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91.
We present a simplified relativistic configuration interaction method (SRCI), by which all the energy levels and oscillator strengths in each transition array can be calculated. There exist generalized quasi-sum relations for the calculated oscillator strengths in the relevant transition arrays by the SRCI and by an unresolved transition array model (UTA). Based on UTA and the detailed configuration accounting (DCA), with a fully relativistic treatment incorporated with the quantum defect theory, the X-ray absorption spectra for any middle- and high-Z plasmas or composite plasmas can be calculated with much less computational efforts. The gross features of calculated spectra by DCA-UTA are in agreement with the relevant experimental measurements, except some detailed structures in some narrow spectral ranges. Such detailed structures can be calculated by SRCI incorporated with DCA-UTA. As an illustrative example, the absorption spectra of Ge plasmas are calculated by DCA-UTA-SRCI and are in agreement with the experimental opacity data. Therefore, the theoretical method (DCA-UTA-SRCI) verified by experimental measurements will not only be a basic tool to provide “precision” opacity data for the inertial confinement fusion research (ICF) and studies in stellar physics but also can be used to analyze the relevant diagnostic measurements for ICF plasmas. 相似文献
92.
Ching Sum Hui Lillian Sze Man Lam Chun Yin Wai Kin Chan Aleksandra B. Djurii 《Journal of polymer science. Part A, Polymer chemistry》2003,41(11):1708-1715
Polyurethanes incorporated with rhenium diimine complexes were synthesized. The polymers exhibited interesting morphologies and solution properties. Results from gel permeation chromatography suggested the formation of polymer aggregates in solutions. The polymers could act as probes for metal ions. The addition of metal ions to polymer solutions led to significant changes in the electronic absorption properties of the polymer solutions. This was attributed to the interactions between the polyether moieties and metal ions. The metal complexes could also act as efficient photosensitizers. After doping with charge‐transport viologens, the photoconductivity of the polymers was greatly enhanced. The experimental quantum efficiency was simulated with Onsager's theory. The thermalization distances and the primary yields were typically 12–14 Å and 10?3, respectively. © 2003 Wiley Periodicals, Inc. J Polym Sci Part A: Polym Chem 41: 1708–1715, 2003 相似文献
93.
S. Koh K. Konishi Y. Shiraki 《Physica E: Low-dimensional Systems and Nanostructures》2004,21(2-4):440
Self-assembled GeSiC dots stacked on a Ge hut-cluster layer buried in Si have been investigated. The critical thickness for formation of GeSiC dots is reduced owing to the strain fields from the buried hut-clusters. By utilizing the stacked structure, the dot size is decreased and the uniformity is improved. The highest density of the GeSiC dots with stacked structures is 7.4×1010 cm−2, which is six times larger than that of single GeSiC dots. The formation of the self-assembled GeSiC dots is strongly influenced by being stacked with buried Ge dots as well as C incorporation. 相似文献
94.
Timothy M. Chan 《Discrete and Computational Geometry》2005,34(1):11-24
We give a surprisingly short proof that in any planar arrangement of n curves where each pair intersects at most a fixed number (s) of
times, the k-level has subquadratic (O(n2-1/2s) complexity. This answers one of the main open problems from the author’s previous paper [DCG 29, 375-393 (2003)],
which provided a weaker upper bound for a
restricted class of curves only (graphs of degree-s polynomials).
When combined with existing tools (cutting curves, sampling, etc.),
the new idea generates a slew of improved k-level results for
most of the curve families studied earlier, including a
near-O(n3/2 bound for parabolas. 相似文献
95.
96.
Ergodic isospectral theory of the Lax pairs of Euler equations with harmonic analysis flavor 总被引:2,自引:0,他引:2
Y. Charles Li 《Proceedings of the American Mathematical Society》2005,133(9):2681-2687
Isospectral theory of the Lax pairs of both 3D and 2D Euler equations of inviscid fluids is developed. Eigenfunctions are represented through an ergodic integral. The Koopman group and mean ergodic theorem are utilized. Further harmonic analysis results on the ergodic integral are introduced. The ergodic integral is a limit of the oscillatory integral of the first kind.
97.
In this work, we elucidate the effect of the less mobile ions on the dynamics of the more mobile ions by molecular dynamics simulations of lithium ions motion in lithium metasilicate glass by freezing some randomly chosen lithium ions (5%, 10% and 25%) at their initial locations at 700 K. A remarkable slowing down of the dynamics of the majority mobile Li ions was observed both in the self-part of the density–density correlation function, Fs(k,t), and in the diffusion coefficients. On the other hand, there is no significant change in the structure. These results show many similarities to the mixed alkali effect (MAE) with mixing of the small content of foreign alkali (10% and 25% of K2O), where large reduction of the dynamics was also observed in both experiments and MD simulations. This immobilization of faster ions causes the large MAE as already discussed in relation to the mechanism of the cooperative ion jump motions. Although of lesser importance, the ion dynamics are influenced by the matrix of oxygen atoms, because the jump motions of Li ions are assisted by the localized motions of oxygen atoms. 相似文献
98.
Using radical chemistry novel highly condensed heterocycles have been synthesized. The mechanism for their formation is discussed. 相似文献
99.
This paper presents an evaluation of the capability of turbulence models available in the commercial CFD code FLUENT 6.0 for their application to hydrofoil turbulent boundary layer separation flow at high Reynolds numbers. Four widely applied two‐equation RANS turbulence models were assessed through comparison with experimental data at Reynolds numbers of 8.284×106 and 1.657×107. They were the standard k–εmodel, the realizable k–εmodel, the standard k–ωmodel and the shear‐stress‐transport (SST) k–ωmodel. It has found that the realizable k–εturbulence model used with enhanced wall functions and near‐wall modelling techniques, consistently provides superior performance in predicting the flow characteristics around the hydrofoil. Copyright © 2004 John Wiley & Sons, Ltd. 相似文献
100.
A least‐squares meshfree method based on the first‐order velocity–pressure–vorticity formulation for two‐dimensional incompressible Navier–Stokes problem is presented. The convective term is linearized by successive substitution or Newton's method. The discretization of all governing equations is implemented by the least‐squares method. Equal‐order moving least‐squares approximation is employed with Gauss quadrature in the background cells. The boundary conditions are enforced by the penalty method. The matrix‐free element‐by‐element Jacobi preconditioned conjugate method is applied to solve the discretized linear systems. Cavity flow for steady Navier–Stokes problem and the flow over a square obstacle for time‐dependent Navier–Stokes problem are investigated for the presented least‐squares meshfree method. The effects of inaccurate integration on the accuracy of the solution are investigated. Copyright © 2004 John Wiley & Sons, Ltd. 相似文献