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561.
562.
Observation of stimulated Raman scattering in polar tetragonal crystals of barium antimony tartrate trihydrate,Ba[Sb2((+)C4H2O6)2]·3H2O 下载免费PDF全文
Alexander A. Kaminskii Hanjo Rhee Hans J. Eichler Oliver Lux Ivan Němec Hitoki Yoneda Akira Shirakawa Petra Becker Ladislav Bohatý 《Annalen der Physik》2017,529(4)
The non‐centrosymmetric polar tetragonal (P 41) barium antimony tartrate trihydrate, Ba[Sb2((+)C4H2O6)2]·3H2O, was found to be an attractive novel semi‐organic crystal manifesting numerous χ (2)‐ and χ (3)‐nonlinear optical interactions. In particular, with picosecond single‐ and dual‐wavelength pumping SHG and THG via cascaded parametric four‐wave processes were observed. High‐order Stokes and anti‐Stokes lasing related to two SRS‐promoting vibration modes of the crystal, with ωSRS1 ≈ 575 cm?1 and ωSRS2 ≈ 2940 cm?1, takes place. Basing on a spontaneous Raman investigation an assignment of the two SRS‐active vibration modes is discussed.
563.
Jana Honová Stanislav Luňák Martin Vala Stanislav Stříteský Ladislav Fekete Martin Weiter Alexander Kovalenko 《Chemical Papers》2016,70(10):1416-1424
An extended study on a group of four soluble diphenyl-amino-stilbene based diphenyl-diketopyrrolo- pyrrole molecules has been carried out. Using the materials in thin-film transistors it was shown that the above-mentioned compounds can be successfully used as donors in organic photovoltaic devices. Influence of the molecular symmetry and solubilizing chain on the morphology and solar cell performance are described. It was shown that a shorter and non-branched ethyl acetate chain leads to higher charge carrier mobility, short circuit current, and better fill factor. After the basic optimization, a power conversion efficiency of about 1.5 % was reached. This, to the best of our knowledge, is the highest reported efficiency of thiophene-free small-molecule diketo-pyrrolopyrroles. 相似文献
564.
The Riesz potential is known to be an important building block of many interactions, including Lennard-Jones–type potentials , that are widely used in molecular simulations. In this paper, we investigate analytically and numerically the minimizers among three-dimensional lattices of Riesz and Lennard-Jones energies. We discuss the minimality of the body-centered-cubic (BCC) lattice, face-centered-cubic (FCC) lattice, simple hexagonal (SH) lattices, and hexagonal close-packing (HCP) structure, globally and at fixed density. In the Riesz case, new evidence of the global minimality at fixed density of the BCC lattice is shown for and the HCP lattice is computed to have higher energy than the FCC (for ) and BCC (for ) lattices. In the Lennard-Jones case with exponents , the ground state among lattices is confirmed to be an FCC lattice whereas an HCP phase occurs once added to the investigated structures. Furthermore, phase transitions of type “FCC-SH” and “FCC-HCP-SH” (when the HCP lattice is added) as the inverse density V increases are observed for a large spectrum of exponents . In the SH phase, the variation of the ratio Δ between the interlayer distance d and the lattice parameter a is studied as V increases. In the critical region of exponents , the SH phase with an extreme value of the anisotropy parameter Δ dominates. If one limits oneself to rigid lattices, the BCC-FCC-HCP phase diagram is found. For , the BCC lattice is the only energy minimizer. Choosing , the FCC and SH latices become minimizers. 相似文献
565.