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111.
Effect of Acid Treatment of Montmorillonite on “Support‐Activator” Performance to Support Metallocene for Propylene Polymerization Catalyst 下载免费PDF全文
Takao Tayano Hideshi Uchino Takehiro Sagae Katsuyuki Yokomizo Koji Nakayama Shigeki Ohta Hiroshi Nakano Masahide Murata 《大分子反应工程》2017,11(2)
This work is focused on montmorillonite (MMT)‐based “support‐activators” (S‐As) for the metallocene‐catalyzed propylene polymerization. This catalyst was previously industrialized; however, for further technological advances, the activation mechanism is investigated. The chemical and morphological requirements of the S‐A are surveyed using both commercially available raw clay minerals (non‐acid‐treated) and acid‐treated clay minerals. The S‐A possessing strong‐acid sites (pK a < ?8.2) gives a highly active catalyst. Acid treatment of MMT induces morphological changes as well as the formation of strong acid sites. Based on pore size distribution analysis and atomic force microscopy observations, it is concluded that the strong acid sites are located in the small pores around the edge of the clay mineral (not in the interlayer), where the structure is disordered by the acid treatment.
112.
Yorihiko Sasaki Shigehiro Konaka Takao Iijima Masao Kimura 《International journal of quantum chemistry》1982,21(2):475-485
The total (elastic and inelastic) intensity of electrons scattered by CO2 was measured in the s range of 1 to 12 Å?1 and compared with the theoretical intensity calculated from the Hartree-Fock molecular wave function and those calculated for the independent-atom-model (IAM ) molecule. In the range of s ? 4 Å?1 the electron correlation effect on the total scattered intensity was found to be represented by that for the IAM molecule. 相似文献
113.
Takashi Fujita Takao Yoshioka 《Journal of polymer science. Part A, Polymer chemistry》1982,20(6):1639-1647
Copolymerization of N-oxyl biradical with α-chloro-p-xylylene was carried out by varying the feed ratio of α,α′-dichloro-p-xylene which was the precursor of α-chloro-p-xylylene. The structures of the obtained copolymers were determined spectroscopically. The results that the N-oxyl attacked the carbon-bearing chlorine atom of α-chloro-p-xylylene suggest a nucleophilic reactivity of N-oxyl radical. The copolymerization process was also discussed. 相似文献
114.
In this paper we investigate linear three-term recurrence formulae with sequences of integers (T(n))n?0 and (U(n))n?0, which are ultimately periodic modulo m, e.g.
115.
Takao Watanabe 《Monatshefte für Mathematik》2006,61(5):155-172
We generalize the notion of successive minima, Minkowski’s second theorem and Siegel’s lemma to a free module over a simple
algebra whose center is a global field. 相似文献
116.
In this paper we determine the topology of three-dimensional complete orientable Riemannian manifolds with a uniform lower bound of sectional curvature whose volume is sufficiently small. 相似文献
117.
Takao Yamazaki 《Mathematische Zeitschrift》2009,261(1):109-121
We prove that the kernel of the reciprocity map for a product of curves over a p-adic field with split semi-stable reduction is divisible. We also consider the K
1 of a product of curves over a number field.
相似文献
118.
Xiao Zhou Hitoshi Suzuki Takao Nishizeki 《Journal of Algorithms in Cognition, Informatics and Logic》1997,23(2):359-374
Many combinatorial problems can be efficiently solved in parallel for series–parallel multigraphs. The edge-coloring problem is one of a few combinatorial problems for which no NC parallel algorithm has been obtained for series–parallel multigraphs. This paper gives an NC parallel algorithm for the problem on series–parallel multigraphsG. It takesO(log n) time withO(Δn/log n) processors, wherenis the number of vertices and Δ is the maximum degree ofG. 相似文献
119.
A total coloring of a graph G is a coloring of all elements of G, i.e. vertices and edges, such that no two adjacent or incident elements receive the same color. A graph G is s-degenerate for a positive integer s if G can be reduced to a trivial graph by successive removal of vertices with degree ≤s. We prove that an s-degenerate graph G has a total coloring with Δ+1 colors if the maximum degree Δ of G is sufficiently large, say Δ≥4s+3. Our proof yields an efficient algorithm to find such a total coloring. We also give a lineartime algorithm to find a total
coloring of a graph G with the minimum number of colors if G is a partial k-tree, that is, the tree-width of G is bounded by a fixed integer k. 相似文献
120.
For a smooth projective irreducible algebraic curve C of odd gonality, the maximal possible dimension of the variety of special linear systems W
d
r
(C) is d-3r by a result of M. Coppens et al. Furthermore it is known that if the maximum dimension of W(C) for a curve C of odd gonality is attained then C is of very special type of curves by the recent progress made by G. Martens. The purpose of this paper is to chase an extension of the result of G. Martens; if dim W(C)=d-3r-1 for a curve C of odd gonality for some dg-4 and r1, then C must be either a smooth plane sextic, a pentagonal curve of bounded genus or a smooth plane octic. 相似文献