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B. Wallbank C.E. Johnson I.G. Main 《Journal of Electron Spectroscopy and Related Phenomena》1974,4(3):263-269
Pronounced surface reduction of some 3d transition metal compounds has been observed during measurements with an AEI ES200 X-ray photoelectron spectrometer. Systematic data indicate that the degree of reduction in a given compound does not depend on temperature, vacuum pressure or X-ray flux, but is a function only of the integrated X-ray dose. Particularly strong effects were found in cupric fluoride and potassium ferricyanide. 相似文献
23.
From the measurement of a reflection spectrum of an open microwave cavity, the poles of the scattering matrix in the complex plane have been determined. The resonances have been extracted by means of the harmonic inversion method. By this, it became possible to resolve the resonances in a regime where the linewidths exceed the mean level spacing up to a factor of 10, a value inaccessible in experiments up to now. The obtained experimental distributions of linewidths were found to be in perfect agreement with predictions from random matrix theory when wall absorption and fluctuations caused by couplings to additional channels are considered. 相似文献
24.
Main M Snaith JS Meloni MM Jauregui M Sykes D Faulkner S Kenwright AM 《Chemical communications (Cambridge, England)》2008,(41):5212-5214
The Ugi reaction offers an effective method for preparing chromophore-appended DOTA-monoamide ligands, which can readily be elaborated to their lanthanide complexes. 相似文献
25.
The dynamics of quantum systems can be approximated by the time propagation of Gaussian wave packets. Applying a time dependent variational principle, the time evolution of the parameters of the coupled Gaussian wave packets can be calculated from a set of ordinary differential equations. Unfortunately, the set of equations is ill behaved in most practical applications, depending on the number of propagated Gaussian wave packets, and methods for regularization are needed. We present a general method for regularization based on applying adequate nonholonomic inequality constraints to the evolution of the parameters, keeping the equations of motion well behaved. The power of the method is demonstrated for a nonintegrable system with two degrees of freedom. 相似文献
26.
An embedded boundary framework for compressible turbulent flow and fluid–structure computations on structured and unstructured grids 下载免费PDF全文
The finite volume method with exact two‐phase Riemann problems (FIVER) is a two‐faceted computational method for compressible multi‐material (fluid–fluid, fluid–structure, and multi‐fluid–structure) problems characterized by large density jumps, and/or highly nonlinear structural motions and deformations. For compressible multi‐phase flow problems, FIVER is a Godunov‐type discretization scheme characterized by the construction and solution at the material interfaces of local, exact, two‐phase Riemann problems. For compressible fluid–structure interaction (FSI) problems, it is an embedded boundary method for computational fluid dynamics (CFD) capable of handling large structural deformations and topological changes. Originally developed for inviscid multi‐material computations on nonbody‐fitted structured and unstructured grids, FIVER is extended in this paper to laminar and turbulent viscous flow and FSI problems. To this effect, it is equipped with carefully designed extrapolation schemes for populating the ghost fluid values needed for the construction, in the vicinity of the fluid–structure interface, of second‐order spatial approximations of the viscous fluxes and source terms associated with Reynolds averaged Navier–Stokes (RANS)‐based turbulence models and large eddy simulation (LES). Two support algorithms, which pertain to the application of any embedded boundary method for CFD to the robust, accurate, and fast solution of FSI problems, are also presented in this paper. The first one focuses on the fast computation of the time‐dependent distance to the wall because it is required by many RANS‐based turbulence models. The second algorithm addresses the robust and accurate computation of the flow‐induced forces and moments on embedded discrete surfaces, and their finite element representations when these surfaces are flexible. Equipped with these two auxiliary algorithms, the extension of FIVER to viscous flow and FSI problems is first verified with the LES of a turbulent flow past an immobile prolate spheroid, and the computation of a series of unsteady laminar flows past two counter‐rotating cylinders. Then, its potential for the solution of complex, turbulent, and flexible FSI problems is also demonstrated with the simulation, using the Spalart–Allmaras turbulence model, of the vertical tail buffeting of an F/A‐18 aircraft configuration and the comparison of the obtained numerical results with flight test data. Copyright © 2014 John Wiley & Sons, Ltd. 相似文献
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Gabriel Wittum 《计算数学(英文版)》2009,(5):563-572
In this paper, we obtain optimal error estimates in both L^2-norm and H(curl)-norm for the Nedelec edge finite element approximation of the time-harmonic Maxwell's equations on a general Lipschitz domain discretized on quasi-uniform meshes. One key to our proof is to transform the L^2 error estimates into the L^2 estimate of a discrete divergence-free function which belongs to the edge finite element spaces, and then use the approximation of the discrete divergence-free function by the continuous divergence-free function and a duality argument for the continuous divergence-free function. For Nedelec's second type elements, we present an optimal convergence estimate which improves the best results available in the literature. 相似文献
29.
Sanguinetti S Chiantoni G Miotto A Grilli E Guzzi M Henini M Polimeni A Patane A Eaves L Main PC 《Micron (Oxford, England : 1993)》2000,31(3):309-313
We have investigated the In(Ga)As island formation, in the Stranski-Krastanov growth mode, on (311)A GaAs substrates. The surface topography of InAs and InGaAs strained epilayers was studied by contact microscopies. The different substrate affects the overgrown island shape. In(Ga)As grown on (311)A gives rise to quantum wire-like islands. Quantum dots (QDs), but with highly anisotropic shapes, are the outcomes of InAs deposition. QD samples were also characterized by photoluminescence (PL) measurements. Correlation between optical and morphological properties was observed. 相似文献
30.
Periodic orbit quantization requires an analytic continuation of non-convergent semiclassical trace formulae. We propose two different methods for semiclassical quantization. The first method is based upon the harmonic inversion of semiclassical recurrence functions. A band-limited periodic orbit signal is obtained by analytical frequency windowing of the periodic orbit sum. The frequencies of the periodic orbit signal are the semiclassical eigenvalues, and are determined by either linear predictor, Padé approximant, or signal diagonalization. The second method is based upon the direct application of the Padé approximant to the periodic orbit sum. The Padé approximant allows the resummation of the, typically exponentially, divergent periodic orbit terms. Both techniques do not depend on the existence of a symbolic dynamics, and can be applied to bound as well as to open systems. Numerical results are presented for two different systems with chaotic and regular classical dynamics, viz. the three-disk scattering system and the circle billiard. 相似文献