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971.
Lance Nielsen 《Mathematical Physics, Analysis and Geometry》2011,14(4):279-294
In this paper we investigate the relation between weak convergence of a sequence \(\left\{ \mu_{n}\right\} \) of probability measures on a Polish space S converging weakly to the probability measure μ and continuous, norm-bounded functions into a Banach space X. We show that, given a norm-bounded continuous function f:S→X, it follows that \(\lim_{n\to\infty}\int_{S}f\, d\mu_{n}=\int_{S}f\, d\mu\)—the limit one has for bounded and continuous real (or complex)—valued functions on S. This result is then applied to the stability theory of Feynman’s operational calculus where it is shown that the theory can be significantly improved over previous results. 相似文献
972.
Zhan-Shuo Hu Fei-Yi Hung Shoou-Jinn Chang Kuan-Jen Chen Yi-Wei Tseng Bohr-Ran Huang Bo-Cheng Lin Wei-Yang Chou Jay Chang 《Journal of nanoparticle research》2011,13(10):4757-4763
The photo-current of n-ZnO/p-Si heterojunction photodiodes was improved by embedding Ag nanoparticles in the interface (ZnO/nano-PAg/p-Si), and the ratio between photo- and dark-current increased by about three orders more than that of a n-ZnO/p-Si specimen. The improvement in the photo-current resulted from the light scattering of embedded Ag nanoparticles. The I–V curve of n-ZnO/p-Si degraded after thermal treatment (A-ZnO/p-Si) because the silicon robbed the oxygen from ZnO to form amorphous silicon dioxide and left an oxygen vacancy. Notably,
the properties of ZnO/nano-PAg/p-Si were better in the time-dependent photoresponse under 10 V bias. Ag nanoparticles (15–20 nm) scattered the UV light randomly
and increased the probability for the absorption of ZnO to enhance the properties of the photodiode. 相似文献
973.
A green method, using pulsed spark-discharge (PSD) to synthesize gold nanoparticles (AuNPs) in ethanol, is studied in this
article. Unlike conventional methods for metal nanoparticles synthesis, the PSD method does not require the addition of chemical
surfactants and stabilizers. The size of PSD–AuNPs is examined by transmission electron microscopy, with a range 5–50 nm.
The chemical compounds, crystal structure, and surface plasmon resonance of PSD–AuNPs are studied using energy dispersive
X-ray spectroscopy, X-ray diffraction, and UV–Visible spectroscopy, respectively. Zeta potential analysis shows that a negative
charge (−40 mV) on the surface of the PSD–AuNPs may be contributing to the stability of the suspension. During the gold electrodes
discharge in the ethanol, under an intensive electric field and thermal energy, bulk metallic gold and ethanol may produce
AuNPs and varieties of chemical derivatives, which are also studied by GC/MS and FTIR to investigate the suspension mechanism.
The analysis results show that there is an oxidation reaction of ethanol occurring during the PSD process to produce ethanol
derivatives, such as acetaldehyde, acetic acid, and ethyl acetate, which may modify the surface of AuNPs by coordination of
oxygen atoms. However, only acetic acid can form a negative charge by the deprotonation of the carboxylic group of surface
in ethanol, resulting in the creation of a repulsion force between the particles to form the stable colloid system. The experimental
results indicate that PSD is an alternative green process to synthesize gold nanoparticles suspension in ethanol. Moreover,
with a gold rod consumption rate of 15 mg/L, concentrations of gold nanoparticles ~9 ppm have been observed; therefore, the
net production rate is around 60%. 相似文献
974.
Wen-ting Xu Hai-ling Tu Da-li Liu Ran Teng Qing-hua Xiao Qing Chang 《Journal of nanoparticle research》2011,13(12):7095-7098
An innovative fabrication technique for the nanometer-sized SiGe/Si heterostructure was developed in this study. Ge was induced
in Si substrate by two-step ion implantation. The spherical SiGe nanoclusters are self-assembled in the Si substrate by subsequent
rapid thermal annealing at 1,100 °C. The diameter of the spherical SiGe nanoclusters is 5–7 nm. Visible photoluminescence
from this nanometer-sized SiGe/Si heterostructure at room temperature was investigated. We found three peak energies of visible
luminescence spectra at 1.97, 2.13, and 2.16 eV, respectively. The luminescence intensity depends on the number of the nanoclusters
and will be decreased because of the micro-defects around the heterostructure, which is discussed in detail. 相似文献
975.
Khaled Habib 《Optical Review》2011,18(4):324-330
A critical (steady state) value of the thermal expansion coefficients of different coatings was determined by a nondestructive
technique (NDT) known as laser shearography. The behavior of organic coatings, i.e., ACE premium-grey enamel, a yellow acrylic
lacquer, and a gold nail polish on a metallic alloy, i.e., a carbon steel, was investigated over a temperature range of 20–60
°C. The value of the thermal expansion coefficients of coatings was derived from the slope of the plot of the thermal deformation
(strain) versus the applied temperature. The integrity of the coatings with respect to time was assessed by comparison the
measured coefficients of thermal expansion (CTE) to the critical (steady state) or asymptotic value of CTE. By shearography,
measurement of coating properties could be performed independent of parameters such as UV exposure, humidity, presence of
chemical species, and other parameters which may normally interfere with conventional methods of the assessing of the integrity
of coatings. Therefore, one may measure CTE of coatings, regardless of the history of the coating, in order to assess the
integrity of coatings. Also, the obtained shearography data were found to be in a reasonable trend with the data of electrochemical
impedance spectroscopy (EIS) in 3%NaCl solution. 相似文献
976.
