Controlling optical responses through local dielectric resonance in nanometre metallic clusters

Optical responses in dilute composites are controlled through the local dielectric resonance of metallic clusters. We consider two located metallic clusters close to each other with admittances \varepsilon₁ and \varepsilon₂. Through varying the difference admittance ratio \eta [ = (\varepsilon₂- \varepsilon ₀) / (\varepsilon₁- \varepsilon₀)], we find that their optical responses are determined by the local resonance. There is a blueshift of absorption peaks with the increase of \eta. Simultaneously, it is known that the absorption peaks will be redshifted by enlarging the cluster size. By adjusting the nano-metallic cluster geometry, size and admittances, we can control the positions and intensities of absorption peaks effectively. We have also deduced the effective linear optical responses of three-component composites \varepsilon_e= \varepsilon₀ \bigl(1 + \sum_n=1^{n_s} [(\gamma_n2+ \eta \gamma_n2)/({\varepsilon₀(s - s_n))]} \bigr), and the sum rule of cross sections: \sum_n=1^{n_s} {(\gamma_n2+ \eta \gamma_n2 ) = N_h1+ N_h2, where N_h1and N_h2 are the numbers of \varepsilon₁ and \varepsilon₂ bonds along the electric field, respectively. These results may be beneficial to the study of surface plasmon resonances on a nanometre scale.     

Polymer-assisted complexing controlled orientation growth of ZnO nanorods

The growth of the oriented zinc oxide (ZnO) nanorods on silicon substrates based on a simple novel chemical transformation and thermal hydrolysis by using polyvinyl alcohol (PVA) as self-assembling complex polymer was introduced in this paper. All the polymers were removed after chemical oxidation and only the carbonized grid backbones remained that confines the ZnO nanorod’s diameter and enhance the absorption and diffusion of ZnO at the tips of the nanorods during growth. The ZnO nanorods are investigated by FTIR, XRD and FE-SEM. The results indicated that these nanorods have fine hexagonal wurtzite crystal structure and their diameter varies from 20 to 90 nm and the length up to about 1 μm. A polymer-localized ZnO growth model is proposed, which well explains the growth behavior of ZnO nanorods.This revised version was published online in August 2005 with a corrected issue number.     

Frequency-stabilized semimonolithic frequency doubler with high output power

We present a semimonolithic frequency-doubler from 1080 to 540 nm with 80% doubling efficiency and up to 849-mW output power of green light.     

基于倏逝波的光纤生物传感器研究

构建了一种以光纤束作为激发光信号和荧光信号传输通道的光纤生物传感器结构.根据光纤探针的倏逝波理论和模式匹配理论对光纤探针的几何形状进行了设计,制作了数组光纤探针并根据需要对其中一部分进行荧光标记.选择了光纤探针置于空气中和水溶液中两种情况,对光纤传感器系统进行了信号检测实验,对比标记了的和未标记的相同几何结构参数的光纤探针两者在系统中被探测的信号差异.从二者的差别区分出系统所探测的倏逝波激发的荧光信号,证明了该光纤传感器系统的可行性.     

监测点波长对高双折射光纤环镜轴向应变灵敏度的影响

研究了高双折射光纤环镜监测点波长对轴向应变灵敏度的影响. 经理论推导得出高双折射光纤环镜轴向应变灵敏度公式. 结果表明: 当高双折射光纤材料选定后, 灵敏度随着监测点波长的增大而增大; 当监测点选定后, 监测点的灵敏度为常数, 波长变化与应变成线性关系. 实验选取不同波长的波峰进行应变灵敏度监测, 对各监测点进行数据拟合, 实验结果与理论分析一致. 研究结果对提高高双折射光纤环镜应变、温度等灵敏度具有指导意义. 关键词： 波长 灵敏度 监测点 高双折射光纤环镜     

Blocked-micropores,surface functionalized,bio-compatible and silica-coated iron oxide nanocomposites as advanced MRI contrast agent

Quasi-critical fluctuations occur close to critical points or close to continuous phase transitions. In three-dimensional systems, precision tuning is required to access the fluctuation regime. Lowering the dimensionality enhances the parameter space for quasi-critical fluctuations considerably. This enables one to make use of novel properties emerging in fluctuating systems, such as giant susceptibilities, Casimir forces or novel quasi-particle interactions. Examples are discussed ranging from simple metal–adsorbate systems to unconventional superconductivity in iron-based superconductors.     

扩展基于AD9874数字接收机谱宽的二次抽取算法

针对基于AD9874芯片的数字接收机的最小谱宽和谱宽允许设置的数目均不能满足常规临床用磁共振成像技术的要求,本文从软件角度提出了一种扩展数字接收机谱宽的二次抽取算法. 该算法具体实现过程主要包括两个步骤：(1) 自适应过采样倍率和自动谱宽调整;(2) 数字滤波和抽取. 为了验证这个二次抽取算法的有效性,本文分别用单脉冲实验和磁共振成像实验加以了验证.     

准晶体中八方晶系点群的对称性与矩阵表示

从理论上对准晶体中八方晶系各点群进行了研究.运用八方晶系各点群的极赤投影图,列出了各点群的所有对称操作;填出了固有点群822的群乘表.运用坐标变换和群论在自定义的八方坐标系中,推导出八方晶系点群所有对称操作的矩阵.这32个3×3矩阵的结构是相当简洁的,它们的矩阵元只有5种可能取值:0,±1,±2.其中2是反映八方晶系准晶体所具有的准周期性的特殊无理数.     

哈密顿算符的对角化与能量本征值问题的代数解法

提出了将哈密顿算符对角化的一种方法.围绕一维谐振子讨论了如何将哈密顿算符对角化、引进的是玻色算符还是费米算符的问题,并分析了能量量子化的原因及能量子与声子的区别.     

纳米晶ZrO2:Er3+-Yb3+的制备及其室温上转换发射

用化学共沉淀法制备了ZrO₂:Er³⁺-Yb³⁺纳米晶粉体，所制备的纳米晶粉体具有较强的室温上转换发射和红外发射.研究了样品的晶体结构和上转换发光性质随着Yb³⁺掺杂浓度和煅烧温度的变化关系.通过X射线衍射谱分析发现，经800℃煅烧2h后得到的ZrO₂:Er³⁺-Yb³⁺纳米晶是四方相和单斜相的混合结构，经950℃煅烧2h后得到的样品以单斜相为主，随着Y