Nuclear liquid-gas phase transition within the lattice gas model

We study the nuclear liquid-gas phase transition on the basis of a two-component lattice gas model. A Metropolis type of sampling method is used to generate microscopic states in the canonical ensemble. The effective equation of state and fragment mass distributions are evaluated in a wide range of temperatures and densities. A definition of the phase coexistence region appropriate for small systems is proposed. The caloric curve resulting from different types of freeze-out conditions are presented.     

First measurements with the neutron decay spectrometer a SPECT

The neutron decay spectrometera SPECT has been built to perform a precise measurement of the proton spectrum shape in the decay of free neutrons. Such a measurement allows a determination of the neutrino electron angular-correlation coefficienta . The present best experiments have an uncertainty of Δa/a = 5% and since the seventies there is no substantial improvement. Witha SPECT, we aim for an uncertainty which is lower by more than an order of magnitude, thus enabling us to perform several precise tests of the Standard Model. In our first beam time at the particle physics beam MEPHISTO at the Forschungsneutronenquelle Heinz Maier-Leibnitz, we studied the properties of the spectrometer. The most serious problem turned out to be the situation- and time-dependent behavior of the background. From the data sets from this beam time in which a background problem was not obvious, we could extract a value ofa = - 0.1151±0.0040^stat , but we could not quantify the background uncertainty. We show ways to deal with the background and other problems for future beam times.     

Corrective measures in turbulent pipe flows and extended self-similarity

Significant statistical bias in LDA measurements and how to adequately deal with it is a subtle problem when dealing with turbulent flows. In order to attempt a clarification we have performed measurements on a non-standard “grid experiment” where a clear bias effect is found. We have investigated the effect of several corrective measures and find that best results, in the sense of having the first moment converge to zero, are obtained when using the time between events as statistical weights. The corrected time series have been used to check for extended self-similarity (ESS). Even though no scaling regime is seen for the third moment and the flow certainly is neither isotropic nor homogeneous, perfect ESS scaling based on the absolute third moment is observed up to the twelfth moment, extending into a time domain regime where the Taylor hypothesis of frozen turbulence is obviously violated. Reversing the argument this indicates that the correction scheme needed can be experimentally decided on using the criterion stated above and especially so if ESS is to be expected. Finally we have used the corrected data to quantify the deviations from Gaussian behavior of the velocity difference probability density function for a weakly turbulent flow. Through comparison with results on the Gaussian-Lorentzian distribution we find that the even part of the experimental distribution can be reproduced quite well by a single-parameter family of distributions with second moment equal unity. Received 5 August 1998 and Received in final form 21 December 1998     

Linear viscoelastic models: Part I. Relaxation modulus and melt calibration

Constitutive models for the linear viscoelasticity of polymers are presented for the relation between the relaxation modulus and the molecular weight distribution (MWD). We also compute the MWD from a simulated relaxation modulus curve by first obtaining the rheologically effective distribution (RED) as a function of time, and converting this into the MWD by melt calibration; that is, the relation between timescale and the molecular weight. This procedure has similarities with the widely used universal calibration with solved polymers. The main principles of our technique are applied here to familiar relaxation modulus data, for which we present two models: (1) an analytical model derived from control theory, which is known capable of modelling partially observed system and (2) a practical characteristic model for obtaining usable results. No relaxation time or spectrum procedures are used to model the process of linear viscoelastic relaxation. The use of relative calculations and melt calibration dispenses with the need to know the real chain structures such as branching and entangled chain dynamics, and the model remains useful for future investigations of polymer chain structures and dynamics, such as using tube theory.     

One-dimensional PtO2 at Pt steps: formation and reaction with CO

Using core-level spectroscopy and density functional theory we show that a one-dimensional (1D) oxide structure forms at the steps of the Pt(332) surface after exposure. The 1D oxide is found to be stable in an oxygen pressure range, where bulk oxides are only metastable, and is therefore argued to be a precursor to the Pt oxidation. As an example of the consequences of such a precursor exclusively present at the steps, we investigate the reaction of CO with oxygen covered Pt(332). Albeit more strongly bound, the oxidic oxygen is found to react more easily with CO than oxygen chemisorbed on the Pt terraces.     

Excitation of ground and gamma bands in the 24Mg(α, α')24Mg reaction at 120 MeV

The cross sections for excitation of the members of the ground state (g.s.) band 0^?(g.s.), 2⁺ (1.37 MeV) and 4⁺ (4.12 MeV) and the γ-band 2⁺_γ (4.24 MeV), 3_γ⁺(5.24 MeV) and 4_γ⁺(6.01 MeV) in ²⁴Mg have been measured in inelastic α-scattering at E_α = 120 MeV. The excitation of these states are found to be well described by a coupled-channel calculation (CCBA) performed in the framework of the asymmetric rotational model. Two sets of parameters are found to give excellent fits to the data, but in both a direct coupling between the ground state and the 4⁺ state is found necessary.     

