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91.
S. Fujita J.P. Riley C.C. Chen Ching-Lung Ko C.S. Raju T. Yamaguchi 《Journal of Physics and Chemistry of Solids》1973,34(12):2075-2089
The correlation function formula for the dynamic conductivity of a system of non-interacting electrons in the field of impurities is analyzed in terms of proper connected diagrams. By selecting those diagrams appropriate in the region of weak coupling and low impurity concentration, a set of coupled equations for the energy broadening γ (ω, ε, ns) and the energy shift Δ(ω, ε, ns) is derived, where both γ and Δ depend on the frequency ω of a probing field, the energy ε of the electron, and the concentration, ng, of impurities. With the assumption of a finite range potential, these equations are solved. It is found that γ (ω, ns) is smaller than that extrapolated value which the conventional expression γ0 for the low-concentration collision frequency would predict, in the entire region studied, that the difference γ0-γ becomes appreciable when the ratio of the average time between scatterings, τc, to the average duration of a scattering, τd, is 100 or less, that γ (ω, ns) decreases monotonically from its static value γ (0, ns), and becomes vanishingly small in the region ω≈1/τd, and that in the static limit (ω=0), γ=γ0[1?(2/π) (γ0τd)+…], that the energy shift Δ is positive, and increases from 0 and reach a peak of magnitude γ0 as ω is raised from 0. By using the γ and Δ obtained, the dynamic conductivity σ(ω, ns) for degenerated electrons is calculated. The deviation, σ-σ0, from the conventional expression σ0=(?i) (nee2/M) [ω-iΓ0]?1, (ne]=number density of electrons), for 0°K, is appreciable when the ratio τc/τd is 100 or less. The field-term correction, which arises from the modification of the scattering due to the probing field, is found to be negligible in the entire region studied. 相似文献
92.
M.J. Campbell J. Liesegang J.D. Riley R.C.G. Leckey J.G. Jenkin R.T. Poole 《Journal of Electron Spectroscopy and Related Phenomena》1979,15(1):83-90
The results of a photoelectron study using ultraviolet 40.81 eV photons (UPS) of the outermost bands of the molecular solids NH3 and H2O are reported. The binding energies, the energy separation, the band widths and the branching ratio of the two outermost bands of solid NH3 are found not to be significantly different from the 3al and 1e molecular orbital states of the gaseous NH3 UPS spectrum. This implies that hydrogen bonding has not produced any significant change in the electronic structure of the valence bands of solid NH3. Because of a much smaller intermolecular hydrogen bond length in solid H2O compared to that in solid NH3, the hydrogen bond does, however, produce a significant change in the valence bands of H2O on solidification, and because of the orbital geometry it predominantly affects the 3al molecular orbital state. 相似文献
93.
A heterogeneous reduction method is described for the determination of nitrate in sea water. Nitrate is reduced to nitrite with 91% efficiency by passing the water through a column of amalgamated cadmium filings. The nitrite produced is determined spectrophotometrically by the method of BENDSCHNEIDER and ROBINSON. The method has a coefficient of variation of ca. 2% and is free from salt error. Temperature in the range o°–35° has no effect on the reduction. Interference from nitrite is discussed and a method is described for its destruction if necessary. Sulphide does not interfere. 相似文献
94.
95.
Methods are described for the microscale analysis of aquatic and sedimentary humic substances for several oxygen-containing functional groups including total acidity, carboxylic and phenolic hydroxyl groups, quinone groups and hydroxamate linkages. Coefficients of variation of the methods range from 4.9 to 12.9%. 相似文献
96.
A spectrophotometric procedure, which has a coefficient of variation of ca. 2%, is described for the determination of up to 80 μg of cerium. Ceric ion formed by oxidation with persulphate, in the presence of catalytic amounts of silver, is reduced to the cerous state by treatment with excess ferrous-phenanthroline reagent. The decrease in optical density of the ferrous-phenan-throline compared with the reagent blank is a measure of the amount of cerium present. The only common cations which cause serious interference are Mn+2and Cr+3. 相似文献
97.
