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排序方式: 共有137条查询结果,搜索用时 140 毫秒
91.
Sebastian Kunze Philipp Grosse Dr. Miguel Bernal Lopez Dr. Ilya Sinev Dr. Ioannis Zegkinoglou Dr. Hemma Mistry Dr. Janis Timoshenko Michael Y. Hu Jiyong Zhao Ercan E. Alp Dr. See Wee Chee Prof. Beatriz Roldan Cuenya 《Angewandte Chemie (Weinheim an der Bergstrasse, Germany)》2020,132(50):22856-22863
Operando nuclear resonant inelastic X-ray scattering (NRIXS) and X-ray absorption fine-structure spectroscopy (XAFS) measurements were used to gain insight into the structure and surface composition of FeCu and FeAg nanoparticles (NPs) during the electrochemical CO2 reduction (CO2RR) and to extract correlations with their catalytic activity and selectivity. The formation of a core–shell structure during CO2RR for FeAg NPs was inferred from the analysis of the operando NRIXS data (phonon density of states, PDOS) and XAFS measurements. Electrochemical analysis of the FeAg NPs revealed a faradaic selectivity of 36 % for CO in 0.1 M KHCO3 at −1.1 V vs. RHE, similar to that of pure Ag NPs. In contrast, a predominant selectivity towards H2 evolution is obtained in the case of the FeCu NPs, analogous to the results obtained for pure Fe NPs, although small Cu NPs have also been shown to favor H2 production. 相似文献
92.
93.
T. Mocek B. Rus M. Kozlová J. Polan P. Homer K. Jakubczak M. Stupka D. Snopek J. Nejdl M. H. Edwards D. S. Whittaker G. J. Tallents P. Mistry G. J. Pert N. Booth Z. Zhai M. Fajardo P. Zeitoun J. Chalupsky V. Hájková L. Juha 《The European Physical Journal D - Atomic, Molecular, Optical and Plasma Physics》2009,54(2):439-444
An overview of recent advances in applications of currently the most energetic X-ray laser at 21 nm is given. The unique parameters
of this half-cavity based X-ray laser such as record output energy of 10 mJ, highly symmetric beam, robustness and reproducibility,
have made it possible to carry out a number of multidisciplinary scientific projects featuring novel applications of intense
coherent X-ray radiation. Selected results obtained in these experiments are reviewed, including X-ray laser probing of dense
plasmas, measurements of transmission of focused soft X-ray radiation at intensities of up to 1012 W cm-2, measurements of infrared laser ablation rates of thin foils, and ablative microstructuring of solids. 相似文献
94.
Csorna SE Danko I McLean KW Xu Z Godang R Bonvicini G Cinabro D Dubrovin M McGee S Zhou GJ Bornheim A Lipeles E Pappas SP Schmidtler M Shapiro A Sun WM Weinstein AJ Jaffe DE Masek G Paar HP Asner DM Eppich A Hill TS Morrison RJ Briere RA Chen GP Ferguson T Vogel H Gritsan A Alexander JP Baker R Bebek C Berger BE Berkelman K Blanc F Boisvert V Cassel DG Drell PS Duboscq JE Ecklund KM Ehrlich R Foland AD Gaidarev P Galik RS Gibbons L Gittelman B Gray SW Hartill DL Heltsley BK Hopman PI Hsu L 《Physical review letters》2001,86(19):4243-4246
Using 13.7 fb(-1) of data recorded by the CLEO detector at Cornell Electron Storage Ring, we report evidence of two new charmed baryons: one decaying into Xi(0')(c)pi(+) with the subsequent decay Xi(0')(c)-->Xi(0)(c)gamma, and its isospin partner decaying into Xi(+')(c)pi(-) followed by Xi(+')(c)-->Xi(+)(c)gamma. We measure the following mass differences for the two states: M(Xi(0)(c)gammapi(+))-M(Xi(0)(c)) = 318.2+/-1.3+/-2.9 MeV and M(Xi(+)(c)gammapi(-))-M(Xi(+)(c)) = 324.0+/-1.3+/-3.0 MeV. We interpret these new states as the J(P) = 1 / 2(-) Xi(c1) particles, the charmed-strange analogs of the Lambda(+)(c1)(2593). 相似文献
95.
Bonvicini G Cinabro D Dubrovin M McGee S Bornheim A Lipeles E Pappas SP Shapiro A Sun WM Weinstein AJ Masek G Paar HP Mahapatra R Morrison RJ Briere RA Chen GP Ferguson T Tatishvili G Vogel H Adam NE Alexander JP Bebek C Berkelman K Blanc F Boisvert V Cassel DG Drell PS Duboscq JE Ecklund KM Ehrlich R Gibbons L Gittelman B Gray SW Hartill DL Heltsley BK Hsu L Jones CD Kandaswamy J Kreinick DL Magerkurth A Mahlke-Krüger H Meyer TO Mistry NB Nordberg E Palmer M Patterson JR Peterson D Pivarski J 《Physical review letters》2002,88(11):111803
We search and find no evidence for CP violation in tau decays into the K(pi)nu(tau) final state. We provide limits on the imaginary part of the coupling constant Lambda describing a relative contribution of the CP violating processes with respect to the standard model to be -0.172相似文献
96.
