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81.
T.B. Settersten A. Dreizler B.D. Patterson P.E. Schrader R.L. Farrow 《Applied physics. B, Lasers and optics》2003,76(4):479-482
This study reports on photochemical interferences affecting atomic oxygen detection using two-photon laser-induced fluorescence
at 226 nm. In contrast to previous studies in which molecular oxygen was proven to be the relevant photochemical precursor
molecule in a hydrogen-fueled flame, the present investigations were carried out in a laminar diffusion flame of methane and
air. The most significant interferences were found at the fuel side of the flame in the absence of molecular oxygen, and vibrationally
excited carbon dioxide was identified as the most probable precursor molecule for the photochemical production of oxygen atoms.
Received: 11 December 2002 / Revised version: 10 March 2003 / Published online: 16 April 2003
RID="*"
ID="*"Corresponding author. Fax: +1-925/294-2595, E-mail: tbsette@sandia.gov 相似文献
82.
83.
84.
E. I. Moses R. E. Bonanno C. A. Haynam R. L. Kauffman B. J. MacGowan R. W. Patterson Jr R. H. Sawicki B. M. Van Wonterghem 《The European Physical Journal D - Atomic, Molecular, Optical and Plasma Physics》2007,44(2):215-218
The National Ignition Facility (NIF) is a 192-beam laser
facility presently under construction at LLNL. When completed, NIF will be a
1.8-MJ, 500-TW ultraviolet laser system. Its missions are to obtain fusion
ignition and to perform high energy density experiments in support of the
US nuclear weapons stockpile. Four of the NIF beams have been commissioned
to demonstrate laser performance and to commission the target area including
target and beam alignment and laser timing. During this time, NIF
demonstrated on a single-beam basis that it will meet its performance goals
and demonstrated its precision and flexibility for pulse shaping, pointing,
timing and beam conditioning. It also performed four important experiments
for Inertial Confinement Fusion and High Energy Density Science. Presently,
the project is installing production hardware to complete the project in
2009 with the goal to begin ignition experiments in 2010. An integrated plan
has been developed including the NIF operations, user equipment such as
diagnostics and cryogenic target capability, and experiments and
calculations to meet this goal. This talk will provide NIF status, the plan
to complete NIF, and the path to ignition. 相似文献
85.
Eann A. Patterson Erwin Hack Philippe Brailly Richard L. Burguete Qasim Saleem Thorsten Siebert Rachel A. Tomlinson Maurice P. Whelan 《Optics and Lasers in Engineering》2007,45(5):550
The design and testing of a reference material for the calibration of optical systems for strain measurement is described, together with the design and testing of a standardized test material that allows the evaluation and assessment of fitness for purpose of the most sophisticated optical system for strain measurement. A classification system for the steps in the measurement process is also proposed and allows the development of a unified approach to diagnostic testing of components or sub-systems in an optical system for strain measurement based on any optical technique. The results described arise from a European study known as SPOTS whose objectives were to begin to fill the gap caused by a lack of standards. 相似文献
86.
We report improved measurements of the temperature-dependent cross sections for the quenching of fluorescence from the A 2Sigma+(v'=0) state of NO. Cross sections were measured for gas temperatures ranging from 294 to 1300 K for quenching by NO(X (2)Pi), H(2)O, CO(2), O(2), CO, N(2), and C(2)H(2). The A 2Sigma+(v'=0) state was populated via two-photon excitation with a picosecond laser at 454 nm, and the decay rate of the fluorescence originating from A 2Sigma+(v'=0) was measured directly. Thermally averaged quenching cross sections were determined from the dependence of the fluorescence decay rate on the quencher gas pressure. Our measurements are compared to previous measurements and models of the quenching cross sections, and new empirical fits to the data are presented. Our new cross-section data enable predictions in excellent agreement with prior measurements of the fluorescence lifetime in an atmospheric-pressure methane-air diffusion flame. The agreement resolves discrepancies between the lifetime measurements and predictions based on the previous quenching models, primarily through improved models for the quenching by H(2)O, CO(2), and O(2) at temperatures less than 1300 K. 相似文献
87.
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89.
H. Bendiab G. Roux-Desgranges A. H. Roux J. -P. E. Grolier D. Patterson 《Journal of solution chemistry》1994,23(2):307-323
Densities and heat capacities of ternary systems were determined at 25°C. The ternary systems consisted of: a polar molecule (component 1) + a mixture of alkanes (components 2 and 3) of different sizes and shapes. Five such systems were studied: chlorobenzene + cyclohexane + n-heptane; chlrobenzene + cyclohexane + n-hexadecane; chlorobenze + cyclohexane + isooctane; chlorobenzene + isooctane + n-heptane; 1-chloronaphthalene + isooctane + n-heptane. The excess molar volumes and heat capacities were obtained along dilution lines by component 1 (chlorobenzene or 1-chloronaphthalene) of mixtures of components 2 and 3 (at fixed component 2 mole fraction X2). Unexpectedly the excess heat capacities C
p1(23)
E
of the pseudo-binaries {1+(2+3)} do not always fall between the two (limiting) curves of C
p12
E
and C
p13
E
corresponding to the two binaries {1+2} and {1+3}. Instead, especially for {chlorobenzene + cyclohexane + an n-alkane} the C
p1(23)
E
curves are displaced toward less negative values, even beyond the limiting values corresponding to the binaries. This correlates semi-quantitatively with the negative C
p23
E
of the binary {2+3}.Presented at the Symposium, 76th CSC Congress, Sherbrooke, Quebec, May 30-June 3, 1993, honoring Professor Donald Patterson on the occasion of his 65th birthday. 相似文献
90.
Emilio Aicart Huu Van Tra Lina Andreoli-Ball Donald Patterson 《Journal of solution chemistry》1994,23(11):1183-1201
Expansion coefficients , isothermal compressibilities, thermal pressure coefficients and heat capacities have been measured at 25°C for the cyclohexane+trans-decalin system. An S-shaped composition dependence, positivelnegative for highllow cyclohexane compositions is found for C
p
E
dV
E
/dT and the thermal expansion contribution to C
p
E
namely VT. The thermal motion contribution to C
p
E
, namely C
v
is close to zero. The positive excursion of these mixing quantities at high cyclohexane content is anomalous. Correspondingly, the mixing quantity-VT deviates strongly in this region from the predicted equality with H
E
. The literature and this work show that all these excess quantities behave similarly for cyclohexane mixed with cyclooctane, methylcyclohexane and some highly branched alkanes. The unusual composition dependence of the thermodynamic quantities is consistent with order occurring when any large alkane molecule of globular shape is added to cyclohexane. This is speculatively associated with an interference by the globular alkane with the relatively free rotation of cyclohexane molecules. 相似文献