C.G. Cassapakis H.C. Bryant B.D. Dieterle C.P. Leavitt D.M. Wolfe B.E. Bonner J.E. Simmons C.W. Bjork P.J. Riley M.L. Evans G. Glass J.C. Hiebert M. Jain R.A. Kenefick L.C. Northcliffe D.W. Werren 《Physics letters. [Part B]》1976,63(1):35-38
The measured cross sections show a narrow high-energy peak (20–30 MeV/cFWHM) and a broad bump at lower momenta associated with pion production. Comparison is made to an intranuclear cascade calculation. 相似文献
98.
Technetium-99 is preconcentrated from acidified seawater containing a trace of bromine by adsorbing it as the pertechnetate ion on the anion exchanger Duolite A101D. After elution with 4 M nitric acid, it is purified from other radionuclides by scavenging with hydrous iron(III) oxide and extracting from 5 M sodium hydroxide medium into methyl ethyl ketone. The organic phase is then evaporated and technetium is electrodeposited from oxalic acid medium onto a bronze disc and counted with a low background β-counter. Overall recovery is > 90% and the precision is ±0.2 pCi l-1 at a technetium level of 0.6–1.0 pCi l-1. Concentrations of the radionuclide in the central Irish Sea were found to lie in the range 0.4–2 pCi l-1. The same analytical scheme can be used for determining the element in nitric acid digests of marine algae. 相似文献
99.
Rosner JL Adam NE Alexander JP Berkelman K Cassel DG Duboscq JE Ecklund KM Ehrlich R Fields L Galik RS Gibbons L Gray R Gray SW Hartill DL Heltsley BK Hertz D Jones CD Kandaswamy J Kreinick DL Kuznetsov VE Mahlke-Krüger H Meyer TO Onyisi PU Patterson JR Peterson D Phillips EA Pivarski J Riley D Ryd A Sadoff AJ Schwarthoff H Shi X Stroiney S Sun WM Wilksen T Weinberger M Athar SB Avery P Breva-Newell L Patel R Potlia V Stoeck H Yelton J Rubin P Cawlfield C Eisenstein BI Karliner I Kim D Lowrey N 《Physical review letters》2006,96(9):092003
We determine the dielectron widths of the Gamma(1S), Gamma(2S), and Gamma(3S) resonances with better than 2% precision by integrating the cross section of e+e- -->Gamma over the e+e- center-of-mass energy. Using e+e- energy scans of the Gamma resonances at the Cornell Electron Storage Ring and measuring Gamma production with the CLEO detector, we find dielectron widths of 1.252+/-0.004(sigma(stat))+/-0.019(sigma(syst)) keV, 0.581+/-0.004+/-0.009 keV, and 0.413+/-0.004+/-0.006 keV for the Gamma(1S), Gamma(2S), and Gamma(3S), respectively. 相似文献
100.
Adam NE Alexander JP Berkelman K Cassel DG Crede V Duboscq JE Ecklund KM Ehrlich R Fields L Galik RS Gibbons L Gittelman B Gray R Gray SW Hartill DL Heltsley BK Hertz D Jones CD Kandaswamy J Kreinick DL Kuznetsov VE Mahlke-Krüger H Meyer TO Onyisi PU Patterson JR Peterson D Phillips EA Pivarski J Riley D Ryd A Sadoff AJ Schwarthoff H Shi X Shepherd MR Stroiney S Sun WM Urner D Wilksen T Weaver KM Weinberger M Athar SB Avery P Breva-Newell L Patel R Potlia V Stoeck H Yelton J Rubin P Cawlfield C 《Physical review letters》2006,96(8):082004
We observe signals for the decays psi(3770) --> XJ/psi from data acquired with the CLEO detector operating at the CESR e+ e- collider with square root of s = 3773 MeV. We measure the following branching fractions Beta(psi(3770) --> XJ/psi and significances: (189 +/- 20 +/- 20) x 10(-5) (11.6sigma) for X = pi+ pi-, (80 +/- 25 +/- 16) x 10(-5) (3.4sigma) for X = pi0 pi0, and (87 +/- 33 +/- 22) x 10(-5) (3.5sigma) for X = eta, where the errors are statistical and systematic, respectively. The radiative return process e+ e- --> gamma psi(2S) populates the same event sample and is used to measure Gamma ee[psi(2S)] = (2.54 +/- 0.03 +/- 0.11) keV. 相似文献