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131.
P. PALMIERI C. PUZZARINI V. AQUILANTI G. CAPECCHI S. CAVALLI D. DE FAZIO 《Molecular physics》2013,111(21):1835-1849
The reaction He + H+ 2(v,j = 0) → HeH+(v′ = 0, j′) for v = 0, 1,2 and 3 and for scattering energies near the threshold (0.95–1.15 eV) has been studied by calculating ab initio points at MRCI level and ‘exact’ integral quantum reactive cross-sections. More than 1400 nuclear geometries have been chosen to cover the most important regions for the dynamics, an extended set of points being taken directly on a hyperspherical coordinate grid. A many-body expansion with a large number of terms permits an accurate analytical representation of the potential energy surface with a root-mean-square deviation <12meV. The hyperquantization algorithm has been extended to obtain quantum mechanical integral cross-sections which are compared with previous calculations and with experimental results. 相似文献
132.
J. MEDINA YU. G. GUREVICH G. N. LOGVINOV P. RODRÍGUEZ G. GONZÁLEZ DE LA CRUZ 《Molecular physics》2013,111(19):3133-3138
The problem of the effective thermal diffusivity of two-layer systems is investigated using the photoacoustic spectroscopy. The experimental results are examined in terms of the effective thermal parameters of the composite system determined from a homogeneous material that produces the same physical response under an external perturbation in the detector device. It is shown that the effective thermal conductivity is not symmetric under exchange of the two layers of the composite, i.e. the effective thermal parameters depend upon which layer is illuminated in the photoacoustic experiments. Particular emphasis is given to the characterization of the interface thermal conductivity between the layer system. 相似文献
133.
This paper investigates the random buffeting excitation forces that apply to tubes in two-phase cross-flows. The spectral magnitude of these forces is studied with the help of a database that includes most of the available experimental data on direct or indirect force measurements. Different fluid mixtures, namely steam–water, air–water and various types of Freon, as well as different thermohydraulic or geometrical situations are included in the database. Using a formalism similar in principle to that used successfully in the modelling of buffeting in single-phase flows, the scaling of the data is undertaken. While dynamic pressure, viscosity or surface tension are found not to be relevant parameters, gravity forces allow us to define appropriate dimensionless spectra for all cases. The meaning of these parameters as well as the effects of flow regimes or fluid mixtures are discussed. Finally, an upper bound on the magnitude of these forces, which is of practical applicability, is proposed. 相似文献
134.
M DE SANCTIS 《Pramana》2013,81(3):467-483
Hypothetical superheavy fourth-generation fermions with a very small coupling with the rest of the Standard Model can give rise to long enough lived bound states. The production and the detection of these bound states would be experimentally feasible at the LHC. Extending, in the present study, the analysis of other authors, a semirelativistic wave equation is solved using an accurate numerical method to determine the binding energies of these possible superheavy fermion-bound states. The interaction given by the Yukawa potential of the Higgs boson exchange is considered; the corresponding relativistic corrections are calculated by means of a model based on the covariance properties of the Hamiltonian. We study the effects given by the Coulomb force. Moreover, we calculate the contributions given by the Coulombic and confining terms of the strong interaction in the case of superheavy quark bound states. The results of the model are critically analysed. 相似文献
135.
New low molar mass liquid crystalline vitrifying materials have been synthesized and tested for application in optical films. The molecules were based on spiro compounds derived from pentaerythritol and mesogenic groups derived from cyanobiphenylyl moieties. The resulting materials showed glass transition temperatures as high as 85 degrees C and nematic to isotropic phase transition temperatures up to 222 degrees C. Crystallization from the melt was strongly suppressed. Well-aligned, solid, birefringent layers were obtained from the materials by spincoating. Uniaxially oriented layers with an optic axis tilted with respect to the substrate were obtained by spincoating the liquid crystals on pretilt amplification layers. When an anisotropic dye was incorporated in the liquid crystals, polarizers with a tilted absorption axis were obtained. In addition, the compounds were found to be suitable as hosts for photo-induced reorientation of photo-isomerizable dyes. 相似文献
136.
