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51.
Pau S Pai CS Low YL Moxom J Reilly PT Whitten WB Ramsey JM 《Physical review letters》2006,96(12):120801
An array of miniaturized cylindrical quadrupole ion traps, with a radius of 20 microm, is fabricated using silicon micromachining using phosphorus doped polysilicon and silicon dioxide for the purpose of creating a mass spectrometer on a chip. We have operated the array for mass-selective ion ejection and mass analysis using Xe ions at a pressure of 10(-4). The scaling rules for the ion trap in relation to operating pressure, voltage, and frequency are examined. 相似文献
52.
53.
Esen S Schwartz AJ Adachi I Aihara H Arinstein K Aulchenko V Aushev T Aziz T Bakich AM Balagura V Barberio E Bay A Bischofberger M Bondar A Bozek A Bračko M Browder TE Chang MC Chang P Chen A Chen P Cheon BG Chiang CC Choi Y Dalseno J Dash M Doležal Z Drásal Z Drutskoy A Eidelman S Goldenzweig P Golob B Ha H Haba J Hara T Hayasaka K Higuchi T Hoshi Y Hou WS Hsiung YB Hyun HJ Iijima T Inami K Itoh R Iwabuchi M Joshi NJ Julius T Kang JH Kawasaki T Kichimi H Kim HJ Kim HO Kim JH Kim YJ Kinoshita K 《Physical review letters》2010,105(20):201802
We have made the first observation of B(s)(0)→D(s)(*)+ D(s)(*)- decays using 23.6 fb(-1) of data recorded by the Belle experiment running on the Υ(5S) resonance. The branching fractions are measured to be B(B(s)(0)→D(s)+ D(s)-)=(1.03(-0.32-0.25)(+0.39+0.26))%, B(B(s)(0)→D(s)(*±) D(s)(?))=(2.75(-0.71)(+0.83)±0.69)%, and B(B(s)(0)→D(s)*+ D(s)*-)=(3.08(-1.04-0.86)(+1.22+0.85))%; the sum is B[B(s)(0)→D(s)(*)+ D(s)(*)-]=(6.85(-1.30-1.80)(+1.53+1.79))%. Assuming B(s)(0)→D(s)(*)+ D(s)(*)- saturates decays to CP-even final states, the branching fraction determines the ratio ΔΓ(s)/cosφ, where ΔΓ(s) is the difference in widths between the two B(s)-B(s) mass eigenstates, and φ is a CP-violating weak phase. Taking CP violation to be negligibly small, we obtain ΔΓ(s)/Γ(s)=0.147(-0.030)(+0.036)(stat)(-0.041)(+0.042)(syst), where Γ(s) is the mean decay width. 相似文献
54.
Zhang LM Zhang ZP Li J Abe K Abe K Adachi I Aihara H Anipko D Arinstein K Asano Y Aushev T Bahinipati S Bakich AM Balagura V Barbero M Bay A Bedny I Belous K Bitenc U Bizjak I Blyth S Bondar A Bozek A Bracko M Brodzicka J Browder TE Chang MC Chang P Chao Y Chen A Chen WT Cheon BG Chistov R Choi SK Choi Y Choi YK Chuvikov A Cole S Dalseno J Danilov M Dash M Drutskoy A Eidelman S Gabyshev N Gershon T Go A Gokhroo G Golob B Gorisek A Ha HC Haba J Hara T Hastings NC Hayasaka K Hayashii H Hazumi M 《Physical review letters》2006,96(15):151801
We report the results of a search for D0-D0 mixing in D0 --> K+ pi- decays based on 400 fb(-1) of data accumulated by the Belle detector at KEKB. Both assuming CP conservation and allowing for CP violation, we fit the decay-time distribution for the mixing parameters x and y, as well as for the parameter R(D), the ratio of doubly Cabibbo-suppressed decays to Cabibbo-favored decays. The 95% confidence level region in the (x'2,y') plane is obtained using a frequentist method. Assuming CP conservation, we find x'2 < 0.72 x 10(-3) and -9.9 x 10(-3) < y' < 6.8 x 10(-3) at the 95% confidence level; these are the most stringent constraints on the mixing parameters to date. The no-mixing point (0,0) has a confidence level of 3.9%. Assuming no mixing, we measure R(D) = (0.377 +/- 0.008 +/- 0.005)%. 相似文献
55.
