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131.
Hans-Detlev Gilsing Jürgen Angerer Dietrich Prescher 《Monatshefte für Chemie / Chemical Monthly》2003,134(9):1207-1213
Summary. Two ring-deuterated major metabolites of bis(2-ethylhexyl) phthalate were obtained in excellent yields by means of an improved oxidation procedure. The by-product of their interconversion by Swern oxidation is elucidated and a possible mechanism of its formation is proposed.Received February 27, 2003; accepted March 3, 2003
Published online July 28, 2003 相似文献
132.
A complex spectral grating is accumulated by repeated application of a pair of low-power optical programming pulses to a short-term persistent inhomogeneously broadened transition in Tm:YAG at 4.5 K and then probed to investigate the buildup dynamics. The necessary frequency stability is obtained by locking a cw Ti:sapphire laser to a regenerating transient spectral hole in the same transition. Grating accumulation is demonstrated for both a periodic spectral grating, representing a true-time delay, and a complex spectral grating, permitting correlation-based pattern recognition. This work is a step toward demonstrating an optical coherent transient continuously programmed continuous processor. 相似文献
133.
采用多级方案是高频脉冲管制冷机获得低于20 K以下制冷温度的主要方法,以不锈钢金属丝网为蓄冷材料的二级高频脉冲管制冷机,实验已经达到了20 K以下温度.理论上讲,由于热容大,以铅为主的蓄冷材料比不锈钢更适合40~10 K温区工作,这在低频回热制冷机中得到了证明.本文介绍了我们采用不同铅球和铅网为低温蓄冷材料的研究结果.实验表明,小铅球对于高频脉冲管制冷机是不很合适的,导致制冷温度的明显升高.镀铅的不锈钢丝网和已有不锈钢丝网的性能相似,可进一步深入研究.该研究对于20 K以至更低温度的高频回热制冷机研究有一定的借鉴意义. 相似文献
134.
Three-dimensional linearised Euler model simulations of sound propagation in idealised urban situations with wind effects 总被引:1,自引:0,他引:1
Dietrich Heimann 《Applied Acoustics》2007,68(2):217-237
A three-dimensional numerical time-domain model based on the linearised Euler equation is applied to idealised urban situations with elongated, isolated buildings beside a straight street with sound emissions. The paper aims at the investigation of principle relationships between the source-receiver geometry (street and building facades) and sound propagation under the consideration of ground and wind. By applying cyclic lateral boundary conditions for either one or both horizontal co-ordinates, two different idealised urban environments were considered: a single street and parallel streets. Numerical experiments were performed to elaborate the effects of different roof types, ground properties, wind flow, and turbulence in both urban environments with the focus on the back facades (‘quiet’ sides) of the buildings. As a result it was found that the back facades of flat-roof buildings are quieter than those of hip roof buildings despite equal cross-cut areas. The wind effect (resulting in quieter upwind and louder downwind facades) is more pronounced for hip-roof buildings. In the case of parallel streets upwind facades are slightly louder than downwind facades because they are simultaneously exposed to downwind propagating sound from the next parallel street. 相似文献
135.
Brandon J. O'Neill David H. K. Jackson Dr. Anthony J. Crisci Carrie A. Farberow Fengyuan Shi Dr. Ana C. Alba‐Rubio Dr. Junling Lu Dr. Paul J. Dietrich Dr. Xiangkui Gu Dr. Christopher L. Marshall Prof. Peter C. Stair Dr. Jeffrey W. Elam Dr. Jeffrey T. Miller Prof. Fabio H. Ribeiro Prof. Paul M. Voyles Prof. Jeffrey Greeley Prof. Manos Mavrikakis Prof. Susannah L. Scott Prof. Thomas F. Kuech Prof. James A. Dumesic 《Angewandte Chemie (International ed. in English)》2013,52(51):13824-13824
136.
John Conrad Merkel 《Journal of Dynamics and Differential Equations》2008,20(3):653-668
In the spirit of Palmore and Pacella, Morse Theory is used to obtain a lower bound for the number of central configurations
in the spatial N-body problem. The homology of the configuration ellipsoid with the collision and collinear manifolds removed and the SO(3) symmetry quotiented out is calculated. As intermediate steps, homology calculations are carried out for several additional
manifolds naturally arising in the N-body problem. 相似文献
137.
A scheme for systematic reduction of the theoretical treatment of elementary reactions involving polyatomic molecules is described; it consists of (1) limitation to the energetically relevant regions of the nuclear configuration space (the reaction path and its near environs) and (2) restriction to the dynamically relevant subspace of the nuclear configuration space (the active modes). Starting from a generalized reaction path Hamiltonian of Nauts and Chapuisat allowing for the use of arbitrary curvilinear coordinates and several large-amplitude modes, the realization of the above-sketched scheme is discussed. A compilation of recent work along these lines, mostly based on the simplified Miller-Handy-Adams reaction path Hamiltonian, is given with particular emphasis on applications of a statistical adiabatic model. 相似文献
138.
139.
L. de Arcangelis H. J. Herrmann M. Kolb René Thomas C. Amitrano L. Peliti M. Saber G. Weisbuch Sara A. Solla F. Bagnoli A. Francescato R. Livi S. Ruffo Pablo Tamayo Michel Droz Peter Jörg Plath S. Romano Yves Pomeau Stéphane Zaleski D. Stauffer Luciano R. da Silva Alex Hansen Stéphane Roux Antonio Coniglio B. Derrida Henrik Flyvbjerg Naeem Jan Dietrich Stauffer Peter Grassberger A. Zippelius K. E. Kurten Werner Krauth Jean -Pierre Nadal Marc Mézard Per Bak Chao Tang Itzhak Webman M. L. Martins H. F. V. Resende C. Tsallis A. C. N. Magalhaes 《Journal of statistical physics》1989,55(5-6):1333-1359
140.