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111.
Zhakhovsky VV Budzevich MM Inogamov NA Oleynik II White CT 《Physical review letters》2011,107(13):135502
By decoupling time and length scales in moving window molecular dynamics shock-wave simulations, a new regime of shock-wave propagation is uncovered characterized by a two-zone elastic-plastic shock-wave structure consisting of a leading elastic front followed by a plastic front, both moving with the same average speed and having a fixed net thickness that can extend to microns. The material in the elastic zone is in a metastable state that supports a pressure that can substantially exceed the critical pressure characteristic of the onset of the well-known split-elastic-plastic, two-wave propagation. The two-zone elastic-plastic wave is a general phenomenon observed in simulations of a broad class of crystalline materials and is within the reach of current experimental techniques. 相似文献
112.
I. Usman Z. Buthelezi J. Carter G.R.J. Cooper R.W. Fearick S.V. Förtsch H. Fujita Y. Fujita Y. Kalmykov P. von Neumann-Cosel R. Neveling P. Papakonstantinou A. Richter R. Roth A. Shevchenko E. Sideras-Haddad F.D. Smit 《Physics letters. [Part B]》2011
The fragmentation of the Isoscalar Giant Quadrupole Resonance (ISGQR) in 40Ca has been investigated in high energy-resolution experiments using proton inelastic scattering at Ep=200 MeV. Fine structure is observed in the region of the ISGQR and its characteristic energy scales are extracted from the experimental data by means of a wavelet analysis. The experimental scales are well described by Random Phase Approximation (RPA) and second-RPA calculations with an effective interaction derived from a realistic nucleon–nucleon interaction by the Unitary Correlation Operator Method (UCOM). In these results characteristic scales are already present at the mean-field level pointing to their origination in Landau damping, in contrast to the findings in heavier nuclei and also to SRPA calculations for 40Ca based on phenomenological effective interactions, where fine structure is explained by the coupling to two-particle–two-hole (2p–2h) states. 相似文献
113.
The control of regiochemistry in the synthesis of polysaccharide derivatives is one of the most significant scientific challenges
in the field. Its importance is only further highlighted by the individual successes in synthesis of regioselectively substituted
derivatives, in particular cellulose esters and ethers, over the last 20 years. The availability of these samples and studies
of their properties versus randomly substituted analogs has shown clearly that properties like solubility, aggregation phenomena,
and optical properties depend heavily on the regiochemistry of substitution. We report here on the one-pot synthesis of novel
6-bromo-6-deoxy-2,3-O-acylcellulose derivatives, which as more organic soluble derivatives of 6-bromo-6-deoxycellulose should allow broader exploitation
of the highly regioselective cellulose 6-bromination chemistry. We illustrate the potential of these new derivatives by conversion
to 6-cyano-6-deoxycellulose esters. 相似文献
114.
The objective of this research is to determine whether Systems Dynamics (SD) is a beneficial method for modelling hospital patient flow from a strategic planning perspective. While discrete event simulation has frequently been used as a tool for analysing and improving patient flow in health care settings, the desire to assess and understand patient flow and resource demand from a more strategic, and therefore aggregate, perspective led to the use of SD. To evaluate the suitability of such an approach, a model was developed in collaboration with the General Campus at The Ottawa Hospital with particular attention paid to the delays experienced by patients in the emergency department. The modelling techniques used, model validation and scenarios tested with the model are discussed, accompanied by comments regarding the appropriateness of SD for such a model. 相似文献
115.
116.
Substitution effects on the stereochemical outcome of bisspiroketalization on the C1-C17 carbon backbone of azaspiracid is presented. A possible explanation is offered to explain the observed stereochemical outcome. 相似文献
117.
118.
Liondas CA; Chrissoulidis DP 《The Quarterly Journal of Mechanics and Applied Mathematics》2007,60(3):275-287
This paper is intended to clarify a misunderstanding concerningthe source singularity of the electric Green's tensor for aperfectly conducting semi-infinite cone of circular cross-section.Tai's series expansion of the Green's tensor is known to lacka singular term at the source region. Jones has reconstructedthe solution to this problem and has pointed out the differencebetween his result and that of Tai. The aim of our paper isto demonstrate that, although Jones's closed-form solution iscorrect, there is a mistake in his comparison with Tai's seriessolution. We conclude that one of the two additional singularterms that Jones claims as missing from Tai's formula must beomitted. Besides, we compare Jones's closed-form solution withSmyshlyaev's solution to the very same problem. We concludethat the magnetic field expressions given by Jones and Smyshlyaevcoincide, but a singular term is missing from Smyshlyaev's expressionfor the electric field. 相似文献
119.
120.
Goodman TNT; Micchelli CA; Rodriguez G; Seatzu S 《IMA Journal of Numerical Analysis》1998,18(3):331-354
It is shown that, under certain conditions, orthonormalizingthe positive integer shifts of an exponentially decaying functionon the half line by the Gram-Schmidt process leads to a limitingprofile given by orthonormalizing all their integer shifts onthe whole line. These results derive from properties of Choleskyfactorization of bi-infinite and semi-infinite matrices. Anexample is provided by the negative exponential function andconjectures are given, supported by numerical evidence, forthe Gaussian and Lorentz function. 相似文献