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11.
Adriana Aniceto Julia Montenegro Rafael da Silva Cadena Anderson Junger Teodoro 《Molecules (Basel, Switzerland)》2021,26(2)
Amazonian fruits are excellent sources of bioactive compounds and can be used in beverages to improve the nutritional and sensorial characteristics. The present study aimed to develop a blend of murici (Byrsonima Crassifolia (L.) Kunth) and taperebá (Spondias Mombin L.) through experimental design and investigating the nutritional and sensorial characteristics of fruits and beverages. The murici was highlighted as higher vitamin C content (58.88 mg · 100 g−1) compared to taperebá (25.93 mg · 100 g−1). The murici and taperebá are good sources of total phenolic compounds (taperebá 1304.15 ± 19.14 mgGAE · 100 g−1 and the murici of 307.52 ± 19.73 mg GAE · 100 g−1) and flavonoids (174.87 ± 1.76 μgQE/g and 129.46 ± 10.68 μgQE/g, murici and taperebá, respectively), when compared to other Brazilian fruits. The antioxidant capacity in different methods revealed that the taperebá had a higher average in the results, only in the ORAC method and did not present a significant difference (p > 0.05) in relation to the murici. The beverage development was performed using experimental design 23, showed through sensory analysis and surface response methodology that murici and high sugar content (between 12.5 and 14.2% of sugar) influenced in sensory acceptance. Our findings indicate that beverages with improved nutrition and a sensory acceptance can be prepared using taperebá and murici fruits. 相似文献
12.
To clarify the role played by water in facilitating long-range DNA charge transport, carefully designed, state-of-the-art, self-interaction corrected density-functional quantum mechanical and molecular mechanical (SIC-QM/MM) simulations are performed for the first time on two ionized adenine:thymine bridge models in explicit water solvent at finite temperature. For random solvent configurations, the charge is partially delocalized. However, a charge localization on different, well-separated adenines can be induced and is correlated with a restructuring of their first solvation shells. Thus, the importance of water in the mechanism of long-range charge transport is explicitly demonstrated, and the microscopic conditions for a charge localization are revealed. 相似文献
13.
Stephanie A. Grimmel Tiago Q. Teodoro Lucas Visscher 《International journal of quantum chemistry》2020,120(21):e26111
Frozen density embedding (FDE) theory is one of the major techniques aiming to bring modeling of extended chemical systems into the realm of high accuracy calculations. To improve its accuracy it is of interest to develop kinetic energy density functional approximations specifically for FDE applications. In the study reported here we focused on optimizing parameters of a generalized gradient approximation-like kinetic energy functional with the purpose of better describing electron excitation energies. We found that our optimized parametrizations, named excPBE and excPBE-3 (as these are derived from a Perdew-Burke-Ernzerhof-like parametrization), could not yield improvements over available functionals when applied on a test set of systems designed to probe solvatochromic shifts. Moreover, as several different functionals yielded very similar errors to the simple local-density approximation (LDA), it is questionable whether it is worthwhile to go beyond the LDA in this context. 相似文献
14.
Diffraction-limited, 300-kW peak-power pulses from a coiled multimode fiber amplifier 总被引:1,自引:0,他引:1
We report a multimode, double-clad, Yb-doped fiber amplifier that produces diffraction-limited, 0.8-ns pulses with energies of 255 muJ and peak powers in excess of 300 kW at a repetition rate of ~8 kHz . Single-transverse-mode operation was obtained by bend-loss-induced mode filtering of the gain fiber. 相似文献
15.
We report on the use of a single-polarization, 41 μm core-diameter, intrinsically single-mode photonic crystal fiber (PCF) to obtain high peak power (up to 800 kW), 1 ns-duration pulses in a 100:1 linearly polarized, intrinsically single-mode (M2 1.2) output. By transmitting the PCF output through nonlinear crystals, we also obtained efficient second, third, and fourth harmonic generation resulting in peak power >400 kW in the visible (green, 531 nm) and 200 kW in the UV (265.5 nm). To our knowledge these results represent the highest peak power obtained in a linearly polarized output from a fiber and the highest peak power in the visible and UV obtained through harmonic generation of the direct fiber output. 相似文献
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17.
We report on a mid-infrared (mid-IR) source consisting of an approximately 10 W average-power, linearly polarized 1.54 microm wavelength pulsed fiber source pumping an optical parametric oscillator. From this source, we obtained average power in excess of 1 W in the 3.8-4.0 microm wavelength range at a pulse repetition frequency of 100 kHz. With a slightly different setup, we also achieved an average power of 0.25 W at 4.5 microm wavelength. To our knowledge, these values represent the highest mid-IR power obtained through wavelength conversion of an eye-safe fiber source. 相似文献
18.
A large displacement formulation for anisotropic beam analysis 总被引:1,自引:0,他引:1
Summary The displacement of a beam can be conveniently resolved into a roto-translational section displacement and a section warping. The correct second order approximation of the strain is deduced accounting for large displacements and thus for large rotations. On the basis of displacement method, both linear and nonlinear formulations are given: the first one leads to the elastic section properties and to the correct characterization of section warping; the second one leads to the so-called geometric section stiffness, accounting for prestress. Both formulations are general with respect to elastic material properties, thus allowing to deal with aniso-tropic and unhomogeneous cross-sections. Elastic and geometric section rigidities here proposed can then be easily used in second order problems on beam frames: either initial buckling eigenvalue analyses, either large displacement incremental analyses.
Sommario E' conveniente scomporre lo spostamento di un punto di una trave in una rototraslazione della sezione cui appartiene e in uno spostamento che deforma la sezione (in-gobbamento). Si deduce la corretta approssimazione al second'ordine della deformazione per grandi spostamenti e quindi grandi rotazioni. Vengono presentate sia la formulazione lineare che quella non lineare, basate sul metodo degli spostamenti: dalla prima si ottengono le caratteristiche elastiche della sezione e la corretta caratterizzazione dell'ingob-bamento; dalla seconda la cosiddetta rigidezza geometrica della sezione che tiene conto dello stato di presforzo. Entrambe le formulazioni sono generali per quanto riguarda le proprietà del materiale elastico, potendosi così considerare anche sezioni anisotrope e non omogenee. Le caratteristiche di rigidezza elastica e geometrica della sezione possono quindi facilmente essere usate in problemi del second'ordine su strutture a travi: sia analisi agli autovalori della stabilità, sia analisi incrementali con grandi spostamenti.相似文献
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20.
Efficient second, third, fourth, and fifth harmonic generation of a Yb-doped fiber amplifier 总被引:1,自引:0,他引:1
Dahv A. V. Kliner Fabio Di Teodoro Jeffrey P. Koplow Sean W. Moore Arlee V. Smith 《Optics Communications》2002,210(3-6):393-398
We report generation of the second, third, fourth, and fifth harmonics of the output of a Yb-doped fiber amplifier seeded by a passively Q-switched Nd:YAG microchip laser. We obtained high conversion efficiencies using a simple optical arrangement and critically phase-matched nonlinear crystals. Starting with 320 mW of average power at 1064 nm (86 μJ per pulse at a 3.7 kHz repetition rate), we generated 160 mW at 532 nm, 38 mW at 355 nm, 69 mW at 266 nm, and 18 mW at 213 nm. The experimental results are in excellent agreement with calculations. 相似文献