(111)取向(Pb,La)TiO3铁电薄膜中90°纳米带状畴与热释电性能的研究

采用射频磁控溅射技术在Pt/Ti/SiO2/Si(100)衬底上生长了掺镧钛酸铅(PLT)铁电薄膜.用X射线衍射技术(XRD)研究了PLT薄膜结晶性能,结果表明PLT薄膜为(111)择优取向钙钛矿相织构.使用原子力显微镜(AFM)和压电响应力显微镜(PFM)分别观察了PLT薄膜的表面形貌和对应区域的电畴结构.PFM观察显示PLT薄膜中存在90°纳米带状畴,电畴的极化为首尾相接的低能量的排列方式,带状畴的宽度为20-60nm.研究了PLT10铁电薄膜的制备条件与性能之间的关系.发现在优化条件下制备的PLT10铁电薄膜的介电常数εr为365、介电损耗tgδ为0.02,热释电系数γ为2.18×10-8C·(cm2·K)-1,可以满足制备非制冷红外探测器的需要.     

PVP掺杂-ZrO2溶胶-凝胶工艺制备多层激光高反射膜的研究

以丙醇锆(ZrPr)为锆源,二乙醇胺(DEA)为络合剂,原位引入聚乙烯吡咯烷酮(PVP),在乙醇体系中成功地合成了PVP掺杂-ZrO2溶胶.采用旋涂法在K9玻璃基片上制备了PVP-ZrO2单层杂化薄膜.用不同掺杂量的PVP-ZrO2高折射率膜层与相同的SiO2低折射率膜层交替沉积四分之一波堆高反射膜.借助小角X射线散射研究胶体微结构,用红外光谱、原子力显微镜、紫外/可见/近红外透射光谱、椭圆偏振仪以及1064nm的强激光辐照实验对薄膜的结构、光学和抗激光损伤性能进行表征.研究发现,体系组成的适当配置可以在溶胶稳定的前提下实现ZrPr的充分水解,赋予薄膜良好的结构、光学和抗激光损伤性能.杂化体系中,DEA与ZrPr之间强的配合作用大大降低了ZrO2颗粒表面羟基的活性,使得PVP大分子只是以微弱的氢键与颗粒的表面羟基作用而均匀分散于ZrO2颗粒的周围,对颗粒的形成和生长无显著影响.因而在实验研究范围内,随PVP含量的增大,PVP-ZrO2杂化膜层的折射率和激光损伤阈值均无显著变化.但是,薄膜中均匀分布的PVP柔性链可以有效促进膜层应力松弛,显著削弱不同膜层之间的应力不匹配程度、大大方便多层光学薄膜的制备.当高折射率膜层中PVP的质量分数达到15%-20%时,膜层之间良好的应力匹配使得多层高反射膜的沉积周期数可达到10以上.沉积1O个周期的多层反射膜,在中心波长1064nm处透射率约为1.6%-2.1%,接近全反射特征,其激光损伤阈值为16.4-18.2J/cm2(脉冲宽度为1ns).     

Impact of polarization dependent loss on degree of polarization as feedback signal of polarization mode dispersion

Polarization dependent loss (PDL) has been recognized as a critical issue because various inline optical components may have nonnegligible PDL effect that interacts with polarization mode dispersion (PMD).We investigated the impact of PMD-PDL interaction on degree of polarization (DOP), which is the most commonly used feedback signal in PMD compensation. The simulation results of a 40-Gb/s NRZ code optical transmission system show that the maximum PMD increases from approximately 40 ps to more than 45 ps, while minimum DOP declines from approximately 0.6 to approximately 0.2. The interaction of PMD and PDL also induces residual PMD underestimation of 5-8 ps, which causes degradation of PMD compensation performance.     

Distributed optical fiber surface plasmon resonance sensors

The relationships of the resonant wavelength of optical fiber surface plasmon resonance (SPR) sensors to the modulation layer refractive index, thickness and the refractive index of the bulk medium are obtained by using theoretical calculation model of optical fiber SPR sensors under certain conditions, which indicates that resonant wavelength of the sensors is approximately linear with modulation layer thickness. Based on the linear relationship, multiple SPR sensors with different resonant wavelengths can be fabricated in a single optical fiber named as distributed optical fiber surface plasmon resonance sensors (DOFSPRSs).Experimental results are presented, showing that it is practical to fabricate more than one SPR sensors in a single optical fiber.     

