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51.
We present a stable regime of asymmetric bound states for spiral pairs in a generic numerical model of a homogeneous excitable medium. In this regime, one spiral tip (slave) rotates around the other (master). Master-slave dynamics occur for both same-chirality and opposite-chirality spiral pairs in a range of parameters and initial conditions. We study the dependency of master-slave characteristics on the medium's excitation threshold and present a phenomenological model that accounts for the qualitative properties of master-slave dynamics. 相似文献
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In ligand design for asymmetric catalysis, the usual norm is to derive the face shielding elements from a chiral source. New ligands in which the face shielding is determined by fluxional groups are introduced. Their design, modular synthesis, and experiments to demonstrate the significance of the fluxional groups are discussed. The advantage is that the fluxional groups, introduced at a later stage, allow for simple tuning of the face shielding group. 相似文献
54.
55.
J. Rana G.L. Goswami S.K. Jha P.K. Mishra B.V.S.S.S. Prasad 《Optics & Laser Technology》2007,39(2):385-393
An experimental investigation with 5 kW CW CO2 laser system was carried out to study the effects of different laser and process parameters on the microstructure and hardness of carbon steel specimen with varying carbon percentage. The laser beam is allowed to scan on the surface of the work piece varying the power (1.1–2.5 kW) and traverse speed (6–15 mm/s) at two different spot sizes using TEM01* mode laser beam. The most hardenable microstructure achieved in case of three grades of carbon steel and the most influencing parameter on the value of hardness are reported. Besides the above study, some multipass operations are also carried out to recommend an appropriate gap between consecutive passes. 相似文献
56.
Himadri R. Soni Venu Mankad Sanjay D. Gupta Sanjeev K. Gupta Prafulla K. Jha 《Journal of Thermal Analysis and Calorimetry》2012,107(1):39-44
In the present paper, we report an ab initio calculation of the ground state, electronic and thermodynamical properties like
constant volume lattice specific heat, vibrational energy, internal energy, and entropy for GaP and Ga2P is presented. These properties are obtained after calculating the phonon spectrum over the entire Brillouin zone. The calculations
were performed using the ABINIT program package, which is based on density functional theory (DFT) method and the use of pseudopotentials
and plane wave expansion. Difference in the ground state properties such as electronic structure and thermodynamical properties
are discussed. The thermodynamical properties follow the expected trend. There is a good agreement between present theoretical
and limited available experimental data in the case of ground state such as lattice constant and bulk modulus and electronic
properties. With the increase of Ga atoms in the unit cell the semiconducting nature of Ga2P turns to metallic. There is a noticeable difference in the thermodynamical properties in the case of both gallium compounds. 相似文献
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Recent progress made in the use of time-resolved pump-probe Raman scattering technique to study the dynamics of photo-excited nonequilibrium carriers and LO-phonons in III–V semiconductors up to the sub-picosecond time scale will be discussed. It will be shown how this technique has allowed direct time-domain measurements of electron-LO-phonon scattering times for “hot” carriers and lifetimes for “hot” LO-phonons in semiconductors like GaAs. The presentation will include new experimental results of Kash, Jha and Tsang on picosecond Raman studies of the Fröhlich interaction in alloys like Al x Ga 1?x As and In x Ga 1?x As. The present theoretical understanding of the dynamics of the highly excited carriers, dominated by strong LO-phonon emission, will be examined along with the discussion of a recent calculation of transient electrical conductivity of such hot carriers, showing extremely interesting oscillations with respect to the pump laser frequency, on the scale of the long wavelength LO-phonon frequency, and a highly nonlinear behaviour as a function of time. 相似文献
59.
The diastereoselective synthesis of the macrolactone core of amphidinolide W was successfully accomplished using Evans’ asymmetric alkylation, Aldol reaction, Julia-Kocienski olefination, and Kita’s macrocyclization protocol. 相似文献
60.