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81.
Molecular dynamics simulations were conducted for a cubic Cu cluster supported on a graphite bilayer. The Sutten–Chen and Lennard–Jones potentials were used for metal–metal and metal–graphite interactions, respectively. Heating and cooling processes were performed by NVT simulations at different temperatures in the range 200 to 1800?K. The melting point was identified on the basis of caloric and heat capacity curves. The calculated melting point was 770?K, far below the bulk melting point of crystalline copper. Several phenomena such as the appearance of a hysteresis (irreversibility) in caloric curves, surface melting, and cluster-induced surface wetting were justified from the results. The simulation of cluster in the presence of gas atmosphere showed that the CO gas is adsorbed more than H2 and it has a greater impact on the cluster's structure.  相似文献   
82.
In this article, a capacitated location allocation problem is considered in which the demands and the locations of the customers are uncertain. The demands are assumed fuzzy, the locations follow a normal probability distribution, and the distances between the locations and the customers are taken Euclidean and squared Euclidean. The fuzzy expected cost programming, the fuzzy β-cost minimization model, and the credibility maximization model are three types of fuzzy programming that are developed to model the problem. Moreover, two closed-form Euclidean and squared Euclidean expressions are used to evaluate the expected distance between customers and facilities. In order to solve the problem at hand, a hybrid intelligent algorithm is applied in which the simplex algorithm, fuzzy simulation, and a modified genetic algorithm are integrated. Finally, in order to illustrate the efficiency of the proposed hybrid algorithm, some numerical examples are presented.  相似文献   
83.
A mixed binary integer mathematical programming model is developed in this paper for ordering items in multi-item multi-period inventory control systems, in which unit and incremental quantity discounts as well as interest and inflation factors are considered. Although the demand rates are assumed deterministic, they may vary in different periods. The situation considered for the problem at hand is similar to a seasonal inventory control model in which orders and sales happen in a given season. To make the model more realistic, three types of constraints including storage space, budget, and order quantity are simultaneously considered. The goal is to find optimal order quantities of the products so that the net present value of total system cost over a finite planning horizon is minimized. Since the model is NP-hard, a genetic algorithm (GA) is presented to solve the proposed mathematical problem. Further, since no benchmarks can be found in the literature to assess the performance of the proposed algorithm, a branch and bound and a simulated annealing (SA) algorithm are employed to solve the problem as well. In addition, to make the algorithms more effective, the Taguchi method is utilized to tune different parameters of GA and SA algorithms. At the end, some numerical examples are generated to analyze and to statistically and graphically compare the performances of the proposed solving algorithms.  相似文献   
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85.
Digoxin is widely used as a cardiac glycoside drug in the treatment of various heart conditions. Because it is a toxic drug, it should be regularly monitored in the serum of patients under treatment. In this study, colloidal nanogold is synthesized and the preparation of nanogold-labeled monoclonal antibody probe to digoxin is described under optimal conditions. In addition, an immunochromatographic (IC) method for digoxin analysis employing nanogold-labeled probe is developed. With this technique, it requires only 5 min to complete the quantitative detection of digoxin. The detection time is decreased 20–30 times in comparison to radioimmunoassay (RIA). The sensitivity to digoxin was about 2 ng/ml by naked eye, which is within the therapeutic and toxic ranges of digoxin. The results of serum samples obtained by IC strip were in agreement with those obtained by RIA. The IC strip was sufficiently sensitive and accurate to be used for the rapid detection of digoxin in serum samples.  相似文献   
86.
The effect of 4,4′-diaminodiphenylsulfone (DADPS) as a co-additives in iodide/triiodide redox electrolyte on the performance of dye-sensitized solar cell based on the 2-cyano-3-(4-(diphenylamino)phenyl)acrylic acid (TPA) and 2-cyano-3-(2΄-(5΄,10΄,15΄,20΄- tetraphenylporphyrinato Zinc (II)yl) acrylic acid (Zn-1) dyes have been investigated. Compared withstandard electrolyte (0.1 M LiI, 0.05 M I2, 0.6 M 1-butyl-2,3-dimethylimidazolium iodide (BDMII) and TBP (0.5, 1 M)), adding 0.5 M of DADPS, as a co-additive, into the electrolyte system has caused increasing short current density (Jsc) and open-circuit potential (Voc) consequently the energy conversion (η) improved. Electrochemical impedance results indicate adsorbing of DADPS on the titanium dioxide surface leads to an increase in the lifetime (τ). Adsorbing of DADPS on the semiconductor surface retards the interfacial charge recombination that has a beneficial effect on the Voc and Jsc. The results showed that amine groups of DADPS attach to the conduction band (CB) of TiO2 film and suppress the electron recombination process and as a result, it can be applied as a promising co-additive in DSSCs.  相似文献   
87.
88.
Hollow microblocks of [Zn(anic)2], as a novel coordination compound, were synthesized using 2-aminonicotinic acid (Hanic) and zinc (II) nitrate tetrahydrate. The chemical composition of the zinc comple...  相似文献   
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90.
A nonwoven fabric with paperlike qualities composed of silicon nanowires is reported. The nanowires, made by the supercritical-fluid-liquid-solid process, are crystalline, range in diameter from 10 to 50 nm with an average length of >100 μm, and are coated with a thin chemisorbed polyphenylsilane shell. About 90% of the nanowire fabric volume is void space. Thermal annealing of the nanowire fabric in a reducing environment converts the polyphenylsilane coating to a carbonaceous layer that significantly increases the electrical conductivity of the material. This makes the nanowire fabric useful as a self-supporting, mechanically flexible, high-energy-storage anode material in a lithium ion battery. Anode capacities of more than 800 mA h g(-1) were achieved without the addition of conductive carbon or binder.  相似文献   
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