Beta decay studies in the vicinity of 13250Sn82: Excited states in 13051Sb, 13052Te and 13252Te

Using the OSIRIS on-line isotope separator facility, the decays of ¹³⁰Sn and ^{130, 132}Sb have been studied. On the basis of singles γ and γ-γ coincidence Ge(Li) spectra and conversion electron Si(Li) measurements, level schemes for ¹³⁰Sb, ¹³⁰Te and ¹³²Te have been constructed. The corresponding half-lives have been measured using multiscaling technique. The 3.8 min ground state of ¹³⁰Sn populates only positive parity states in the πν^?3 nucleus ¹³⁰Sb: the energetically lowest 5⁺ state with the $\text{(π1}\text{g}{}_{\mathrm{<mtext>7</mtext><mtext>2</mtext>}}\text{, ν2}\text{d}{}_{\mathrm{<mtext>3</mtext><mtext>2</mtext>}}\text{)}$ configuration assignment; the $\text{T}{}_{\mathrm{<mtext>1</mtext><mtext>2</mtext>}}\text{= 3.6 ± 0.3}\text{ns}\text{4}{}^{\mathrm{+}}$ state at 70.0 keV; the 2⁺ state at 262.5 keV; the (0, 1)⁺ state at 697.2 keV; the 3⁺ state at 813.1 keV and the 1⁺ state at 1042.3 keV excitation energy. A 1.7 min isomeric state in ¹³⁰Sn, with the tentative spin assignment (7^?), populates several odd parity levels in ¹³⁰Sb. These arise from the $\text{(π1}\text{g}{}_{\mathrm{<mtext>7</mtext><mtext>2</mtext>}}\text{, ν1}\text{h}{}_{\mathrm{<mtext>11</mtext><mtext>2</mtext>}}{}^{-1}\text{)}$ and/or $\text{(π2}\text{d}{}_{\mathrm{<mtext>5</mtext><mtext>2</mtext>}}\text{, ν1}\text{h}{}_{\mathrm{<mtext>11</mtext><mtext>2</mtext>}}{}^{-1}\text{)}$ configurations and are located 84.7 keV (6^?), 144.9 keV (7^?), 688.5 keV and 1044.0 keV above the 40 min 8^? β- decaying state. No transitions between odd and even parity states have been observed.The most important excited states in ¹³⁰Te found in the β^? decay of the 6.6 min ¹³⁰Sb 5⁺ state are: 839.4 keV, 2⁺; 1632.8 keV, 4⁺; 1815.1 keV, 6⁺; 2100.8 keV, 5^?.Levels in the π²ν^?2 nucleus ¹³²Te were observed in the β^? decays of the 2.8 min ¹³²Sb (4⁺) and the 4.2 min ¹³²Sb (8^?) states. Unique spin and parity assignments have been given to the following states: 973.9 keV, 2⁺; 1670.7 keV, 4⁺; 1774.1 keV, 6⁺; 1924.7 keV, 7^?; 2053.0 keV, 5^?.     

Evidence for double dissociation in K-p interactions at 14.3 GeV/c

We have studied the reaction K^-p → K^-π⁺π^-π⁺π^-p at 14.3 GeV/c to search for evidence of the double dissociation process $\text{K}{}^{\mathrm{-}}\text{p}\text{→}\text{QN}{}_{\mathrm{<mtext>1</mtext><mtext>2</mtext>}}{}^1$. In the channel $\text{K}{}^{\mathrm{-}}\text{p}\text{→}\text{K}{}^{10}\text{(890)}$π₁^-π₂^-Δ⁺⁺ (1236) there is evidence for simultaneous production of low-mass enhancements in the $\text{K}{}^{10}\text{π}{}_1{}^{\mathrm{-}}$ and Δ⁺⁺(1236)π₂^- subsystems which correspond to the $\text{Q}\text{→}\text{K}{}^1\text{(890)π}$ and $\text{N}{}_{\mathrm{<mtext>1</mtext><mtext>2</mtext>}}{}^1\text{→ Δπ}$ decay modes. In this particular final state the double fragmentation system is produced with a cross section of the order of a few microbarns. Our data are consistent with the factorizable pomeron exchange model of double diffractive dissociation.     

Two-dimensional oxide on Pd(111)

The oxidation of Pd(111) leads to an incommensurate surface oxide, which was studied by the use of scanning tunneling microscopy, surface x-ray diffraction, high resolution core level spectroscopy, and density functional calculations. A combination of these methods reveals a two-dimensional structure having no resemblance to bulk oxides of Pd. Our study also demonstrates how the atomic arrangement of a nontrivial incommensurate surface can be solved by molecular dynamics in a case where experimental techniques alone give no solution.