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Shekhar KC Roshan K. Dhungana Namrata Khanal Prof. Ramesh Giri 《Angewandte Chemie (Weinheim an der Bergstrasse, Germany)》2020,132(21):8124-8128
We report a Ni-catalyzed regioselective α-carbonylalkylarylation of vinylarenes with α-halocarbonyl compounds and arylzinc reagents. The reaction works with primary, secondary, and tertiary α-halocarbonyl molecules, and electronically varied arylzinc reagents. The reaction generates γ,γ-diarylcarbonyl derivatives with α-secondary, tertiary, and quaternary carbon centers. The products can be readily converted to aryltetralones, including a precursor to Zoloft, an antidepressant drug. 相似文献