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11.
The exciton-exciton interaction is investigated for spatially indirect excitons in coupled quantum wells. The Hartree-Fock and Heitler-London approaches are improved by a full two-exciton calculation including the van der Waals effect. Using these potentials for the singlet and triplet channel, the two-body scattering matrix is calculated and employed to derive a modified relation between exciton density and blue shift. Such a relation is of central importance for gauging exciton densities on the way toward Bose condensation. 相似文献
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Roland A. Fischer Heinz-Josef Kneuper Wolfgang A. Hermann 《Journal of organometallic chemistry》1987,330(3):365-376
Hydrogenchalcogenido complexes of general composition (η5-C5R5)(CO)3M(EH) (R = H, CH3; M = Cr, Mo, W; E = S, Se) can be obtained by three different routes, sometimes in quite good yields. Thus, the sulfur and selenium derivatives can be synthesized by insertion of the respective elements into the metal-hydrogen bonds of the precursor compounds (η5-C5R5)(CO)3MH. This species also reacts with potassium selenocyanate to yield the hydrogenselenido derivatives (η5-C5R5)(CO)3M(SeH) which can also be obtained by treatment of the methyl complexes (η5-C5R5)(CO)3M(CH3 (M = Mo, W) with HBF4 and Li[SeH]. The corresponding hydrogentellurido compounds are probably formed by these preparative methods but appear to be quickly converted into either the dinuclear tellurium bridge products (μ-Te)[(η5-C5R5)(CO)3M]2 (M = Mo) or into the hydrido complexes (η5-C5R5)(CO)3MH (M= Mo, W) by release of elemental tellurium. 相似文献
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Roland Opfer 《Advances in Computational Mathematics》2006,25(4):357-380
This paper reconstructs multivariate functions from scattered data by a new multiscale technique. The reconstruction uses
standard methods of interpolation by positive definite reproducing kernels in Hilbert spaces. But it adopts techniques from
wavelet theory and shift-invariant spaces to construct a new class of kernels as multiscale superpositions of shifts and scales
of a single compactly supported function φ. This means that the advantages of scaled regular grids are used to construct the
kernels, while the advantages of unrestricted scattered data interpolation are maintained after the kernels are constructed.
Using such a multiscale kernel, the reconstruction method interpolates at given scattered data. No manipulations of the data
(e.g., thinning or separation into subsets of certain scales) are needed. Then, the multiscale structure of the kernel allows
to represent the interpolant on regular grids on all scales involved, with cheap evaluation due to the compact support of
the function φ, and with a recursive evaluation technique if φ is chosen to be refinable. There also is a wavelet-like data
reduction effect, if a suitable thresholding strategy is applied to the coefficients of the interpolant when represented over
a scaled grid. Various numerical examples are presented, illustrating the multiresolution and data compression effects. 相似文献
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Spectroscopic determinations of the concentrations associated with the onset of intermolecular interaction in solutions of poly(ethylene terephthalate) (PET) are described. The intersegment forces perturb the electronic spectra and induce ground-state aggregation. These phenomena become observable at different chain densities, reflecting the influence of concentration on the coil dimensions, as well as the dynamical nature of the interactions. An estimate of the equilibrium constant for PET dimer formation in hexafluoroisopropanol is reported. 相似文献
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