NMR on short-lived beta-emitter43Ti using new fragment separator at LBL

The lifetime and magnetic moment of⁴³Ti (I^π-7/2⁻, T_1/2=0.50 sec), one of the mirror beta-radioactive nuclei in the f_7/2-shell, have been measured with a fragment separator built at the Bevalac of the LBL. By means of the beta-NMR method on⁴³Ti, a preliminary value of the magnetic moment of⁴³Ti was determined to be μ=(0.70±0.07) μ_π.     

Quadrupole moment of the doubly closed shell +1 nucleon nucleus41Sc(Iπ=7/2−)

The nuclear electric quadrupole moment of⁴¹Sc(I^π=7/2⁻) was experimentally determined by use of the NMR detection in which the asymmetric β-ray distribution from spin polarized nuclei was monitored. The magnetic interaction of the state with high external magnetic field and the nuclear quadrupole interaction with the electric field gradient obtained in TiO₂ crystal were studied. The field gradient seen to the implanted⁴¹Sc was measured independently by the high field NMR detection on the stable isotope⁴⁵Sc located in the equivalent⁴¹Sc site with. |Q(⁴¹Sc;I^π=7/2⁻)|=(0.120±0.006) b was determined.     

Electromagnetic moments of the beta-emitting nucleus 16N

The nuclear magnetic dipole moment mu and electric quadrupole moment Q of the beta-emitting 16N(Ipi = 2(-), T(1/2) = 7.13 s) nucleus have been determined for the first time by detecting its beta-NMR in a MgO crystal and beta-NQR (nuclear quadrupole resonance) in a TiO (2) crystal to be /mu/ = (1.9859+/-0.0011) mu(N) and /Q/ = (17.9+/-1.7) mb, respectively. Although the prediction of mu given by the Hartree-Fock calculation agrees well with the experiment, an abnormally small effective charge for neutrons is required to account for the experimental Q.     

β-Ray angular distribution from purely nuclear spin aligned 20F

The alignment correlation term in the β-ray angular distribution from purely nuclear spin aligned ²⁰F has been measured to test the G-parity conservation law which is one of the fundamental symmetries in the weak nucleon current. We utilized the hyperfine interaction of ²⁰F in an MgF₂ single crystal and successfully created the pure alignment from the polarization by means of the spin manipulation technique based on the β-NMR method.     

Magnetic moment of short lived β-emitter 24mAl

The magnetic moment of short lived β-emitter ^24mAl (426 keV, I ^π ?=?1^?+?, T _1/2?=?131 ms) has been measured by means of β-NMR technique, for the first time. From the β-NMR spectrum, the magnetic moment was determined as $\left| {\upmu}\left( ^{\rm 24m}{\rm Al} \right) \right|=\left( {2.99\pm 0.09} \right){\upmu}_{\rm N}$ . Combined with the known magnetic moment of the mirror partner ^24mNa, the expectation value of <?S _z?> is obtained to be (0.08 ± 0.12). These values are reproduced well by the shell model calculation.     

Polarization of 23Ne, 24m,25Al and 28P produced through single nucleon pickup and charge-exchange reactions at 100 AMeV

We measured the polarization of the $\upbeta $ -emitting ²³Ne (I ^π ?= 5/2^?+?, T _1/2?= 37.24 s) and ²⁵Al(I ^π ?= 5/2^?+?, T _1/2?= 7.18 s) produced through the one nucleon pickup reactions and ^24mAl(I ^π ?= 1^?+?, T _1/2?= 131 ms, E _ex?= 426 keV) and ²⁸P(I ^π ?= 3^?+?, T _1/2?= 270 ms) produced through charge-exchange reactions in the intermediate energy heavy ion collisions. We compared them with those from the projectile fragmentation process. The larger polarization seems to persistently be positive throughout the momentum distribution, and sharper momentum distributions suggest that nuclear friction mechanism is responsible for the polarization phenomena.     

Hyperfine interactions of 19O in TiO2 and quadrupole moments of 13,19O

The electric quadrupole interaction of ¹⁹O(I^π=(5/2)⁺, T_1/2=27.0 s) in TiO₂ single crystal was studied in detail by means of the β-NQR to determine the electric quadrupole moments Q of short-lived β-emitting nuclei ¹⁹O and ¹³O(I^π=(3/2)^-, T_1/2=8.6 ms). Two implantation sites were found for the implanted O nucleus and the quadrupole coupling constants of ¹⁹O at these sites were determined. We observed FT-NMR of the enriched stable isotope ¹⁷O in TiO₂ and obtained the electric field gradient (EFG) at the oxygen substitutional site. With this knowledge, we have determined Q(¹³O)=11.0 ± 1.3 mb and Q(¹⁹O)=3.7 ± 0.4 mb. The present results are compared with the theoretical values calculated by the shell model code, OXBASH and by the Hartree–Fock calculation with the realistic potential. This revised version was published online in August 2006 with corrections to the Cover Date.     

Ab initio calculations of electric field gradients detected by impurities in TiO2, Al2O3 and CaCO3

We present ab initio calculations of electric field gradients (EFGs) at impurity sites in ionic crystals TiO₂, Al₂O₃ and CaCO₃. The electronic structure was calculated self-consistently by the KKR method in the framework of the local spin density approximation of the density functional theory. The system with a single impurity was simulated by the super cell method. It was found that EFGs for the transition metal impurities (Sc, Nb, Cd and Ta) in TiO₂ were well reproduced by the calculations if the charge state of them in TiO₂ was taken into account. The present method was applied to the determination of the implantation sites of N and O nuclei in TiO₂. The calculation of EFGs at a Si impurity in Al₂O₃ and at Ca site in CaCO₃ were used to derive the quadrupole moments of ²⁷Si and ³⁹Ca from their quadrupole coupling constants. This revised version was published online in August 2006 with corrections to the Cover Date.     

Knight shifts for short-lived β emitters in Pt

The Knight shifts K for short-lived β emitters ¹²N and ²⁷Si implanted in Pt have been measured by means of β-NMR technique. The results were K(¹²N in Pt)= +(5.8 ± 2.1)× 10^-4 and K(²⁷Si in Pt)= +(1.4 ± 0.8)× 10^-3. The spin–lattice relaxation time T₁ was measured for ¹²N in Pt. The result was T₁(¹²N in Pt, T=300 K)= 66 ± 8 ms, thus, T₁T= 20 ± 2 Ks. The present Knight shifts are in good agreement with the KKR band structure calculation with local lattice relaxation determined theoretically. This revised version was published online in August 2006 with corrections to the Cover Date.