Briere RA Chen GP Ferguson T Tatishvili G Vogel H Adam NE Alexander JP Berkelman K Boisvert V Cassel DG Drell PS Duboscq JE Ecklund KM Ehrlich R Galik RS Gibbons L Gittelman B Gray SW Hartill DL Heltsley BK Hsu L Jones CD Kandaswamy J Kreinick DL Magerkurth A Mahlke-Krüger H Meyer TO Mistry NB Patterson JR Peterson D Pivarski J Richichi SJ Riley D Sadoff AJ Schwarthoff H Shepherd MR Thayer JG Urner D Wilksen T Warburton A Weinberger M Athar SB Avery P Breva-Newell L Potlia V Stoeck H Yelton J 《Physical review letters》2003,90(18):181802
From electron-positron collision data collected with the CLEO detector operating at Cornell Electron Storage Ring near sqrt[s]=10.6 GeV, improved measurements of the branching fractions for tau decays into three explicitly identified hadrons and a neutrino are presented as B(tau(-)-->pi(-)pi(+)pi(-)nu(tau))=(9.13+/-0.05+/-0.46)%, B(tau(-)-->K-pi(+)pi(-)nu(tau))=(3.84+/-0.14+/-0.38) x 10(-3), B(tau(-)-->K-K+pi(-)nu(tau))=(1.55+/-0.06+/-0.09) x 10(-3), and B(tau(-)-->K-K+K-nu(tau))<3.7 x 10(-5) at 90% C.L., where the uncertainties are statistical and systematic, respectively. 相似文献
97.
We report the successful size-based separations of large, neutral polysaccharides using capillary electrochromatography (CEC). As the polysaccharides possessed little chromophore for photometric detection, two separate approaches were taken. In the first approach, indirect detection was combined with size-exclusion chromatography using a sulfonated polystyrene/divinylbenzene stationary phase. The separations were performed using a 300 A pore size stationary phase under aqueous conditions. Non-size based interactions were minimal using this material, resulting in an effective calibration range of molecular masses 180 to 112 000 g.mol(-1) for pullulans. In the second approach, the polysaccharides were derivatized with phenylisocyanate and were subsequently separated on columns made using a combination of high capacity ion-exchanger and a neutral polystyrene/divinylbenzene material of various pore sizes. The sulfonated ion-exchange phase provided the electroosmotic flow, while the mixed pore size material provided the extended calibration range. The linear range for this primarily nonaqueous system using tetrahydrofuran was determined to be from molecular masses 738 to 404 000 g.mol(-1) of the original, untagged pullulan. This approach overcame the limited solubility issue associated with analysis of some polysaccharides. Analysis of pullulan and amylose samples by CEC correlated well with results obtained by conventional high-performance liquid chromatography (HPLC). The size-exclusion electrochromatographic separations provide an alternative mode for determining the relative molecular weights of polysaccharides with reduced sample and solvent consumption, as well as analysis times. 相似文献
98.
99.
Alam MS Katayama N Kim IJ Li WC Lou XC Sun CR Tanikella V Bortoletto D Chen A Goldberg M Holmes R Horwitz N Jawahery A Lubrano P Moneti GC Sharma V Shipsey IP Thoma P Csorna SE Mestayer MD Panvini RS Word GB Bean A Bobbink GJ Brock IC Engler A Ferguson T Kraemer RW Rippich C Vogel H Bebek C Berkelman K Blucher E Cassel DG Copie T DeSalvo R DeWire JW Ehrlich R Galik RS Gilchriese MG Gittleman B Gray SW Halling AM Hartill DL Heltsley BK Holzner S Kandaswamy J Kowalewski R Kreinick DL Kubota Y 《Physical review letters》1987,59(1):22-25
100.
Behrends S Guida JM Guida JA Morrow F Poling R Thorndike EH Tipton P Alam MS Katayama N Kim IJ Li WC Lou XC Sun CR Tanikella V Bortoletto D Chen A Goldberg M Holmes R Horwitz N Jawahery A Lubrano P Moneti GC Sharma V Shipsey IP Thoma P Csorna SE Mestayer MD Panvini RS Word GB Bean A Bobbink GJ Brock IC Engler A Ferguson T Kraemer RW Rippich C Vogel H Bebek C Berkelman K Blucher E Cassel DG Copie T DeSalvo R DeWire JW Ehrlich R Galik RS Gilchriese MG Gittelman B Gray SW Halling AM Hartill DL 《Physical review letters》1987,59(4):407-410