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71.
Electrically contacted gold-nanocluster arrays formed within electromigration-induced break junctions exhibit bright, field-dependent electroluminescence in the near infrared (650-800 nm). Intensity autocorrelation of spatially isolated individual nanocluster emission driven at high electrical frequency (f(ac)= approximately 200 MHz) reveals antibunched electroluminescence at room temperature. These results demonstrate the single quantum nature of several-atom gold molecules and suggest their use as room-temperature electrically driven single-photon sources. 相似文献
72.
73.
Jenkinson Oliver; Gonzalez Luis Felipe; Urbanski Mariusz 《Proceedings London Mathematical Society》2003,86(3):755-778
For any non-empty subset I of the natural numbers, let I denotethose numbers in the unit interval whose continued fractiondigits all lie in I. Define the corresponding transfer operator
for , where Re (rß) = I is the abscissa of convergence of the series . When acting on a certain Hilbert space HI, rß, weshow that the operator LI, rß is conjugate to an integraloperator KI, rß. If furthermore rß is real,then KI, rß is selfadjoint, so that LI, rß: HI, rß HI, rß has purely real spectrum.It is proved that LI, rß also has purely real spectrumwhen acting on various Hilbert or Banach spaces of holomorphicfunctions, on the nuclear space C [0, 1], and on the Fréchetspace C [0, 1]. The analytic properties of the map rß LI, rßare investigated. For certain alphabets I of an arithmetic nature(for example, I = primes, I = squares, I an arithmetic progression,I the set of sums of two squares it is shown that rß LI, rß admits an analytic continuation beyond thehalf-plane Re rß > I. 2000 Mathematics SubjectClassification 37D35, 37D20, 30B70. 相似文献
74.
We propose a picture of Wigner function scars as a sequence of concentric rings along a two-dimensional surface inside a periodic orbit. This is verified for a two-dimensional plane that contains a classical hyperbolic orbit of a Hamiltonian system with 2 degrees of freedom. The stationary wave functions are the familiar mixture of scarred and random waves, but the spectral average of the Wigner functions in part of the plane is nearly that of a harmonic oscillator and individual states are also remarkably regular. These results are interpreted in terms of the semiclassical picture of chords and centers. 相似文献
75.
Sun R Colin E Ajitanand NN Alexander JM Barton MA DeYoung PA Drake KL Elmaani A Gelderloos CJ Gualtieri EE Guinet D Hannuschke S Jaasma JA Kowalski L Lacey RA Lauret J Norbeck E Pak R Peaslee GF Stern M Stone NT Sundbeck SD Vander Molen AM Westfall GD Yang LB Yee J 《Physical review letters》2000,84(1):43-46
For central collisions of (17-115)A MeV 40Ar+Cu, Ag, Au, an overall balance is determined for the average mass, energy, and longitudinal momentum. Light charged particles and fragments are separated into forward-focused and isotropic components in the frame of the heaviest fragment. Energy removal by the isotropic component reaches 1-2 GeV. For such high deposition energies, statistical multifragmentation models predict much more extensive nuclear disassembly than is observed. 相似文献
76.
Fujiwara M Akimune H van Den Berg AM Cribier M Daito I Ejiri H Fujimura H Fujita Y Goodman CD Hara K Harakeh MN Ihara F Ishikawa T Janecke J Kawabata T Raghavan RS Schwarz K Tanaka M Yamanaka T Yosoi M Zegers RG 《Physical review letters》2000,85(21):4442-4445
Discrete Gamow-Teller (GT) transitions 176Yb-->176Lu at low excitation energies have been measured via the ( 3He,t) reaction at 450 MeV and at 0 degrees. For 176Yb, two low-lying states are observed, setting low thresholds Q(nu) = 301 and 445 keV for neutrino ( nu) capture. Capture rates estimated from the measured GT strengths, the simple two-state excitation structure, and the low Q(nu) in Yb-Lu indicate that Yb-based nu detectors are well suited for a direct measurement of the sub-MeV solar electron-neutrino ( nu(e)) spectrum including pp neutrinos. 相似文献
77.
D.C. Gonzalez M.E. Kiziroglou X. Li A.A. Zhukov H. Fangohr P.A.J. de Groot P.N. Barttlet C.H. de Groot 《Journal of magnetism and magnetic materials》2007
We have succeeded in aligning self-assembled structures by using a lithographically defined stripe. The 140 nm wide by 100 nm high SiO2 strip is shown to guide the assembly of 500 nm latex spheres so that spheres are aligned along the strip and are in registration on either side of the strip. This method can be used to increase long-range ordering in magnetic storage systems without compromising the density. Inverse sphere Ni arrays were made by electrodeposition through the latex template. We also show that the hexagonal symmetry of the resulting inverse sphere Ni arrays can be simulated using the approach presented below. 相似文献
78.
The reactions of the tert-butyldimethylsilylated acyloins of five-, six- and seven-membered rings with the lithium reagents of benzyltrimethylsilane, thiophenoxymethyltrimethylsilane and tri-methylsilyl acetonitrile were studied. These reactions favor formation of the substituted (Z) exo methylidene silyl ethers in moderate yields. 相似文献
79.
The bimolecular rate constants for the reactions of sulfate radicals with epicatechin (EC), epicatechingallate (ECG), and epigallocatechingallate (EGCG) were found to be (1.46 ± 0.06) × 109, (1.20 ± 0.08) × 109, and (1.04 ± 0.07) × 109, respectively. The activation energy [EA = 9 ± 3 kJ mol?1] and preexponential factor [A = (4.8 ± 0.6) × 1010] for the reaction of EC with the sulfate radical were measured in the temperature range 288–303 K. The phenoxyl radicals of EC (λmax = 310 nm) were obtained both by the reaction of this flavonoid with the sulfate radicals and by photoionization. The measured bimolecular rate constants for the reactions of the dihydrogen phosphate radicals with EC, ECG, and EGCG were (7.8 ± 0.9) × 108, (8.5 ± 0.4) × 108, and (6.8 ± 0.4) × 108, respectively. © 2010 Wiley Periodicals, Inc. Int J Chem Kinet 42: 391–396, 2010 相似文献