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951.
ABSTRACTThe stable configurations, electronic structures and catalytic activities of single-atom metal catalyst anchored silicon-doped graphene sheets (3Si-graphene-M, M?=?Ni and Pd) are investigated by using density functional theory calculations. Firstly, the adsorption stability and electronic property of different gas reactants (O2, CO, 2CO, CO/O2) on 3Si-graphene-M substrates are comparably analysed. It is found that the coadsorption of O2/CO or 2CO molecules is more stable than that of the isolated O2 or CO molecule. Meanwhile, the adsorbed species on 3Si-graphene-Ni sheet are more stable than those on the 3Si-graphene-Pd sheet. Secondly, the possible CO oxidation reactions on the 3Si-graphene-M are investigated through Eley–Rideal (ER), Langmuir–Hinshelwood (LH) and new termolecular Eley–Rideal (TER) mechanisms. Compared with the LH and TER mechanisms, the interaction between 2CO and O2 molecules (O2?+?CO → CO3, CO3?+?CO → 2CO2) through ER reactions (< 0.2?eV) are an energetically more favourable. These results provide important reference for understanding the catalytic mechanism for CO oxidation on graphene-based catalyst. 相似文献
952.
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955.
为消除传统单元中心型Godunov方法在求解稀疏波问题时的非物理过热现象,发展一种适用于等熵流动的交错拉氏Godunov方法.主要的特征是采用速度与热力学变量交错分布的形式,避免在单元内进行速度平均,从而消除由于动量平均过程导致的动能耗散.与传统的von Neumann型交错网格方法相比,网格的边界通量由节点处的多维黎曼求解器提供,克服了多维人工粘性选取带来的困难.为减少多维黎曼求解器在求解稀疏波问题时的非物理熵增,给出稀疏波出现的合理判据,从而保证了热力学关系式的满足.数值实验表明:该方法能很好地消除稀疏波的过热现象,同时在求解激波问题时又能保持与传统单元中心型拉氏方法相同的激波捕捉能力. 相似文献
956.
Scaling theory predicts complete localization in d = 2 in quantum systems belonging to the orthogonal class(i.e., with timereversal symmetry and spin-rotation symmetry). The conductance g behaves as g^exp(-L/l) with system size L and localization length l in the strong disorder limit. However, classical systems can always have metallic states in which Ohm’s law shows a constant g in d=2. We study a two-dimensional quantum percolation model by controlling dephasing effects. The numerical investigation of g aims at simulating a quantum-to-classical percolation evolution. An unexpected metallic phase, where g increases with L, generates immense interest before the system becomes completely classical. Furthermore, the analysis of the scaling plot of g indicates a metal-insulator crossover. 相似文献
957.
Biqun Chen Karthikeyan Rajagopal Fatemeh Parastesh Hamed Azarnoush Sajad Jafari Iqtadar Hussain 《理论物理通讯》2020,72(10):105003-28
The economic and financial systems consist of many nonlinear factors that make them behave as the complex systems. Recently many chaotic finance systems have been proposed to study the complex dynamics of finance as a noticeable problem in economics. In fact, the intricate structure between financial institutions can be obtained by using a network of financial systems. Therefore, in this paper, we consider a ring network of coupled symmetric chaotic finance systems, and investigate its behavior by varying the coupling parameters. The results show that the coupling strength and range have significant effects on the behavior of the coupled systems, and various patterns such as the chimera and multi-chimera states are observed. Furthermore, changing the parameters' values, remarkably influences on the oscillators attractors. When several synchronous clusters are formed, the attractors of the synchronized oscillators are symmetric, but different from the single oscillator attractor. 相似文献
958.
We investigate the quantum numbers of the pentaquark states ${{\rm{P}}}_{{\rm{c}}}^{+}$, which are composed of 4 (three flavors) quarks and an antiquark, by analyzing their inherent nodal structure in this paper. Assuming that the four quarks form a tetrahedron or a square, and the antiquark is at the ground state, we determine the nodeless structure of the states with orbital angular moment L≤3, and in turn, the accessible low-lying states. Since the inherent nodal structure depends only on the inherent geometric symmetry, we propose the quantum numbers JP of the low-lying pentaquark states ${{\rm{P}}}_{c}^{+}$ may be ${\tfrac{3}{2}}^{-}$, ${\tfrac{5}{2}}^{-}$, ${\tfrac{3}{2}}^{+}$and ${\tfrac{5}{2}}^{+}$, independent of dynamical models. 相似文献
959.
Hyper-parallel quantum information processing is a promising and beneficial research field. Herein, a method to implement a hyper-parallel controlled-phase-flip (hyper-CPF) gate for frequency-, spatial-, and time-bin-encoded qubits by coupling flying photons to trapped nitrogen vacancy (NV) defect centers is presented. The scheme, which differs from their conventional parallel counterparts, is specifically advantageous in decreasing against the dissipate noise, increasing the quantum channel capacity, and reducing the quantum resource overhead. The gate qubits with frequency, spatial, and time-bin degrees of freedom (DOF) are immune to quantum decoherence in optical fibers, whereas the polarization photons are easily disturbed by the ambient noise. 相似文献
960.
大气压空气电火花激波等离子体射流的电子密度在亚微秒时间尺度上瞬变,其电子密度的测定很难.基于微波瑞利散射原理,本文测量了空气电火花冲击波流注放电等离子体射流的时变电子密度.实验结果表明:测量系统的标定参数A为1.04 × 105 V·Ω·m–2;空气流注放电等离子体射流的电子密度与等离子体射流的半径和长度有关,结合高速放电影像展示的等离子体射流的等效半径和等效长度,测定的电子密度在1020 m–3的量级,且随时间先快速增长至峰值再成指数衰减.此外,本文还探讨了等离子体射流的不同等效尺度对测定结果的影响;分析结果表明,采用时变等效半径和时变等效长度的计算结果最有效,且第1个快速波峰是由光电离的电离波导致的. 相似文献