spectrum becomes very crowded when one wants to study weaker bands, so that the average accuracy of the intensities reported in the present work is 5%. From these data, vibrational transition dipole moments squared and Herman-Wallis coefficients have been determined for all the bands. 相似文献
144.
145.
Two main existence conditions for solutions of variational relation problems are established without convexity. The first one is based on a finite solvability property and the second one on generalized KKM mappings. These conditions unify and strengthen several existing results in the literature on the topic. A model of satisficing process by rejection is considered which gives an economic interpretation of the introduced concepts. 相似文献
146.
H. Isnard M. Granet C. Caussignac E. Ducarme A. Nonell B. Tran F. Chartier 《Spectrochimica Acta Part B: Atomic Spectroscopy》2009,64(11-12):1280-1286
In the nuclear domain, precise and accurate isotopic composition determination of elements in spent nuclear fuels is mandatory to validate neutron calculation codes and for nuclear waste disposal. The present study presents the results obtained on Cs isotope ratio by mass spectrometric measurements. Natural cesium is monoisotopic (133Cs) whereas cesium in spent fuels has 4 isotopes (133Cs, 134Cs, 135Cs, and 137Cs). As no standard reference material is available to evaluate the accuracy of Cs isotopic measurements, a comparison of cesium isotopic composition in spent nuclear fuels has been performed between Thermal Ionization Mass Spectrometry (TIMS) and a new method involving Multiple Collector Inductively Coupled Plasma Mass Spectrometry (MC-ICPMS) measurements. For TIMS measurements, isotopic fractionation has been evaluated by studying the behavior of cesium isotope ratios (133Cs/137Cs and 135Cs/137Cs) during the analyses. For MC-ICPMS measurements, the mass bias effects have been corrected with an external mass bias correction using elements (Eu and Sb) close to cesium masses. The results obtained by the two techniques show good agreement: relative difference on 133Cs/137Cs and 135Cs/137Cs ratios for two nuclear samples, analyzed after chemical separation, ranges from 0.2% to 0.5% depending on the choice of reference value for mass bias correction by MC-ICPMS. Finally the quantification of the 135Cs/238U ratio by the isotope dilution technique is presented in the case of a MOx (mixed oxide) spent fuel sample. Evaluation of the global uncertainties shows that this ratio could be defined at an uncertainty of 0.5% (k = 2). The intercomparison between two independent mass spectrometric techniques is fundamental for the evaluation of uncertainty when no isotopic standard is available. 相似文献
147.
148.
In this paper we give an introduction to the notion of meromorphic transform. We describe some equidistribution problems and their solution, using the ddc-method. In particular, we give some statistical properties of the equilibrium measure for meromorphic maps on compact Kähler manifolds: K-mixing, exponential decay of correlations and central limit theorem. 相似文献
149.
Z. Szeglowski Dinh Thi Lien S. N. Timokhin A. B. Yakushev I. Zvara 《Journal of Radioanalytical and Nuclear Chemistry》2001,247(2):451-452
The seconds living mercury isotopes have been isolated from nuclear reaction products arising in the bombardment of 147Sm target with 40Ar ions at the U-400 cyclotron of JINR-Dubna. 相似文献
150.