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21.
The theory for a general departure function, f, for laser-irradiated cavities was previously developed to estimate laser energy coupling to an opaque solid target as a function of heat transfer and the cavity shape and size. In this article, a specific form of f is calculated for ultraviolet (UV) laser ablation of copper (Cu) and aluminum (Al) targets. Methods are also given for calculating the geometric factor, a, and experimentally determining the heat transfer parameter, ν, which is shown for this form of f to be the intensity-dependent effective reflectivity of the material. Experimental results for different gauges of laser energy coupling with a solid target are given and compared to calculations of net absorbed energy based on f and the incident laser energy. Using the simplified cavity analysis, the results demonstrate that the experimental values for f fall within the limits predicted by the theory, and that energy coupling can be predicted to within a mean of 2% of experimental gauges. Neglecting the factors in f from calculations of energy coupling can lead to large errors for laser-irradiated cavities, establishing that both cavity shape and heat transfer should be simultaneously considered. In addition, a first-order sensitivity analysis based on f shows that the initial rate of change in material removal strongly increases with reflectivity, which can lead to runaway cavity formation for highly reflective materials. 相似文献
22.
The general strategy to construct D-A type conjugated polymers is alternating copolymerization of electron-donating(D)monomer and electron-accepting(A) monomer. In this article, we report a new strategy to develop D-A type conjugated polymers, i.e. first fuse the D and A units into a polycyclic structure to produce a building block and then polymerize the building block with another unit. We develop a new building block with ladder structure based on B←N unit, B←N bridged dipyridylbenzene(BNDPB). In the skeleton of BNDPB, one diamine-substituted phenylene ring(D unit) and two B←N-linked pyridyl rings(A unit) are fused together to produce the polycyclic structure. Owning to the presence of intramolecular D-A character, the building block itself exhibits narrow bandgap of 1.74 eV. The conjugated polymers based on BNDPB show unique electronic structures, i.e. localized HOMOs and delocalized LUMOs, which are rarely observed for conventional D-A conjugated polymers. The polymers exhibit smaller bandgap than that of the building block BNDPB and display near-infrared(NIR)light absorption(λabs=ca. 700 nm). This study thus provides not only a new strategy to design D-A conjugated polymers but also a new kind of building block with narrow bandgap. 相似文献
23.
This paper further investigates the lag synchronization of coupled delayed systems with parameter mismatch. Different from the most existing results, we formulate the intermittent control system that governs the dynamics of the synchronization error. As a result of parameter mismatch, complete lag synchronization cannot be achieved. In this paper, a lag quasisynchronization scheme is proposed to ensure that coupled systems are in a state of lag synchronization with an error level. We estimate the error bound of lag synchronization by rigorously theoretical analysis. Numerical simulations are presented to verify the theoretical results. 相似文献
24.
超分子聚合物,即单体通过非共价键作用连接而成的链状聚集体,具有独特的物化性质和功能.经过30年的发展,超分子聚合物领域已取得了一系列重大创新成果.目前,超分子聚合物领域亟需探索的问题主要在超分子聚合驱动力、超分子构筑基元、可控超分子聚合、超分子聚合物功能等方面.近期,荷兰埃因霍温理工大学的Meijer课题组和日本名古屋... 相似文献
25.
用准连续60W的二极管激光列阵侧面泵浦“之”字形Nd:YAG板条激光器,当泵浦功率为45W,脉宽为400μs时,得到3.5mJ的激光输出。用KD*P电光开关调Q,得到18ns(FWHM)、2mJ的脉冲激光输出,用KTP晶体作腔内倍频,得到15ns、0.85mJ的二次谐波激光输出。在腔内无调Q元件且腔长小于5cm时,于近阈值处得到单频绿光输出,而当泵浦功率稍大,腔内有数个纵模振荡时,观察到激光的反相态,并用数值模拟的结果对此作了解释。 相似文献
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The issue of impulsive synchronization of a class of chaotic systems is investigated. Based on the impulsive theory and linear matrix inequality technique, some less conservative and easily verified criteria for impulsive synchronization of chaotic systems are derived. The proposed method is applied to the original Chua oscillators, and the corresponding synchronization conditions are obtained. Moreover, the boundary of the stable region is also estimated in terms of the equidistant impulse interval. The effectiveness of our method is shown by computer simulation. 相似文献
29.
The problems of control and synchronization of a class of chaotic systems with time delay via the impulsive control approach are investigated. Based on the Lyapunov-like stability theory for impulsive functional differential equations, several sufficient conditions are derived to guarantee chaos control and synchronization. Furthermore, we address the chaos quasisynchronization in the presence of single-parameter mismatch. Several illustrated examples are also given to show the effectiveness of the proposed methods. 相似文献
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