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971.
972.
G. M. Maksimova A. L. Chuvilin E. M. Moroz V. A. Likholobov K. I. Matveev 《Kinetics and Catalysis》2004,45(6):870-878
Conditions for the preparation of stable aqueous monometallic and bimetallic colloidal solutions (sols) of noble metals (Ru, Rh, Pd, Pt, Ir, Ag, and Au) in the presence of polyoxometalates containing W, Mo, V, and Nb were found. The stability of sols against coagulation at room temperature was studied. The metal/C samples prepared by metal adsorption from sols were studied by powder X-ray diffraction analysis and transmission electron microscopy. The following factors of importance for the preparation of a stable sol are discussed: (1) the formation of a sol of a metal polyhydroxo complex stabilized by a polyoxometalate (preliminary stage) and (2) the formation of polyoxometalate-metal clusters in the course of reduction of polyhydroxo complexes.Translated from Kinetika i Kataliz, Vol. 45, No. 6, 2004, pp. 921–929.Original Russian Text Copyright © 2004 by Maksimova, Chuvilin, Moroz, Likholobov, Matveev. 相似文献
973.
974.
975.
E. A. Bogdanov A. A. Kudryavtsev L. D. Tsendin R. R. Arslanbekov V. I. Kolobov V. V. Kudryavtsev 《Technical Physics》2003,48(9):1151-1158
Comprehensive self-consistent simulations of the positive column plasma of a dc oxygen discharge are performed with the help
of commercial CFDRC software (), which enables one to carry out computations in an arbitrary 3D geometry using fluid equations for heavy components and
a kinetic equation for electrons. The main scaling laws for the spatial distributions of charged particles are determined.
These scaling laws are found to be quite different in the parameter ranges that are dominated by different physical processes.
At low pressures, both the electrons and negative ions in the inner discharge region obey a Boltzmann distribution; as a result,
a flat profile of the electron density and a parabolic profile of the ion density are established there. In the ion balance,
transport processes prevail, so that ion heating in an electric field dramatically affects the spatial distribution of the
charged particles. At elevated pressures, the volume processes prevail in the balance of negative ions and the profiles of
the charged particle densities in the inner region turn out to be similar to each other. 相似文献
976.
The reasons for the existence of various scenarios for structural transformations in disordered condensed media, such as liquids and amorphous substances, where both smeared transformations and sharp first-order transitions may occur, were analyzed. The ratio between the spatial scale of structural correlations and the size of the smallest possible region occupied by a new phase in the matrix of initial modification is the key parameter determining the scenario for equilibrium phase transformations in liquids. In amorphous substances, the experimentally observed transformations occur far from equilibrium, and the possible size of the region occupied by the new phase corresponds to the minimal nucleus size. For some amorphous solids, quantitative analysis of the transformation width was carried out and the main classes of covalent substances, in which the smeared or sharp transitions occur, were revealed. Specific features of the interparticle interactions determining various transformation scenarios are discussed. 相似文献
977.
V. A. Bednyakov 《Physics of Atomic Nuclei》2003,66(3):490-493
One can expect accessible lower bounds for the dark matter detection rate due to restrictions on masses of the SUSY partners. To explore this correlation, one needs a new-generation large-mass detector. The absolute lower bound for the detection rate can naturally be due to spin-dependent interaction. Aimed at detecting dark matter with sensitivity higher than 10?5 event/kg/d, an experiment should have a nonzero-spin target. Perhaps, it is best to create a GENIUS-like detector with both 73Ge (high spin) and 76Ge nuclei. 相似文献
978.
The catalytic properties of cluster magnesium derivatives were studied using the self-hydrogenation reaction of unsaturated compounds as an example. In the presence of a cluster magnesium–anthracene adduct at 150–298 K, the self-hydrogenation of anthracene occurred with yields of up to 40 molecules per atom of magnesium. 相似文献
979.
V. G. Bozhkov 《Radiophysics and Quantum Electronics》2003,46(8-9):631-656
The state of the art in the development of semiconductor detectors, mixers, and frequency multipliers based on Schottky-barrier diodes (SBDs) and heterojunction structures for uncooled terahertz receivers is reviewed. The present status of this field features a transition from quasi-optical designs based on dot-matrix, whisker-contacted SBDs to the designs with hybrid-integrated and monolithic constructions on the planar SBD base, which are positioned in a waveguide mount. The high-level performance of these planar devices is achieved by partially or completely removing or changing semiconductor substrates and/or using membrane constructions incorporated in the waveguide. 相似文献
980.