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81.
T.B. Settersten A. Dreizler B.D. Patterson P.E. Schrader R.L. Farrow 《Applied physics. B, Lasers and optics》2003,76(4):479-482
This study reports on photochemical interferences affecting atomic oxygen detection using two-photon laser-induced fluorescence
at 226 nm. In contrast to previous studies in which molecular oxygen was proven to be the relevant photochemical precursor
molecule in a hydrogen-fueled flame, the present investigations were carried out in a laminar diffusion flame of methane and
air. The most significant interferences were found at the fuel side of the flame in the absence of molecular oxygen, and vibrationally
excited carbon dioxide was identified as the most probable precursor molecule for the photochemical production of oxygen atoms.
Received: 11 December 2002 / Revised version: 10 March 2003 / Published online: 16 April 2003
RID="*"
ID="*"Corresponding author. Fax: +1-925/294-2595, E-mail: tbsette@sandia.gov 相似文献
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E. I. Moses R. E. Bonanno C. A. Haynam R. L. Kauffman B. J. MacGowan R. W. Patterson Jr R. H. Sawicki B. M. Van Wonterghem 《The European Physical Journal D - Atomic, Molecular, Optical and Plasma Physics》2007,44(2):215-218
The National Ignition Facility (NIF) is a 192-beam laser
facility presently under construction at LLNL. When completed, NIF will be a
1.8-MJ, 500-TW ultraviolet laser system. Its missions are to obtain fusion
ignition and to perform high energy density experiments in support of the
US nuclear weapons stockpile. Four of the NIF beams have been commissioned
to demonstrate laser performance and to commission the target area including
target and beam alignment and laser timing. During this time, NIF
demonstrated on a single-beam basis that it will meet its performance goals
and demonstrated its precision and flexibility for pulse shaping, pointing,
timing and beam conditioning. It also performed four important experiments
for Inertial Confinement Fusion and High Energy Density Science. Presently,
the project is installing production hardware to complete the project in
2009 with the goal to begin ignition experiments in 2010. An integrated plan
has been developed including the NIF operations, user equipment such as
diagnostics and cryogenic target capability, and experiments and
calculations to meet this goal. This talk will provide NIF status, the plan
to complete NIF, and the path to ignition. 相似文献
85.
Eann A. Patterson Erwin Hack Philippe Brailly Richard L. Burguete Qasim Saleem Thorsten Siebert Rachel A. Tomlinson Maurice P. Whelan 《Optics and Lasers in Engineering》2007,45(5):550
The design and testing of a reference material for the calibration of optical systems for strain measurement is described, together with the design and testing of a standardized test material that allows the evaluation and assessment of fitness for purpose of the most sophisticated optical system for strain measurement. A classification system for the steps in the measurement process is also proposed and allows the development of a unified approach to diagnostic testing of components or sub-systems in an optical system for strain measurement based on any optical technique. The results described arise from a European study known as SPOTS whose objectives were to begin to fill the gap caused by a lack of standards. 相似文献
86.
E V Patterson C J Cramer D G Truhlar 《Journal of the American Chemical Society》2001,123(9):2025-2031
Ab initio and density functional levels of electronic structure theory are applied to characterize alternative mechanisms for the reductive dechlorination of hexachloroethane (HCA) to perchloroethylene (PCE). Aqueous solvation effects are included using the SM5.42R continuum solvation model. After correction for a small systematic error in the electron affinity of the chlorine atom, theoretical predictions are accurate to within 23 mV for four aqueous reduction potentials relevant to HCA. A single pathway that proceeds via two successive single-electron transfer/barrierless chloride elimination steps, is predicted to be the dominant mechanism for reductive dechlorination. An alternative pathway predicted to be accessible involves trichloromethylchlorocarbene as a reactive intermediate. Bimolecular reactions of the carbene with other species at millimolar or higher concentrations are predicted to potentially be competitive with its unimolecular rearrangement to form PCE. 相似文献
87.
Gary D. Patterson 《Foundations of Chemistry》2010,12(3):223-233
There have been occasions when the publication of a particular book has had a singular impact on the conceptual world of the chemist. Sometimes the publication occurs near the beginning of a major change in discourse, and sometimes more near the end. Jean Perrin published Les Atomes in 1913 as the culmination of a century-long controversy over the size and physical reality of atoms and molecules. After its publication almost all chemists and physicists agreed that atoms and molecules of the size we currently understand to be appropriate are real physical objects. The story of the background, development, publication, content and response to Les Atomes forms the text of this paper. The content of Les Atomes is also the basis for extended reflection on the philosophical significance of the work of Jean Perrin. 相似文献
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