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排序方式: 共有41条查询结果,搜索用时 15 毫秒
1.
Tran H Joubert P Bonamy L Lavorel B Renard V Chaussard F Faucher O Sinardet B 《The Journal of chemical physics》2005,122(19):194317
With the aim of temperature diagnostic, femtosecond time-resolved CARS (coherent anti-Stokes Raman spectroscopy) is applied to probe H2 in H2-N2 mixtures. In a first part, a Lorentzian profile is used to model the femtosecond CARS response. A difference between the experimental broadening and the expected one is observed in the collision regime. The observed broadening increases strongly in an inhomogeneous way with respect to the perturber concentration. This is of considerable importance for temperature measurements. In a second part, we show that in the collision regime, this inhomogeneous broadening is due to the speed dependence of the collisional parameters and the memory effects of the radiator speed. A new modelization of the time-resolved CARS response taking into account the speed memory effects is presented and applied to the temperature diagnostic in H2-N2 mixtures. The numerical results are in good agreement with experiments. 相似文献
2.
Alexis Bohlin Fredrik Vestin Jeanine Bonamy Pierre Joubert Per‐Erik Bengtsson 《Journal of Raman spectroscopy : JRS》2010,41(8):875-881
Rotational coherent anti‐Stokes Raman spectroscopy (CARS) in fuel‐rich hydrocarbon flames, with a large content of hydrogen in the product gases (∼20%), has in previous work shown that evaluated temperatures are raised several tens of Kelvin by taking newly derived N2 H2 Raman line widths into account. To validate these results, in this work calibrated temperature measurements at around 300, 500 and 700 K were performed in a cell with binary gas mixtures of nitrogen and hydrogen. The temperature evaluation was made with respect to Raman line widths either from self‐broadened nitrogen only, N2 N2 [energy‐corrected‐sudden (ECS)], or by also taking nitrogen broadened by hydrogen, N2 H2 [Robert–Bonamy (RB)], Raman line widths into account. With increased amount of hydrogen in the cell at constant temperature, the evaluated CARS temperatures were clearly lowered with the use of Raman line widths from self‐broadened nitrogen only, and the case with inclusion of N2 H2 Raman line widths was more successful. The difference in evaluated temperatures between the two different sets increases approximately linearly, reaching 20 K (at T ∼ 300 K), 43 K (at T = 500 K) and 61 K (at T = 700 K) at the highest hydrogen concentration (90%). The results from this work further emphasize the importance of using adequate Raman line widths for accurate rotational CARS thermometry. Copyright © 2010 John Wiley & Sons, Ltd. 相似文献
3.
B. Pietrzyk R. Barate P. Bareyre P. Bonamy P. Borgeaud M. David F.X. Gentit G. Laurens Y. Lemoigne G. Villet S. Zaninotti P. Astbury A. Duane G.J. King B.C. Nandi R. Namjoshi D.M. Websdale J. Wiejak T. Marshall 《Physics letters. [Part B]》1982,113(1):105-112
A lepton-pair trigger was used to select a hadronic system in different flavour and colour states: properties of the transformation of this system into hadrons were measured in terms of charge flow, multiplicity distribution, and fragmentation function. It is observed that, while the effects of flavour are clearly seen, the colour degrees of freedom are not observed in the region of low pT. 相似文献
4.
Célarié F Prades S Bonamy D Ferrero L Bouchaud E Guillot C Marlière C 《Physical review letters》2003,90(7):075504
We report in situ atomic force microscopy experiments which reveal the presence of nanoscale damage cavities ahead of a stress-corrosion crack tip in glass. Their presence might explain the departure from linear elasticity observed in the vicinity of a crack tip in glass. Such a ductile fracture mechanism, widely observed in the case of metallic materials at the micrometer scale, might be also at the origin of the striking similarity of the morphologies of fracture surfaces of glass and metallic alloys at different length scales. 相似文献
5.
Gallai’s path decomposition conjecture states that the edges of any connected graph on vertices can be decomposed into at most paths. We confirm that conjecture for all graphs with maximum degree at most five. 相似文献
6.
We investigate steady granular surface flows in a rotating drum and demonstrate the existence of rigid clusters of grains embedded in the flowing layer. These clusters appear to be fractal and their size is power law distributed from the grain size scale up to the thickness of the flowing layer. The implications of the absence of a characteristic length scale on available theoretical models of dense granular flows are discussed. Finally, we suggest a possible explanation of the difference between velocity profiles observed in surface flows and in flows down a rough inclined plane. 相似文献
7.
8.
The exponential perturbation approximation is tested in the semiclassical perturbed stationary states frame, using spline functions for interpolation of the non-adiabatic couplings. An application is realized for the p-H2 + 4He rotational cross sections. 相似文献
9.
We investigate the scaling properties of postmortem fracture surfaces in silica glass and glassy ceramics. In both cases, the 2D height-height correlation function is found to obey Family-Viseck scaling properties, but with two sets of critical exponents, in particular, a roughness exponent zeta approximately 0.75 in homogeneous glass and zeta approximately 0.4 in glassy ceramics. The ranges of length scales over which these two scalings are observed are shown to be below and above the size of the process zone, respectively. A model derived from linear elastic fracture mechanics in the quasistatic approximation succeeds to reproduce the scaling exponents observed in glassy ceramics. The critical exponents observed in homogeneous glass are conjectured to reflect the damage screening occurring for length scales below the size of the process zone. 相似文献
10.
Gómez L Martínez RZ Bermejo D Thibault F Joubert P Bussery-Honvault B Bonamy J 《The Journal of chemical physics》2007,126(20):204302
In this work the authors present an experimental and theoretical study about the Q-branch lines' broadening coefficients of N2 perturbed by H2. Experimental values for these parameters have been obtained at 440 and 580 K, and quantum calculations have been performed using a new ab initio potential energy surface, obtained by quantum chemistry methods. The results of these calculations are compared to experimental data obtained previously at 77 and 298 K [L. Gomez et al., Mol. Phys. 104, 1869 (2006)] and to the present measurements. A satisfactory agreement is obtained for the whole range of temperatures used in the experiments. 相似文献