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111.
S. G. Raptis S. M. Nasiou I. N. Demetropoulos M. G. Papadopoulos 《Journal of computational chemistry》1998,19(15):1698-1715
The structure–polarization relationship was investigated in a series of polysulfanes, H2Sn. The reported results demonstrate that the forms of change of the polarizability components, αii, and the second hyperpolarizability components, γiiii, as well as the average values α and γ, respectively, of H2Sn with n are similar. This shows that polarizability components can be easily used to determine corresponding hyperpolarizability data. A remarkable change of the hyperpolarizabilities with the molecular geometry of H2Sn was found. This result can be used for the design of nonlinear optical materials with optimum properties. The present study uses the flexible σ bonded H2Sn and is complementary to the works that considered the effect of conformational changes of π-conjugated systems on their hyperpolarizabities. The present computations were performed using the semiempirical approaches MNDO and MNDO/d, as well as ab initio methods with STO-3G, extended with polarization and diffuse functions, and [3s2p/7s5p2d] sets for H2Sn. At the ab initio level, the electronic and the vibrational contributions to polarizabilities and hyperpolarizabilities were both computed for several members of H2Sn. The frequency dependence of the above contributions and the static limit were discussed. Electron correlation was taken into account for several test cases using MP2 theory. The selected methods and the variety of the approximations on which they rely allow the systematic consideration of the effect of changes of the geometry of H2Sn on their polarizabilities and second hyperpolarizabilities. © 1998 John Wiley & Sons, Inc. J Comput Chem 19: 1698–1715, 1998 相似文献
112.
Spatio-temporal development of the filaments due to the thermal self-focusing instability near the critical surface in ionospheric plasmas 总被引:1,自引:0,他引:1
N. A. Gondarenko P. N. Guzdar G. M. Milikh A. S. Sharma K. Papadopoulos S. L. Ossakow 《Radiophysics and Quantum Electronics》1999,42(7):589-600
We study fully nonlinear spatio-temporal development of the thermal self-focusing instability of high-power radio waves near
the critical surface of the ionosphere. These simulations improve on our earlier work by including an evolution equation for
the density instead of using the assumption of constant pressure to determine the perturbed density connected with the known
temperature perturbation. Using our two-dimensional nonlinear code we analyze the time scale and associated velocity for the
development of the field-aligned irregularities as they spread from the critical surface both in the underdense as well as
the overdense regions. The scaling of this velocity as a function of the radiated power of the heater electromagnetic wave
(ERP) is determined. We also study the characteristic size of the self-focused filament as a function of ERP. Finally, the
spectrum of the density and temperature fluctuations as well as modifications in the equilibrium values of these parameters
for different values of ERP are presented.
Translated from Izvestiya Vysshikh Uchebnykh Zavedenii, Radiofizika, Vol. 42, No. 7, pp. 670–681, July 1999. 相似文献
113.
This paper has two parts. In the first part, we study shift coordinates on a sphere S equipped with three distinguished points and a triangulation whose vertices are the distinguished points. These coordinates
parametrize a space
(S)\widetilde{{\cal T}}(S)
that we call an unfolded Teichmüller space. This space contains Teichmüller spaces of the sphere with
\frak b{\frak b}
boundary components and
\frak p{\frak p}
cusps (which we call generalized pairs of pants), for all possible values of
\frak b{\frak b}
and
\frak p{\frak p}
satisfying
\frak b+\frak p=3{\frak b}+{\frak p}=3
. The parametrization of
[(T)\tilde](S)\widetilde{{\cal T}}(S)
by shift coordinates equips this space with a natural polyhedral structure, which we describe more precisely as a cone over
an octahedron in
\Bbb R3{\Bbb {R}}^3
. Each cone over a simplex of this octahedron is interpreted as a Teichmüller space of the sphere with
\frak b{\frak b}
boundary components and
\frak p{\frak p}
cusps, for fixed
\frak b{\frak b}
and
\frak p{\frak p}
, the sphere being furthermore equipped with an orientation on each boundary component. There is a natural linear action of
a finite group on
[(T)\tilde](S)\widetilde{{\cal T}}(S)
whose quotient is an augmented Teichmüller space in the usual sense. We describe several aspects of the geometry of the space
[(T)\tilde](S)\widetilde{{\cal T}}(S)
. Stretch lines and earthquakes can be defined on this space. In the second part of the paper, we use the shift coordinates
to obtain estimates on the behaviour of stretch lines in the Teichmüller space of a surface obtained by gluing hyperbolic
pairs of pants. We also use the shift coordinates to give formulae that express stretch lines in terms of Fenchel-Nielsen
coordinates. We deduce the disjointness of some stretch lines in Teichmüller space. We study in more detail the case of a
closed surface of genus 2. 相似文献
114.
