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881.
ZOU XiaoChuan CHEN ShaoCheng REN YanRong SHI KaiYun LI Jun & FU XiangKai 《中国科学:化学(英文版)》2012,(11):2397-2407
Chiral Mn Ⅲ (salen) (Jacobsen’s catalyst) was axially immobilized onto a new type of organic polymer-inorganic hybrid materialzirconium poly(styrene-isopropenyl phosphonate)-phosphate(ZPS-IPPA) with different linkage lengths and evaluated as catalysts for the epoxidation of unfunctionalized olefins. The results demonstrated that the prepared catalysts exhibited moderate to good activity and enantioselectivity in the asymmetric epoxidation of unfunctionalized olefins. Furthermore, the immobilized catalysts were relatively stable and could be conveniently separated from the reaction system by simple precipitation in hexane. Moreover, higher enantioselectivity was obtained with catalyst 2c than that of homogeneous counterpart catalyzed even after eight times. The excellent recycling of the catalyst was attributed to its structure feature of ZPS-IPPA which is different from either pure polystyrene or pure zirconium phosphates. 相似文献
882.
Yong Zhang 《Journal of statistical physics》2010,139(5):915-939
This paper develops moment formulas for exponentially tempered, fractional advection-diffusion equations (TFADEs) that transition
from anomalous to asymptotic diffusion limits over time. Exact analytical expressions or series representations for spatial
moments up to the fourth order are derived by integral transform or asymptotic expansion approach. A fully Lagrangian solver,
cross verified by an implicit Eulerian approach, is also developed to calculate numerically the complete evolution of moments
for the TFADEs with complex initial and boundary conditions. Moment analysis identifies the diffusion equation that attracts
the tempered anomalous diffusion in the long time limit. Fitting of moments measured at two end members of alluvial systems
checks the applicability of moment analysis in understanding real diffusion. 相似文献
883.
Yong He 《Optics Communications》2010,283(7):1558-1560
We propose a scheme to generate a type of genuine four-qubit entangled states, which were firstly introduced by Yeo et al. [Y. Yeo, W. K. Chua, Phys. Rev. Lett. 96 (2006) 060502]. These states have many interesting entanglement properties and possess possible applications in quantum information processing and in fundamental tests of quantum physics. We show that such a type of 16 orthonormal basis states can be deterministically distinguished by a cavity QED system. 相似文献
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887.
Environmental Impacts on Spiking Properties in Hodgkin-Huxley Neuron with Direct Current Stimulus
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Based on the well accepted Hodgkin-Huxley neuron model, the neuronal intrinsic excitability is studied when the neuron is subject to varying environmental temperatures, the typical impact for its regulating ways. With computer simulation, it is found that altering environmental temperature can improve or inhibit the neuronal intrinsic excitability so as to influence the neuronal spiking properties. The impacts from environmental factors can be understood that,the neuronal spiking threshold is essentially influenced by the fluctuations in the environment. With the environmental temperature varying, burst spiking is realized for the neuronal membrane voltage because of the environment-dependent spiking threshold. This burst induced by changes in spiking threshold is different from that excited by input currents or other stimulus. 相似文献
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We thank all the discussants for their interesting and stimulating contributions. They have touched various aspects that have not been considered by the original articles. 相似文献
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An analysis is performed to study the free convection of a dusty‐gas flow along a semi‐infinite isothermal vertical cylinder. The governing equations of the flow problem are transformed into non‐dimensional form and the resulting nonlinear, coupled parabolic partial differential equations have been solved numerically using an implicit finite difference scheme of Crank–Nicholson type. The flow variables such as gas–velocity, dust‐particle velocity and temperature, shearing stress and heat transfer coefficients are calculated numerically for various parameters occurring in the problem. It is observed that due to the presence of dust particles, the gas velocity is found to decrease. Copyright © 2009 John Wiley & Sons, Ltd. 相似文献
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