DE Blumling T Tokumoto S McGill KL Knappenberger 《Physical chemistry chemical physics : PCCP》2012,14(31):11053-11059
The influence of temperature and applied magnetic fields on photoluminescence (PL) emission and electronic energy transfer (ET) of both isolated and aggregated CdSe nanocrystals was investigated. Following 400-nm excitation, temperature-dependent, intensity-integrated and energy-resolved PL measurements were used to quantify the emission wavelength and amplitude of isolated CdSe nanocrystals. The results indicated an approximately three-fold increase in PL intensity upon decreasing the temperature from 300 K to 6 K; this was attributed to a reduction of charge carrier access to nanocrystal surface trap states and suppression of thermal loss channels. Temperature-dependent PL measurements of aggregated CdSe nanocrystals, which included both energy-donating and -accepting particles, were analyzed using a modified version of F?rster theory. Temperature-dependent ET efficiency increased from 0.55 to 0.75 upon decreasing the sample temperature from 225 K to 6 K, and the ET data contained the same trend observed for the PL of isolated nanoclusters. The application of magnetic fields to increase nanocrystal ET efficiency was studied using magneto-photoluminescence measurements recorded at a sample temperature of 1.6 K. We demonstrated that the exciton fine structure population of the donor was varied using applied magnetic fields, which in turn dictated the PL yield and the resultant ET efficiency of the CdSe nanocrystal aggregate system. The experimental data indicated an ET efficiency enhancement of approximately 7%, which was limited by the random orientation of the spherical nanocrystals in the thin film. 相似文献
137.
In this article, we analyze the decisional power index, the so called Hoede-Bakker index. This index takes the preferences of the players into account, as well as the social structure in which players may influence each other. We investigate the properties of the Hoede-Bakker index. We adapt some postulates for power indices and voting power paradoxes for the Hoede-Bakker set up. We investigate whether this decisional power index displays the adapted voting power paradoxes and whether it satisfies the adapted postulates for power indices. 相似文献
138.
The authors consider a quarter-symmetric metric connection in a P-Sasakian manifold and study the second order parallel tensor in a P-Sasakian manifold with respect to the quarter-symmetric metric connection. Then Ricci semisymmetric P-Sasakian manifold with respect to the quarter-symmetric metric connection is considered. Next the authors study ξ-concircularly flat P-Sasakian manifolds and concircularly semisymmetric P-Sasakian manifolds with respect to the quarter-symmetric metric connection. Furthermore, the authors study P-Sasakian manifolds satisfying the condition ■(ξ,Y)·■,where ■,■ are the concircular curvature tensor and Ricci tensor respectively with respect to the quarter-symmetric metric connection. Finally, an example of a 5-dimensional P-Sasakian manifold admitting quarter-symmetric metric connection is constructed. 相似文献
139.
140.
Suranjan DE 《Annals of Operations Research》1988,12(1):109-134
This paper reports the development of a computer-based system for production scheduling in a dedicated FMS. The system is based on the state-operator framework commonly used in artificial intelligence. Such a system consists of three components: (i) a knowledge base of states, which describes both the current task domain situation and the goal to be achieved; (ii) a set of operators that are used to manipulate the knowledge base; and (iii) a control strategy to decide which operators to apply next and to resolve conflicts. Some of the interesting features of the scheduling system include: (i) the ability to detect resource conflicts; (ii) the ability to determine alternate routes for a given part in the event of a resource conflict; and (iii) the ability to amend plans if an alternate route is found. These features allow the system to take advantage of the flexible routing for parts that an FMS allows. The system has been implemented using the XLISP programming language. Implementation considerations are discussed. A small but comprehensive example is presented. Further research directions are suggested. 相似文献