E. N. Argyres G. Katsilieris O. Korakianitis C. G. Papadopoulos C. Philippides W. J. Stirling 《Physics letters. [Part B]》1992,280(3-4):324-328
The reaction pp→W±γγX is considered at centre-of-mass energies √s = 16 and 40 TeV, including anomalous three- and four- gauge-boson couplings κ and λ. Limits are obtained on these quantities by comparison with the standard model. 相似文献
115.
116.
The kaon B-parameter is computed in the framework of strictly local QCD sum rules for a threepoint function involving pseudoscalar currents. As an application of these sum rules we derive a low energy formula for the B-parameter. We show that strictly local QCD sum rules yield more reliable results than other QCD sum rules, since they need less phenomenological information and do not suffer from stability problems. Our result for the B-parameter isB=0.74±0.17. 相似文献
117.
Kostas Kleidis Apostolos Kuiroukidis Demetrios Papadopoulos Loukas Vlahos 《International Journal of Theoretical Physics》2007,46(9):2283-2298
We study the linear magnetohydrodynamic (MHD) equations, both in the Newtonian and the general-relativistic limit, as regards
a viscous magnetized fluid of finite conductivity and discuss instability criteria. In addition, we explore the excitation
of cosmological perturbations in anisotropic spacetimes, in the presence of an ambient magnetic field. Acoustic, electromagnetic
(e/m) and fast-magnetosonic modes, propagating normal to the magnetic field, can be excited, resulting in several implications
of cosmological significance. 相似文献
118.
C. Dams R. Kleiss P. Draggiotis E.N. Argyres A. van Hameren C.G. Papadopoulos 《The European Physical Journal C - Particles and Fields》2003,28(4):561-571
We introduce a class of self-interacting scalar theories in which the various coupling constants obey a recursive relation.
These imply a particularly simple form for the generating function of the Feynman amplitudes with vanishing external momenta,
as well as for the effective potential. In addition we discuss an interesting duality inherent in these models. Specializing
to the case of zero spacetime dimensions we find intriguing nullification properties for the amplitudes.
Received: 19 December 2001 / Published online: 5 May 2003
RID="a"
ID="a" e-mail: chrisd@sci.kun.nl
RID="b"
ID="b" e-mail: kleiss@sci.kun.nl
RID="c"
ID="c" e-mail: petros@sci.kun.nl
RID="d"
ID="d" e-mail: andrevh@sci.kun.nl
RID="e"
ID="e" e-mail: papadopo@alice.nuclear.demokritos.gr 相似文献
119.
Aggelos Avramopoulos Manthos G. Papadopoulos Andrzej J. Sadlej 《Chemical physics letters》2003,370(5-6):765-769
The interaction between AuOH and the lone-pair donors (HF, H2O) is shown to result in well-bound complexes whose structure resembles that of the corresponding H-bonded systems with the gold atom replacing hydrogen. The dissociation energies are estimated to be 10.7 and 27.4 kcal/mol for HFAu–OH and H2OAu–OH, respectively. However, the interaction between AuOH and the lone pair donors is found to involve significant charge transfer. Furthermore, the Au–O stretching frequency increases upon the complex formation. It is concluded that, in spite of certain similarity to the H-bonded species, the Au-bonded complexes should be considered as Lewis acid–base pairs. 相似文献
120.
Eisert J Felbinger T Papadopoulos P Plenio MB Wilkens M 《Physical review letters》2000,84(7):1611-1614
We establish a quantitative connection between the amount of lost classical information about a quantum state and the concomitant loss of entanglement. Using methods that have been developed for the optimal purification of mixed states, we find a class of mixed states with known distillable entanglement. These results can be used to determine the quantum capacity of a quantum channel which randomizes the order of transmitted signals. 相似文献