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101.
Mixtures containing ammonia-borane and sec-butylamine-borane remain liquid throughout the hydrogen release process that affords tri(N-sec-butyl)borazine and polyborazylene. Concentrated solutions with metal catalysts afford >5 wt% H(2) in 1 h at 80 °C and addition of (EMIM)EtSO(4) ionic liquid co-solvent eliminates competing formation of insoluble linear poly(aminoborane) (EMIM = 1-ethyl-3-methyl-imidazolium). 相似文献
102.
103.
Dette Holger Dhar Subhra Sankar Wu Weichi 《Annals of the Institute of Statistical Mathematics》2021,73(5):855-889
Annals of the Institute of Statistical Mathematics - This article studies the problem whether two convex (concave) regression functions modelling the relation between a response and covariate in... 相似文献
104.
Subramanian V. Sankar Derek Y. Kamemoto William D. Bachalo 《Particle & Particle Systems Characterization》1993,10(6):321-331
A combined theoretical and experimental study has been conducted to evaluate the effectiveness of using large, hollow micro-balloons as LDV seed particles. The study has focused on the ability of phase Doppler systems to size hollow microballoons, the ability of large micro-balloons to respond to high frequency spatial and temporal flow field variations, and the overall advantages and disadvantages of using large microballoons instead of conventional LDV seed particles, such as very small water droplets or polystyrene latex (PSL) particles. This paper discusses the development of a theoretical phase Doppler response model for stratified spheres, the experimental facility, and the theoretical and experimental results. 相似文献
105.
106.
We present a complete theoretical analysis of the periodic and non-periodic travelling waves in a diatomic chain model, in
the continuum limit by incorporating nonlinear sixth order polarization potential (φ6) at the anion site. We have formulated a nonlinear lattice dynamical theory in which various energy curves are obtained for
different types and magnitudes of the core-shell force constants. For periodic solutions, we have obtained two types of commensurate
wave amplitudes which propagate in the opposite direction with respect to each other. For nonperiodic solutions, we have obtained
various travelling excitations such as kink, antikink, excitons etc. for different values of the mass ratio and velocity parameter.
The dipole moment per unit charge for SrTiO3 has been calculated and it is found that the nonlinear excitations in this model carry large amount of energy as compared
to those obtained from harmonic and anharmonic optical phonons in the φ4-polarizable model. 相似文献
107.
The phonon spectra of unstrained and strained quasiperiodic semiconductor superlattices (QSSL) have been calculated using
one-dimensional linear chain model. We consider two types of quasiperiodic systems, namely cantor triadic bar (CTB) and Fibonacci
sequences (FS), constituting of AlAs, GaAs and GaSb of which the latter two have a lattice mismatch of about 7%. The calculations
have been made using transfer matrix method and also with and without the inclusion of strain. We present the results on phonon
spectra of two component CTB and two as well as three component FS semiconductor superlattices (SSL), thickness and order
dependence on LO mode of GaAs, effect of strain on LO frequency of GaAs. The calculated results show that the strain generated
due to lattice mismatch reduces significantly the magnitudes of the confined optical phonon frequency of GaAs. 相似文献
108.
We have investigated the lattice vibrational properties of a two-component strained layer semiconductor superlattice (GaAs)
n1 (GaSb)
n2 using a one-dimensional linear chain model and transfer matrix method [1]. Effect of strain, arising due to the lattice mismatch
(∼ 7%) has been considered explicitly in the equation of motion. We show for the first time that the optical vibrational frequency
increases (in the case of (GaAs)4 (GaSb)
n
) or decreases (in the case of (GaAs)
n
(GaSb)4) with increase of layer thicknessn, in either type of superlattices. Raman scattering measurements on some other similar systems support our findings. 相似文献
109.
We have calculated the phonon and periodon dispersion relations in IV–VI semi-conducting bulk PbTe and SnTe and their superlattice
structure. The model used here is a one-dimensional lattice which includes harmonic interactions up to second neighbours as
well as on-site nonlinear electron-ion interactions at the anion site. We calculate the phonon and periodon dispersion relations
in bulk and PbTe-SnTe superlattice for the transverse optic and acoustic modes using the transfer matrix method. Our analysis
has predicted correct nature of the folding of acoustic and confinement of optical phonons at various frequency intervals
corresponding to pass and stop bands of the superlattices. 相似文献
110.