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111.
A wavefunction used in an earlier calculation of the nuclear shielding of the hydrogen molecule has been tested by comparing the calculated magnetic susceptibility against that of Kolos and Wolniewicz. Good agreement is obtained. The procedure of Herman and Short for averaging over the nuclear motion has also been tested by comparing the predicted susceptibilities of H2, Hd and D2 with those obtained from averages of the Rydberg-Klein-Rees potential curves by Jain and Sahni. Again, good agreement is found.For the first time calculated values have been obtained for the susceptibilities of the isoropomers of hydrogen which contain tritium. It is predicted that accurate susceptibility measurements should not only be able to distinguish between all the various isotopomers but should also detect the temperature dependence of the susceptibility of any one isotopomer. 相似文献
112.
Mean lifetimes of levels in 22Ne have been measured by the Doppler-shift attenuation method using the inverse reaction 4He(19F, pγ)22Ne. The Doppler-broadened lineshapes observed at 0° were analyzed using scaled experimental stopping powers and give the following results for each of the following levels (energy in keV and lifetime in fs): 4457 ( < 15), 5147 (1300 ± 500), 5522 (27 ± 4), 5641 ( < 20), 6311 (70 ± 10), 6345 ( < 15), 6636 ( < 20) and 6817 ( < 15). The lifetime of the 6311 keV 6+ level is particularly interesting for testing model predictions. The large basis shell model calculations of Preedom and Wildenthal are in good agreement with the experimental B(E2) values for the 2+, 4+ and 6+ members of the ground-state band. 相似文献
113.
B. Davies 《Physics letters. A》1974,48(4):298-300
We show that the Lifshitz and related theories of intermolecular interactions are equivalent to perturbation theory, and therefore subject to the usual restrictions of the latter. 相似文献
114.
R. D. Davies 《Journal of separation science》1981,4(6):270-275
This contribution comprises two parts, the one covering some variables in the dry-packing of columns for liquid chromatography, the other the use of an automatic dry-packer in liquid chromatography. A high-pressure stainless steel column was dry-packed using a 20-44 μm size, irrregularly shaped, silica gel support. It was found that, when support was added in discrete amounts, lateral tapping produced a column of higher efficiency (HETP = 0.69 mm) than was the case for vertical tapping (HETP = 1.37 mm). Simultaneous vertical and lateral tapping produced an intermediate result. Bulk filling of the column followed by tapping was inferior to adding support in discrete amounts. An apparatus constructed to perform the vertical and lateral tapping operations automatically confirmed the above conclusions. It was concluded that commercially available dry-packing apparatus do not offer the best action for packing an efficient column since they involve predominantly vertical tapping. 相似文献
115.
C.J. Batty S.F. Biagi M. Blecher R. Kunselman R.A.J. Riddle B.L. Roberts J.D. Davies G.J. Pyle G.T.A. Squier D.M. Asbury M. Leon 《Nuclear Physics A》1978,296(3):361-372
The attenuation due to the E2 nuclear resonance effect has been measured in hadronic atoms using pions with 111Cd and 112Cd, and for kaons with 122Sn. Energies of the relevant X-ray and γ-ray transitions and of the X-ray cascade intensities have also been measured so as to give a self-consistent set of information. The results are found to be in very good agreement with theoretical calculations. 相似文献
116.
E. B. Davies 《Communications in Mathematical Physics》1970,19(2):83-105
We investigate properties of a class of quantum stochastic processes subject to a condition of irreducibility. These processes must be recurrent or transient and an equilibrium state can only exist in the former case. Every finite dimensional process is recurrent and it is possible to establish convergence in time to a unique equilibrium state. We study particularly the class of transition processes, which describe photon emissions of simple quantum mechanical systems in excited states.Work supported by U.S.A.F. contract number F 44620-67-C-0029. 相似文献
117.
This paper describes the design, construction and use of a field-cycled proton-electron double-resonance imaging (FC-PEDRI) system for the detection and imaging of free radicals. The unique feature of this imager is its use of a 450-mT detection magnetic field in order to achieve good image quality and sensitivity. The detection magnetic field is provided by a superconducting magnet, giving high stability and homogeneity. Field cycling is implemented by switching on and off the current in an internal, coaxial, resistive secondary magnet that partially cancels the superconducting magnet's field at the sample; the secondary magnet is actively shielded to avoid eddy currents. EPR irradiation takes place at approximately 5 mT, following which the field is switched to 450 mT in 40 ms for NMR signal detection. Full details of the imager's subsystems are given, and experiments to image the distribution of stable free radical contrast agents in phantoms and in anesthetized rats are described. 相似文献
118.
[1-14C]-E-dehydromatricaria methyl ester and dimethyl [1-14C]-deca-4,6,8-triyne-1,10-dioate are incorporated into the allene (-)-marasin in Marasmius ramealis without scrambling of the 14C label. This and the levels of the incorporations (0.8% and 4.9% respectively) strongly suggests that the above esters, or close relatives, can be converted directly into (-)-marasin in M. ramealis, and that the diyne-allene moiety in this latter compound arises by the rearrangement, under enzymic control, of an alkyltriyne moiety. 相似文献
119.
Allison IF Davies CT Gray A Kronfeld AS Mackenzie PB Simone JN;HPQCD;Fermilab Lattice;UKQCD 《Physical review letters》2005,94(17):172001
We use lattice QCD to predict the mass of the Bc meson. We use the MILC Collaboration's ensembles of lattice gauge fields, which have a quark sea with two flavors much lighter than a third. Our final result is mBc = 6304+/-12(+18)(-0) MeV. The first error bar is a sum in quadrature of statistical and systematic uncertainties, and the second is an estimate of heavy-quark discretization effects. 相似文献
120.
Beşli S Coles SJ Davies DB Hursthouse MB Ibişoglu H Kiliç A Shaw RA 《Chemistry (Weinheim an der Bergstrasse, Germany)》2004,10(19):4915-4920
X-ray crystallographic evidence shows that nucleophilic substitution reactions of two different types of cyclophosphazene derivatives with relatively rigid nine-membered ansa rings leads to the first demonstration of retention of configuration in these molecular systems. 相似文献