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141.
A new united-atom force field is proposed for branched and linear alkanes. The proposed force field is used to study vapour-liquid equilibria for pure components and binary mixtures. Results of phase equilibria simulations are found to be in good agreement with available experimental data. 相似文献
142.
P. PALMIERI C. PUZZARINI V. AQUILANTI G. CAPECCHI S. CAVALLI D. DE FAZIO 《Molecular physics》2013,111(21):1835-1849
The reaction He + H+ 2(v,j = 0) → HeH+(v′ = 0, j′) for v = 0, 1,2 and 3 and for scattering energies near the threshold (0.95–1.15 eV) has been studied by calculating ab initio points at MRCI level and ‘exact’ integral quantum reactive cross-sections. More than 1400 nuclear geometries have been chosen to cover the most important regions for the dynamics, an extended set of points being taken directly on a hyperspherical coordinate grid. A many-body expansion with a large number of terms permits an accurate analytical representation of the potential energy surface with a root-mean-square deviation <12meV. The hyperquantization algorithm has been extended to obtain quantum mechanical integral cross-sections which are compared with previous calculations and with experimental results. 相似文献
143.
J. MEDINA YU. G. GUREVICH G. N. LOGVINOV P. RODRÍGUEZ G. GONZÁLEZ DE LA CRUZ 《Molecular physics》2013,111(19):3133-3138
The problem of the effective thermal diffusivity of two-layer systems is investigated using the photoacoustic spectroscopy. The experimental results are examined in terms of the effective thermal parameters of the composite system determined from a homogeneous material that produces the same physical response under an external perturbation in the detector device. It is shown that the effective thermal conductivity is not symmetric under exchange of the two layers of the composite, i.e. the effective thermal parameters depend upon which layer is illuminated in the photoacoustic experiments. Particular emphasis is given to the characterization of the interface thermal conductivity between the layer system. 相似文献
144.
This paper investigates the random buffeting excitation forces that apply to tubes in two-phase cross-flows. The spectral magnitude of these forces is studied with the help of a database that includes most of the available experimental data on direct or indirect force measurements. Different fluid mixtures, namely steam–water, air–water and various types of Freon, as well as different thermohydraulic or geometrical situations are included in the database. Using a formalism similar in principle to that used successfully in the modelling of buffeting in single-phase flows, the scaling of the data is undertaken. While dynamic pressure, viscosity or surface tension are found not to be relevant parameters, gravity forces allow us to define appropriate dimensionless spectra for all cases. The meaning of these parameters as well as the effects of flow regimes or fluid mixtures are discussed. Finally, an upper bound on the magnitude of these forces, which is of practical applicability, is proposed. 相似文献
145.
M DE SANCTIS 《Pramana》2013,81(3):467-483
Hypothetical superheavy fourth-generation fermions with a very small coupling with the rest of the Standard Model can give rise to long enough lived bound states. The production and the detection of these bound states would be experimentally feasible at the LHC. Extending, in the present study, the analysis of other authors, a semirelativistic wave equation is solved using an accurate numerical method to determine the binding energies of these possible superheavy fermion-bound states. The interaction given by the Yukawa potential of the Higgs boson exchange is considered; the corresponding relativistic corrections are calculated by means of a model based on the covariance properties of the Hamiltonian. We study the effects given by the Coulomb force. Moreover, we calculate the contributions given by the Coulombic and confining terms of the strong interaction in the case of superheavy quark bound states. The results of the model are critically analysed. 相似文献
146.
New low molar mass liquid crystalline vitrifying materials have been synthesized and tested for application in optical films. The molecules were based on spiro compounds derived from pentaerythritol and mesogenic groups derived from cyanobiphenylyl moieties. The resulting materials showed glass transition temperatures as high as 85 degrees C and nematic to isotropic phase transition temperatures up to 222 degrees C. Crystallization from the melt was strongly suppressed. Well-aligned, solid, birefringent layers were obtained from the materials by spincoating. Uniaxially oriented layers with an optic axis tilted with respect to the substrate were obtained by spincoating the liquid crystals on pretilt amplification layers. When an anisotropic dye was incorporated in the liquid crystals, polarizers with a tilted absorption axis were obtained. In addition, the compounds were found to be suitable as hosts for photo-induced reorientation of photo-isomerizable dyes. 相似文献
147.
148.
In this article, we analyze the decisional power index, the so called Hoede-Bakker index. This index takes the preferences of the players into account, as well as the social structure in which players may influence each other. We investigate the properties of the Hoede-Bakker index. We adapt some postulates for power indices and voting power paradoxes for the Hoede-Bakker set up. We investigate whether this decisional power index displays the adapted voting power paradoxes and whether it satisfies the adapted postulates for power indices. 相似文献
149.
De Paoli VM De Paoli Lacerda SH Spinu L Ingber B Rosenzweig Z Rosenzweig N 《Langmuir : the ACS journal of surfaces and colloids》2006,22(13):5894-5899
The paper describes the effect of an oscillating magnetic field (OMF) on the morphology and release properties of collagen gels containing magnetic nanoparticles and microparticles and fluorescent drug analogues. Collagen gels were prepared through fibrillogenesis of collagen in the presence of iron oxide magnetic particles averaging 10 nm or 3 mum in diameter and rhodamine-labeled dextran (Dex-R) of molecular weights between 3000-70 000 g/mol. Dextran molecules effectively simulate protein-based drugs, since they have similar molecular weights and dimensions. The paper discusses the effect of an OMF on the release properties of the gels and proposes an empirical model to predict the release rate. It also demonstrates the self-repair capability of collagen gels following the structural damage caused by an OMF. 相似文献
150.