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571.
A. V. Pak N. G. Lebedev 《Russian Journal of Physical Chemistry B, Focus on Physics》2012,6(2):321-326
A model of the multiple adsorption of atomic hydrogen on the surface of single-walled carbon nanotubes of the zigzag and arm-chair types was constructed. The adsorption model is based on the Anderson periodic model. An analytic equation for the band structure of carbon nanotubes with adsorbed hydrogen atoms was obtained, and the special features of this structure were studied. The dependence of the band structure of carbon nanotubes on the concentration of adsorbed hydrogen atoms was analyzed. The model constructed can be used to study adsorption of other univalent atoms on the surface of carbon particles. 相似文献
572.
The electrochemical oxidation of catechol (=benzene‐1,2‐diol; 1a ) and some of its derivatives in H2O/MeCN 1 : 1 containing benzoylacetonitrile (=β‐oxobenzenepropanenitrile; 3 ) as a nucleophile was studied by cyclic voltammetry and controlled‐potential coulometry. The voltammetric data showed that electrochemically generated o‐benzoquinones (=cyclohexa‐3,5‐diene‐1,2‐diones) from catechol ( 1a ) and 3‐methylcatechol ( 1b ) participate in a Michael‐addition reaction with 3 to form the corresponding 5,6‐dihydroxybenzofuran‐3‐carbonitrile 8 (Scheme 1). In this work, we report an efficient one‐pot method with high atom economy for the synthesis of new substituted 5,6‐dihydroxybenzofuran‐3‐carbonitriles in an undivided cell under ambient conditions. 相似文献
573.
We study the problem of acute triangulations of convex polyhedra and the space ? n . Here an acute triangulation is a triangulation into simplices whose dihedral angles are acute. We prove that acute triangulations of the n-cube do not exist for n≥4. Further, we prove that acute triangulations of the space ? n do not exist for n≥5. In the opposite direction, in ?3, we present a construction of an acute triangulation of the cube, the regular octahedron and a non-trivial acute triangulation of the regular tetrahedron. We also prove nonexistence of an acute triangulation of ?4 if all dihedral angles are bounded away from π/2. 相似文献
574.
Back BB Baker MD Ballintijn M Barton DS Betts RR Bickley AA Bindel R Budzanowski A Busza W Carroll A Chai Z Decowski MP García E Gburek T George N Gulbrandsen K Gushue S Halliwell C Hamblen J Hauer M Heintzelman GA Henderson C Hofman DJ Hollis RS Hołyński R Holzman B Iordanova A Johnson E Kane JL Katzy J Khan N Kucewicz W Kulinich P Kuo CM Lin WT Manly S McLeod D Mignerey AC Nouicer R Olszewski A Pak R Park IC Pernegger H Reed C Remsberg LP Reuter M Roland C Roland G Rosenberg L Sagerer J 《Physical review letters》2006,97(1):012301
We report on measurements of directed flow as a function of pseudorapidity in Au + Au collisions at energies of square root of SNN = 19.6, 62.4, 130 and 200 GeV as measured by the PHOBOS detector at the BNL Relativistic Heavy Ion Collider. These results are particularly valuable because of the extensive, continuous pseudorapidity coverage of the PHOBOS detector. There is no significant indication of structure near midrapidity and the data surprisingly exhibit extended longitudinal scaling similar to that seen for elliptic flow and charged particle pseudorapidity density. 相似文献
575.
The structures, energetics, and transition states of water clusters (trimer to pentamer, n = 3-5) are investigated as a function of electric field by using ab initio calculations. With an increasing strength of the field, the most stable cyclic structures of trimer, tetramer, and pentamer open up to align their dipole moments along the direction of the field. For the lower strength (below 0.3 V/angstroms) of the electric field, the dipole moment of each water monomer is along the same direction with the field, while it retains the cyclic structure. For the higher strength of the field, to have a higher dipole moment for the cluster along the field direction, each cyclic structure opens up to form a linear chain or "water wire." We have investigated the transition state structures between the cyclic and linear forms for the field strengths of 0.3-0.4 V/angstroms where both cyclic and linear forms are energetically comparable. 相似文献
576.
Zhao Jing Zhu Yajuan Wong Pak Kin Li Wenfeng Yang Zhixin Li Panshuo Song Chonghui 《Nonlinear dynamics》2023,111(9):8275-8291
Nonlinear Dynamics - The vehicle active suspension has attracted considerable attention owing to its great contributions to the vertical dynamics of vehicle. This paper investigates the non-fragile... 相似文献