Interference in the collective electron momentum in double photoionization of H2

We investigate single-photon double ionization of H(2) by 130 to 240 eV circularly polarized photons. We find a double slitlike interference pattern in the sum momentum of both electrons in the molecular frame which survives integration over all other degrees of freedom. The difference momentum and the individual electron momentum distributions do not show such a robust interference pattern. We show that this interference results from a non-Heitler-London fraction of the H(2) ground state where both electrons are at the same atomic center.     

Measurement of vacuum-assisted photoionization at 1 GeV for Au and Ag targets

We report a measurement of photon impact ionization of K and L shell of Au and K shell of Ag targets in the 1-GeV energy range. We show that the cross section is dominated by a contribution from a new channel called vacuum-assisted photoionization. In this process the energy-momentum balance associated with the removal of the innershell electron is obtained by conversion of a high-energy photon into an electron-positron pair. This measurement is consistent with the theoretical prediction that vacuum-assisted photoionization is the most probable ionization mechanism at very high energies.     

Exponential growth of positive initial-energy solutions of a system of nonlinear viscoelastic wave equations with damping and source terms

This work is concerned with a system of nonlinear viscoelastic wave equations with nonlinear damping and source terms acting in both equations. We will prove that the energy associated to the system is unbounded. In fact, it will be proved that the energy will grow up as an exponential function as time goes to infinity, provided that the initial data are large enough. The key ingredient in the proof is a method used in Vitillaro (Arch Ration Mech Anal 149:155–182, 1999) and developed in Said-Houari (Diff Integr Equ 23(1–2):79–92, 2010) for a system of wave equations, with necessary modification imposed by the nature of our problem.     

Ultrafast internal conversion in ethylene. I. The excited state lifetime

Using a combined theoretical and experimental approach, we investigate the non-adiabatic dynamics of the prototypical ethylene (C(2)H(4)) molecule upon π → π? excitation. In this first part of a two part series, we focus on the lifetime of the excited electronic state. The femtosecond time-resolved photoelectron spectrum (TRPES) of ethylene is simulated based on our recent molecular dynamics simulation using the ab initio multiple spawning method with multi-state second order perturbation theory [H. Tao, B. G. Levine, and T. J. Martinez, J. Phys. Chem. A 113, 13656 (2009)]. We find excellent agreement between the TRPES calculation and the photoion signal observed in a pump-probe experiment using femtosecond vacuum ultraviolet (hν = 7.7 eV) pulses for both pump and probe. These results explain the apparent discrepancy over the excited state lifetime between theory and experiment that has existed for ten years, with experiments [e.g., P. Farmanara, V. Stert, and W. Radloff, Chem. Phys. Lett. 288, 518 (1998) and K. Kosma, S. A. Trushin, W. Fuss, and W. E. Schmid, J. Phys. Chem. A 112, 7514 (2008)] reporting much shorter lifetimes than predicted by theory. Investigation of the TRPES indicates that the fast decay of the photoion yield originates from both energetic and electronic factors, with the energetic factor playing a larger role in shaping the signal.     

Decay property of regularity-loss type for solutions in elastic solids with voids

In this paper, we consider the Cauchy problem for a system of elastic solids with voids. First, we show that a linear porous dissipation leads to decay rates of regularity-loss type of the solution. We show some decay estimates for initial data in H^s(R)∩L¹(R)$H^s\left(\mathbb{R}\right)\cap L^1\left(\mathbb{R}\right)$. Furthermore, we prove that by restricting the initial data to be in H^s(R)∩L^1,γ(R)$H^s\left(\mathbb{R}\right)\cap L^{1,\gamma }\left(\mathbb{R}\right)$ and γ∈[0,1]$\gamma \in [0,1]$, we can derive faster decay estimates of the solution. Second, we show that by adding a viscoelastic damping term, then we gain the regularity of the solution and obtain the optimal decay rate.     

Existence and Asymptotic Behavior of the Wave Equation with Dynamic Boundary Conditions

The goal of this work is to study a model of the strongly damped wave equation with dynamic boundary conditions and nonlinear boundary/interior sources and nonlinear boundary/interior damping. First, applying the nonlinear semigroup theory, we show the existence and uniqueness of local in time solutions. In addition, we show that in the strongly damped case solutions gain additional regularity for positive times t>0. Second, we show that under some restrictions on the initial data and if the interior source dominates the interior damping term and if the boundary source dominates the boundary damping, then the solution grows as an exponential function. Moreover, in the absence of the strong damping term, we prove that the solution ceases to exists and blows up in finite time.     

A new criterion of optimization of the simple multipole coefficients in a modified Green’s function for the elastic two-dimensional case

The question of non-uniqueness in the integral formulation of an exterior boundary value problem in the elastic two-dimensional case has been resolved using the modified Green’s function technique. In this work, a new criterion of optimality based on the minimization of the norm of the kernel of the modified integral operator is established.