We address the problem of determining membership in Schatten-Von Neumann ideals S p of integration operators (T g f)(z) = ∫ 0 z = ∫ 0 z f(ξ)g′(ξ)dξ acting on Dirichlet type spaces. We also study this problem for multiplication, Hankel and Toeplitz operators. In particular, we provide an extension of Luecking's result on Toeplitz operators [10, p. 347]. 相似文献
56.
Dr. Hua Tian Dr. Louis J. Sparvero Paul Blenkinsopp Dr. Andrew A. Amoscato Prof. Simon C. Watkins Prof. Hülya Bayır Prof. Valerian E. Kagan Prof. Nicholas Winograd 《Angewandte Chemie (Weinheim an der Bergstrasse, Germany)》2019,131(10):3188-3193
Millions of diverse molecules constituting the lipidome act as important signals within cells. Of these, cardiolipin (CL) and phosphatidylethanolamine (PE) participate in apoptosis and ferroptosis, respectively. Their subcellular distribution is largely unknown. Imaging mass spectrometry is capable of deciphering the spatial distribution of multiple lipids at subcellular levels. Here we report the development of a unique 70 keV gas-cluster ion beam that consists of (CO2)n+(n>10 000) projectiles. Coupled with direct current beam buncher-time-of-flight secondary-ion mass spectrometry, it is optimized for sensitivity towards high-mass species (up to m/z 3000) at high spatial resolution (1 μm). In combination with immunohistochemistry, phospholipids, including PE and CL, have been assessed in subcellular compartments of mouse hippocampal neuronal cells and rat brain tissue. 相似文献
57.
Brodzicka J Palka H Adachi I Aihara H Aulchenko V Bakich AM Barberio E Bay A Bedny I Bitenc U Bondar A Bracko M Browder TE Chang MC Chang P Chen A Chen WT Cheon BG Chiang CC Chistov R Cho IS Choi SK Choi Y Dalseno J Danilov M Dash M Drutskoy A Eidelman S Gabyshev N Go A Gokhroo G Golob B Ha H Haba J Hara T Hayasaka K Hayashii H Hazumi M Heffernan D Hoshi Y Hou WS Hyun HJ Iijima T Ikado K Inami K Ishikawa A Ishino H Itoh R Iwasaki M Iwasaki Y Joshi NJ Kah DH Kang JH Kawai H Kawasaki T Kichimi H 《Physical review letters》2008,100(9):092001
We report the observation of a new DsJ meson produced in B+-->D0DsJ-->D0D0K+. This state has a mass of M=2708+/-9(-10)(+11) MeV/c2, a width Gamma=108+/-23(-31)(+36) MeV/c2 and a 1- spin-parity. The statistical significance of this observation is 8.4 sigma. The results are based on an analysis of 449 x 10(6) BB events collected at the Upsilon(4S) resonance with the Belle detector at the KEKB asymmetric-energy e+e- collider. 相似文献
58.
Heteronuclear long-range scalar coupling constants (nJCH) are a valuable tool for solving problems in organic chemistry and are especially suited for stereochemical and configurational analyses of small molecules and natural products. This tutorial will focus on the step-by-step implementation of several 2D 1H frequency selective HSQMBC experiments for the easy and accurate measurement of either the magnitude or both the magnitude and the sign of long-range nJCH couplings. The performance of these experiments will be showcased with several scenarios in a range of different experimental conditions. 相似文献
59.
Kumar Motiram-Corral Dr. Alexandre A. Souza Dr. Josep Saurí Dr. Pau Nolis Dr. Teodor Parella 《Chemphyschem》2020,21(4):280-283
The optimum detection and accurate measurement of longer-range (4J and higher) heteronuclear NMR correlations is described. The magnitude and/or the sign of a wide range of large and small long-range couplings can be simultaneously determined for protonated and non-protonated 13C and 15N nuclei using the LR-selHSQMBC experiment. 相似文献
60.
Yuanyuan Lu Sílvia Alujas-Burgos Cristina Oliveras-González Laura Vázquez-Jiménez Pep Rojo Ángel Álvarez-Larena Pau Bayón Marta Figueredo 《Tetrahedron》2018,74(1):104-116
An enantioselective approach to substituted indolizidine and quinolizidine frameworks has been developed. Key steps of the synthesis are the enantioselective, palladium-catalyzed N-allylation of an imide, the nucleophilic allylation of an acyliminium ion and a ring closing metathesis. This general strategy has been applied to the synthesis of indolizidine peptide mimics, starting from a chiral imide derived from l-aspartic acid. It was observed that the preexisting stereogenic center of this substrate has a moderate influence on the stereoselectivity of the electrophilic allylation, which is mainly determined by the sense of chirality of the catalyst. 相似文献