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991.
The mechanism of ozone formation has been studied using 16O and 18O2. High-resolution microwave spectroscopy was used to measure the amounts of the isotopomeric ozone species formed. The study is hampered by the very rapid exchange process between the reactants, that tends to scramble the isotopes and hence give a 2:1 statistical ratio between the two possible isotopomers. We have found a strategy to come around this difficulty and conclude that the mechanism is a simple end-on-addition. 相似文献
992.
993.
It is shown that using position-sensitive detectors in μSR experiments to determine the muon stopping site in a target permits
one to study correlation effects in μSR time histograms produced by the decay of muons stopping in the same domain, i.e. to
obtain time correlators of μSR histograms of decays from a small region. These correlators contain information on the spatial
correlation of magnetic fields in the sample under study. The proposed method (μSR2-technique) allows measuring correlation radii (r
c
) down to 10−5 cm in a bulk sample. Among interesting physical phenomena occuring overr
c≥3×10−6 cm are, for instance, long wavelength fluctuations of the order parameter near the phase transition point in ferromagnets
and antiferromagnets and magnetic field correlations in magnet domains and spin glasses. One may use this method also on heavy-current
accelerators producing pulsed muon beams to investigate the variation in time of spatial correlations in magnets, spin glasses
and superconductors. 相似文献
994.
A method of identifying low-energy nuclei from the readings of an ionizational mass spectrometer is considered. The identification principles for particles recorded by a multilayer detector are discussed, together with the fundamentals of a probabilistic approach to the solution of this problem. The method permits correct analysis of the experimental data obtained. The determination of the charge and isotopic composition of radiation consisting of a mixture of different nuclei is considered. The results of calculations by the given method which permit the determination of the optimal detector parameters for the solution of the specific physical problem are outlined. This approach is also applicable for the analysis of data from other types of measuring apparatus.Translated from Izvestiya Vysshikh Uchebnykh Zavedenii, Fizika, No. 7, pp. 84–88, July, 1991. 相似文献
995.
N. Gass 《The Journal of the Operational Research Society》1994,45(2):133-142
A methodology is developed to analyse present and future crisis and conflict potentials of small or large geopolitical regions. A set of criteria is used to describe the present economic, social, political and military conditions of a country and the future criteria trends. A multi-criteria decision analysis model is invoked to compute the crisis and conflict potentials under simultaneous consideration of all other countries in that region. The methodology is demonstrated in the crisis and conflict potentials analysis of the former Soviet republics including bordering countries. 相似文献
996.
Rate constants have been measured by pulse radiolysis for the reactions of the carbonate radical, CO3·?, with a number of organic and inorganic reactants as a function of temperature, generally over the range 5 to 80°C. The reactants include the substitution-inert cyano complexes of FeII, MoIV, and WIV, the simple inorganic anions SO32?, ClO2?, NO2?, I?, and SCN?, several phenolates, ascorbate, tryptophan, cysteine, cystine, methionine, triethylamine, and allyl alcohol. The measured rate constants ranged from less than 105 to 3 × 109 M?1 s?1, the activation energies ranged from ?11.4 to 18.8 kJ mol?1, and the pre-exponential factors ranged from log A = 6.4 to 10.7. The activation energies for the metal complexes and inorganic anions generally decrease with increasing driving force for the reaction, as expected for an outer sphere electron transfer. For highly exothermic reactions, however, the activation energy appears to increase, probably reflecting the temperature dependence of diffusion. For many of the organic reactants, the activation energies were low and independent of driving force, suggesting that the oxidation is via an inner sphere mechanism. 相似文献
997.
998.
O. P. Gorelik G. A. Dyuzhev D. V. Novikov V. M. Oichenko A. A. Sitnikova 《Technical Physics》2002,47(10):1337-1340
Electron microscopy is used in a study of nanoclusters of the carbon soot deposited on a probe in different areas of arc discharge during graphite vaporization under conditions favorable for fullerene synthesis. It is found that the spatial network of soot nanoclusters consists of alternating regions of higher density or associates of carbon particles. Two types of nanoclusters have been identified with the correlation radii of the associates equal to 0.6–0.8 and 1.6–2.2 nm, respectively. Type I nanoclusters are dominant in the soot microparticles, and their structure shows practically no variations with increasing separation r of the soot collector from the discharge axis over the range of distances studied, r=1–9 cm. The effective radius R 0 of the “elementary” particles making up the associates in the soot nanoclusters of Type I calculated with the use of scaling relationships is 0.15–0.17 nm and is close to the gas-kinetic radius of carbon atoms. Type II nanoclusters have been identified in soot collected at r>3 cm. Values of R 0 calculated in this case are 0.6–0.9 nm and decrease with increasing r, which indicates the presence of fullerene molecules in these nanocluster associates. 相似文献
999.
Godwin J. Udo 《The Journal of the Operational Research Society》1994,45(12):1425-1435
This paper is a report of a simulation study that investigates a dynamic approach to scheduling jobs in a multi-machine job shop. The workload information of a job is used in different forms to evaluate the shop performance based on three measures: mean job lateness, percentage of tardy jobs and lateness variance. Different combinations of due-date assignment methods and sequencing rules are compared based on specific performance criteria. The results indicate that using the cumulative distribution function of workload information can yield a better performance than using a proportional function of workload information or ignoring shop congestion information. A few situations are identified in which workload information is not critical. 相似文献
1000.
S. E. Kholodovskii 《Journal of Applied Mechanics and Technical Physics》1991,32(6):931-933
Translated from Prikladnaya Mekhanika i Tekhnicheskaya Fizika, No. 6, pp. 119–122, November–December, 1991. 相似文献