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91.
Jorio A Dresselhaus G Dresselhaus MS Souza M Dantas MS Pimenta MA Rao AM Saito R Liu C Cheng HM 《Physical review letters》2000,85(12):2617-2620
Polarized Raman spectra were obtained from a rope of aligned semiconducting single-wall nanotubes (SWNTs) in the vicinity of the D band and the G band. Based on group theory analysis and related theoretical predictions, the G-band profile was deconvolved into four intrinsic SWNT components with the following symmetry assignments: 1549 cm(-1) [E2(E(2g))], 1567 cm(-1) [A(A(1g))+E1(E(1g))], 1590 cm(-1) [A(A(1g))+E1(E(1g))] and 1607 cm(-1) [E2(E(2g))]. The frequency shifts of the tangential G modes from the 2D graphitelike E(2g(2)) frequency are discussed in terms of the nanotube geometry. 相似文献
92.
M. Mortier J. Y. Gesland M. Rousseau M. A. Pimenta L. O. Ladeira J. C. Machado Da Silva G. A. Barbosa 《Journal of Raman spectroscopy : JRS》1991,22(7):393-396
Single crystals of the fluoride compound KY3F10 (Oh5) were studied by Raman scattering from 40 to 950 K. Group theory analysis predicts 3A1g + 4Eg + 6F2g Raman-active modes, but the experimental spectra show two F2g modes missing. Over the whole temperature range the frequency shifts are negligible whereas the line widths show a strong increase with temperature. Both reversible and irreversible line width behaviour are exhibited for different temperature runs, indicating a complex microscopic phenomenon underlying the creation of defects responsible for these line widths and their interaction with the different phonon modes. An approximate activation energy for defect creation of ΔE ≈︁ 0.3 eV can be obtained from the temperature behaviour of the line widths. This activation energy may be connected with the high-temperature ionic conduction mentioned previously for this crystal. 相似文献
93.
Gustavo M. do Nascimento Wdeson P. Barros Yoong Ahm Kim Hiroyuki Muramatsu Takuya Hayashi Morinobu Endo Noriberto A. Pradie Cristiano Fantini Marcos A. Pimenta Mildred S. Dresselhaus Humberto O. Stumpf 《Journal of Raman spectroscopy : JRS》2012,43(12):1951-1956
The electronic interactions between the [Cu(opba)]2− anions (where opba is orthophenylenebis (oxamato)) and single‐wall carbon nanotubes (SWCNTs) were investigated by resonance Raman spectroscopy. The opba can form molecular magnets, and the interactions of opba with SWCNTs can produce materials with very different magnetic/electronic properties. It is observed that the electronic interaction shows a dependence on the SWCNT diameter independent of whether they are metallic or semiconducting, although the interaction is stronger for metallic tubes. The interaction also is dependent on the amount of complex that is probably adsorbed on the carbon surface of the SWCNTs. Some charge transfer can be also occurring between the metallic complex and the SWCNTs. Copyright © 2012 John Wiley & Sons, Ltd. 相似文献