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41.
Details are given of a selective negative-ion mass-spectrometric method appropriate for the ultratrace determination of metals and organic compounds by means of their complexes. Direct introduction of the sample into the ion-source, attachment of low-energy electrons, and selected-ion monitoring are described, and comparative data are given relating to surface effects at the tips of insertion-probes on detection limits. Detection limits for chromium and cobalt, determined as their tris(2,2,6,6-tetramethylheptane-3,5-dione) chelates, were respectively 1.0 and 0.16 pg, and that for nickel [as its bis(N,N-diethyldithiocarbamate) complex] was 1.0 pg. Detection limits of 2.0 and 1.0 ng are attainable for malathion and ethion by measurement of the nickel(II) complexes of their O,O'-dialkyldithiophosphate hydrolysis products. 相似文献
42.
43.
Morfill GE Rubin-Zuzic M Rothermel H Ivlev AV Klumov BA Thomas HM Konopka U Steinberg V 《Physical review letters》2004,92(17):175004
Fluid flow around an obstacle was observed at the kinetic (individual particle) level using "complex (dusty) plasmas" in their liquid state. These "liquid plasmas" have bulk properties similar to water (e.g., viscosity), and a comparison in terms of similarity parameters suggests that they can provide a unique tool to model classical fluids. This allows us to study "nanofluidics" at the most elementary-the particle-level, including the transition from fluid behavior to purely kinetic transport. In this (first) experimental investigation we describe the kinetic flow topology, discuss our observations in terms of fluid theories, and follow this up with numerical simulations. 相似文献
44.
45.
Malcolm H. Mac Gregor 《Foundations of Physics Letters》2004,17(4):381-391
Quantum Hall plateaus are entered via quantized cyclotron (QC) cloud-chamber orbits that have Landau-level (LL) energies and uniquely-defined angular momenta. The conservation of angular momentum in the quantum Hall system requires both canonical and magnetic angular momentum components, which add together to form the invariant kinematic angular momentum. The only LL radial eigenfunctions that satisfy the conservation-law requirements of the QC to LL transition are the u
n,l eigenstates u
n,2n+1, where n = 0, 1, 2, .... These same eigenstates uniquely have the correct scaled sizes to tile the observed families of = 1/(2n + 1) Hall plateaus. Quantum Hall plateau formation is a direct consequence of this tiling. 相似文献
46.
Enhancement of entanglement is necessary for most quantum communication protocols many of which are defined in Hilbert spaces larger than 2. In this work we present the experimental realization of entanglement concentration of orbital angular momentum entangled photons. We investigate the specific case of three dimensions and the possibility of generating different entangled states out of an initial state. The results presented here are of importance for pure states as well as for mixed states. 相似文献
47.
Valentina?CasarinoEmail author Klaus-Jochen?Engel Rainer?Nagel Gregor?Nickel 《Integral Equations and Operator Theory》2003,47(3):289-306
In this paper we convert a (linear abstract) initial boundary value
problem into an abstract Cauchy problem on some product space and use
semigroup methods to solve it. In particular, we apply spectral theory in
order to discuss stability under boundary feedback. 相似文献
48.
Let G be a complex semisimple group with real form G
. For the action of G
× G
on G by left and right translation, we define and study an orbit-type stratification of G. In particular, we compute the dimension of an arbitrary stratum; we identify certain strata of low codimension in G, the union of whose closures contains every nonprincipal stratum; and we describe the boundaries and adjacency relations of the maximal connected domains in G that contain only principal orbits. 相似文献
49.
Malcolm H. Mac Gregor 《Foundations of Physics Letters》2000,13(5):443-460
Single-wavelength Landau cyclotron orbitals (SWOs) have been used as quantum Hall basis states to reproduce integer quantum Hall plateaus in a two-dimensional (2D) close-packing representation. But at the high magnetic fields B that correspond to fractional Hall plateaus, these SWOs are too small to give close packing. It is conventionally assumed that the fractional quantum Hall states are formed from collective electron excitations (CEEs). However, by invoking the use of multiple-wavelength Landau orbitals (MWOs), we can close-pack the fractional Hall plateaus in the same manner as the integer plateaus. Quantum Hall plateaus are characterized by the filling fractions n
e/n
=k/m, where k=1, 2,... (all integers) and m=1, 3,... (all odd integers), and where n
e and n
are the 2D electron e and magnetic flux =h/e densities, respectively. A composite particle (CP) is a bound state of an electron and m flux quanta . If m is even or odd, the CP is a composite fermion (CF) or composite boson (CB). In the CEE models, both CF and CB formalisms have been used. In the alternative MWO approach introduced here, the close-packed MWOs on a =k/m plateau each contain m de Broglie wavelengths . Each MWO traps m external flux quanta, produces m diamagnetic induced flux quanta, and carries the filling fraction , which accounts for the extreme accuracy (one part in 108) of the Hall plateau conductance,
H=
e
2/h. Since m is odd, these MWOs are CB states, and they form a boson condensate of close-packed composite boson (CPCB) states. The m=1 (m<1) CPCBs tile the integer (fractional) Hall plateaus. The filling fraction index k corresponds to k layers of CPCB orbitals. Plateau formation itself is due to the linear B dependence of the density of CPCB states. The CPCBs are decoupled from the semiconductor substrate, and hence may have large m* effective mass values. THE MWOs near the =1/2 non-plateau region are m=2 CF states. 相似文献
50.
MtsslWizard is a computer program, which operates as a plugin for the PyMOL molecular graphics system. MtsslWizard estimates
distances between spin labels on proteins quickly with user-configurable options through a simple graphical interface. In
default mode, the program searches for ensembles of possible MTSSL conformations that do not clash with a static model of
the protein. Once conformations are assigned, distance distributions between two or more ensembles are calculated, displayed,
and can be exported to other software. The program’s use is evaluated in a number of challenging test cases and its strengths
and weaknesses evaluated. The benefits of the program are its accuracy and simplicity. 相似文献