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In accordance with nonperturbative quantum scattering theory,we investigate photoelectron angular distributions(PADs) from above-threshold detachment(ATD) of negative ions irradiated by circularly polarized few-cycle laser fields.Electrons ejected on the polarization plane demonstrate distinct anisotropies in angular distributions which distinctly vary with the carrier-envelope(CE) phase.The anisotropy is caused by interference between transition channels;it also depends strongly on laser frequency,pulse duration,and kinetic energy of photoelectrons.Optimal emission of photoelectrons,which varies with CE phase,makes it possible to control photoelectron motion. 相似文献
194.
The novel visible-light-activated La/I/TiO2 nanocomposition photocatalyst was successfully synthesized using precipitation-dipping method, and characterized by X-ray powder diffraction (XRD), the Brunauer-Emmett-Teller (BET) method, transmission electron microscopy (TEM), thermogravimetry-differential scanning calorimetry (TG-DSC) and UV-vis diffuse reflectance spectroscopy (UV-vis DRS). The photocatalytic activity of La/I/TiO2 was evaluated by studying photodegradation of reactive blue 19 as a probe reaction under simulated sunlight irradiation. Photocatalytic experiment results showed that the maximum specific photocatalytic activity of the La/I/TiO2 photocatalyst appeared when the molar ratio of La/Ti was 2.0 at%, calcined at 350 °C for 2 h, due to the sample with good crystallization, high BET surface area and small crystal size. Under simulated sunlight irradiation, the degradation of reactive blue 19 aqueous solution reached 98.6% in 80 min, which showed La/I/TiO2 photocatalyst to be much higher photocatalytic activity compared to standard Degussa P25 photocatalyst. The higher visible light activity is due to the codoping of lanthanum and iodine. 相似文献
195.
Fuqiang Tian Wenbin Bu Linshuang Shi Chun Yang Yi Wang Qingquan Lei 《Journal of Electrostatics》2011,69(1):7-10
In order to investigate the trap level distribution in polymer films, a new method is proposed based on modified thermally stimulated current (TSC) theory and numerical calculation of the TSC measurement. In this method, a new function is defined to weight the contribution of every trap level to the external current. The demarcation energy is used to study the trap emptying process. The modified TSC theory shows that only the electrons with trap levels very close to the demarcation energy can significantly contribute to the external circuit at any instant temperature. Based on this method, the trap level distribution of the DuPont original polyimide film 100HN and nanocomposite polyimide film 100CR are investigated as an application example. The effectiveness of the method is confirmed by the experiments. The experimental results show that the trap level density in the 100CR PI films is about six times larger than that in the 100HN PI films through the investigated trap level ranges 06–1.3 eV. The increased traps in 100CR should be introduced by nanofillers, probably come from the interfaces formed between nanofillers and the polymer matrix. 相似文献
196.
Let Q G denote the signless Laplacian matrix of a graph G. An eigenvalue μ of Q G is said to be a main Q-eigenvalue of G if μ has an eigenvector which is not orthogonal to an all-ones vector e. We give some basic properties of main Q-eigenvalues. For a graph G of order n, G is called Q-controllable if G has n distinct main Q-eigenvalues. We show that a graph H is generalized Q-cospectral with a Q-controllable G if and only if H is Q-controllable and there exists a unique rational orthogonal matrix R such that R e = e, Q H = R ? Q G R. 相似文献
197.
Qingying Bu Gerard Buskes Alexey I. Popov Adi Tcaciuc Vladimir G. Troitsky 《Positivity》2013,17(2):283-298
We investigate the relationship between the diagonal of the Fremlin projective tensor product of a Banach lattice E with itself and the 2-concavification of E. 相似文献
198.
A novel design for a highly efficient 1-kHz single-frequency green laser is proposed.An efficient singlefrequency laser pulse output at 532-nm wavelength may be obtained by combining the injection seeding with intracavity frequency doubling in a compact U-shaped cavity formed by two plano dichroic mirrors in an end-pumping arrangement.The laser is capable of producing green pulses with a total energy of 6.3 mJ at a pulse repetition rate of 1 kHz.The pulse width is about 10 ns and the optical-optical efficiency from the 808-nm pump source to the 532-nm green output is around 12.7%. 相似文献
199.
trans‐Dichlorotetrapyridineruthenium(II) [trans‐RuCl2(py)4] was synthesized and the structure was determined by single crystal X‐ray crystallography. Highly efficient formation of propylene carbonate (PC) from carbon dioxide and propylene oxide was achieved by using a catalyst system composed of trans‐RuCl2(py)4 and hexadecyl trimethyl ammonium bromide under mild conditions (4h, 80 °C, 3.0 MPa). PC was obtained in nearly 100% selectivity without the formation of a polymer. The catalyst could be recycled constantly many times without any significant loss of its catalytic activity. On the basis of the results, a mechanism for the reaction was proposed. Copyright © 2010 European Peptide Society and John Wiley & Sons, Ltd. 相似文献
200.