Tunable CW Tm,Ho:YLF laser at 2

A tunable continuous wave (CW) low temperature operating Tm (6 at.-%),Ho (0.6 at.-%):YLF laser pumped by fiber-coupled diode laser is reported. The maximum output power is 4.16 W at 2073 nm by use of 30% output coupling, the slope efficiency is 33%. A tuning range from 2049 to 2081 nm is achieved with a birefringent filter (BF). The factors that contribute to the output power and tuning range are discussed.     

Generation of near transform-limited ultrashort laser pulses in kilohertz chirped-pulse amplification system by compensating high order phase distortions

The effects of gain narrowing and high order dispersions on the pulse duration in our kilohertz chirpedpulse amplification system have been compensated experimentally. Using an acousto-optic programmable dispersive filter (AOPDF), the spectral full-width at half-maximum (FWHM) is expanded from 30 to50 nm. Stable laser pulses with the duration of 30 fs (FWHM), which is 1.07 times Fourier-transformlimitation, have been acquired by pre-compensating the high order phase distortions using the phase measured by spectral phase interferometry for direct electric-field reconstruction (SPIDER).     

Plasma-induced spatiotemporal modulation of propagating femtosecond pulses

The dynamics of the femtosecond pulse propagation in a plasma channel is investigated by the pumpprobe longitudinal diffractometry and second harmonic generation frequency-resolved optical gating (SHGFROG) technique. The spatial characteristics, corresponding to the electronic density and the size of the channel, can be observed by the recorded ring pattern, and the spectral and temporal characteristics are recorded by the SHG-FROG traces. The spatiotemporal characteristics will help us to better understand the dynamics of the plasma induced by the femtosecond pulse and the femtosecond pulse propagating in the plasma channel.     

A spectroscopic method for determining thickness of quartz wave plate

A spectroscopic method to determine thickness of quartz wave plate is presented. The method is based on chromatic polarization interferometry. With the polarization-resolved transmission spectrum (PRTS)curve, the phase retardation of quartz wave plate can be determined at a wide spectral range from 200 to2000 nm obviously. Through accurate judgment of extreme points of PRTS curve at long-wave band, the physical thickness of quartz wave plates can be obtained exactly. We give a measuring example and the error analysis. It is found that the measuring precision of thickness is mainly determined by the spectral resolution of spectrometer.     

Study of passive Q-switching for flash-lamp-pumped 1.34-μm Nd:GdVO4 laser

The static laser performance of a-growth Nd:GdVO4 crystal (a-cut, 4 × 4 × 25 (mm)) at 1.34μm pumped by flash-lamp is investigated with different transmissions of output couplers. With the output coupler transmission of T = 30%, the static output energy of 148 mJ is obtained when the pump energy is 35.2 J,and the corresponding electric-optical conversion efficiency is 0.42%. The Q-switched output of lasers with the output wavelength ranging from 1.3 to 1.6 μm can be realized by using Co2+ :LaMgAl11O19 (Co:LMA)as saturable absorber. A flash-lamp-pumped, passively Q-switched Nd:GdVO4 laser with Co:LMA as saturable absorber is demonstrated in plano-concave laser cavity. With the cavity length of 16.3 cm and pump energy of 19.8 J, the single-pulse output energy, pulse width, and peak power are obtained to be 4m J, 80 ns, and 5 × 104 W, respectively.     

High intensity focused ultrasound-induced gene activation in solid tumors

In this work, the activation of heat-sensitive trans-gene by high-intensity focused ultrasound (HIFU) in a tumor model was investigated. 4T1 cancer cells (2 x 10(6)) were inoculated subcutaneously in the hind limbs of Balb/C mice. The tumors were subsequently transducted on day 10 by intratumoral injection of a heat-sensitive adenovirus vector (Adeno-hsp70B-Luc at 2 x 10(8) pfu/tumor). On day 11, the tumors were heated to a peak temperature of 55, 65, 75, or 85 degrees C within 10-30 s at multiple sites around the center of the tumor by a 1.1- or 3.3-MHz HIFU transducer. Inducible luciferase gene expression was increased from 15-fold to 120-fold of the control group following 1.1-MHz HIFU exposure. Maximum gene activation (120-fold) was produced at a peak temperature of 65-75 degrees C one day following HIFU exposure and decayed to baseline within 7 days. HIFU-induced gene activation (75 degrees C-10 s) could be further improved by using a 3.3-MHz transducer and a dense scan strategy to 170-fold. Thermal stress, rather than nonthermal mechanical stress, was identified as the primary physical mechanism for HIFU-induced gene activation in vivo. Overall, these observations open up the possibility for combining HIFU thermal ablation with heat-regulated gene therapy for cancer treatment.