Gold,silver, and palladium nanoparticle/nano-agglomerate generation,collection, and characterization
Sunita R. Boddu Veera R. Gutti Tushar K. Ghosh Robert V. Tompson Sudarshan K. Loyalka 《Journal of nanoparticle research》2011,13(12):6591-6601
Generation, collection, and characterization of gold, silver, and palladium nanoparticles and nano-agglomerates (collectively
“nanoparticles”) have been explored. The nanoparticles were generated with a spark aerosol generator (Palas GFG-1000). They
were collected using a deposition cell under diffusion and thermophoresis. The shapes and sizes of the deposited particles
were measured using transmission electron microscopy (TEM). TEM images showed that the particles were in the range of 8–100 nm
in diameter, and their shapes varied from nearly spherical to highly non-spherical. Thermophoresis enhanced the deposition
of nanoparticles (over the diffusive or the isothermal deposition) in all cases. Further, the size distributions of the nanoparticles
generated in the gas phase (aerosol) were measured using a scanning mobility particle sizer (SMPS 3080, TSI) spectrometer.
The SMPS results show that an increase in the spark frequency of the generator shifted the size distributions of the nanoparticles
to larger diameters, and the total particle mass production rate increased linearly with increase in the spark frequency.
The computational fluid dynamics code Fluent (Ansys) was used to model the flow in the deposition cell, and the computed results
conform to the observations. 相似文献
977.
Guadalupe Valverde-Aguilar Jorge A. García-Macedo Víctor M. Rentería-Tapia Raúl W. Gómez Manuel Quintana-García 《Journal of nanoparticle research》2011,13(10):4613-4622
Hexagonal mesostructured films containing silver ions were obtained by sol–gel method. Brij 58 was used to produce channels
into the film, which house these ions. The films were exposure to UV radiation to produced silver metallic nanoparticles.
The presence of the metallic nanoparticles was determined by infrared spectroscopy and optical absorption. Besides, these
nanoparticles and core–shell structures of silver–silver oxide nanoparticles were identified by high-resolution transmission
electronic microscopy. From these measurements, the obtained size range for silver nanoparticles was 6.1 nm. The absorption
spectrum located at 440 nm was modelled and well fitted with the Gans theory considering refractive index higher than the
one coming from host matrix. This index is explained because the silver oxide shell modifies the local surrounding medium
of the metallic nanoparticles. 相似文献
978.
A cathode material of an electrically conducting carbon–LiFePO4 nanocomposite is synthesized by wet ball milling and spray drying of precursor powders prior to a solid-state reaction. The
structural characterization shows that the composite is composed of LiFePO4 crystals and 4.8 wt.% amorphous carbon. Galvanostatic charge/discharge measurements indicate that the composite exhibits
a superior high energy and high cycling stability. This composite delivers a discharge capacity of 159.1 mAh g−1 at 0.1 C, 150.8 mAh g−1 at 1 C, and 140.1 mAh g−1 at 2 C rate. The capacity retention of 99% is achieved after 200 cycles at 2 C. The 18,650 cylindrical batteries are assembled
using the composite as cathode materials and demonstrate the capacity of 1,400 mAh and the capacity retention of 97% after
100 cycles at 1 C. These results reveal that the as-prepared LiFePO4–carbon composite is one of the promising cathode materials for high-performance, advanced lithium-ion batteries directed
to the hybrid electric vehicle and pure electric vehicle markets. 相似文献
979.
Deokki Min Nils Hoivik Geir Uri Jensen Frode Tyholdt Camilla Haavik Ulrik Hanke 《Applied Physics A: Materials Science & Processing》2011,105(4):867-874
The dielectric properties of zirconium dioxide (ZrO2) ceramic thin films were characterized up to 50 GHz using coplanar waveguides (CPWs) and metal–insulator–metal (MIM) capacitors
with top circular electrodes. The ZrO2 films were deposited using a chemical solution onto high-resistivity Si wafers and metal layers. The real part of the dielectric
constant of approximately 22 and 26 was extracted at 50 GHz for CPW and MIM structures, respectively, and the loss tangent
was approximately 0.09 at 50 GHz. C–V and I–V measurements were carried out to determine low-frequency and DC dielectric properties. The measurement results indicate that
ZrO2 is a promising material to be used as a dielectric layer for radio-frequency (RF) microelectromechanical systems (MEMS) capacitive
switches. 相似文献
980.
J. Babington B. A. van Tiggelen 《The European Physical Journal D - Atomic, Molecular, Optical and Plasma Physics》2011,65(3):367-372
We consider a simple atomic two-body bound state system that is overall charge neutral
and placed in a static electric and magnetic field, and calculate the magneto-electric
response function as a function of frequency. This is done from first principles using a
two-particle Hamiltonian for both an harmonic oscillator and Coulomb binding potential. In
the high frequency limit, the response function falls off as
1/ω
2 whilst at low frequencies it tends to a constant
value. 相似文献