磁性纳米结构中由激光引起的超快自旋动力学研究

以单个磁性中心的NiO以及由Co和Ni等元素构成的双磁性中心的纳米结构为例,总结了近年所做的主要工作.为了在理论上实现磁性纳米结构中的超快自旋翻转和转移,提出了一种称为Λ进程(Λ process)的超快自旋转换机理.在实际计算中,首先采用量子化学第一性原理计算得到磁性纳米结构中精确的隙间d电子态,然后考虑外加磁场和自旋轨道耦合分析磁性原子中的自旋局域化程度,最后引入激光脉冲项,研究在其作用下材料的自旋态经由Λ进程实现转换的时间历程.研究结果表明自旋翻转和转移可以在线偏振光的作用下在亚皮秒的时间尺度内完成. 关键词： 超快自旋动力学 第一性原理计算 Λ进程 磁性纳米结构     

Optical interconnection between different spatial modes using double phase conjugate mirror with polarization alignment system

We propose a fundamental interconnection method using a polarization alignment system for waveguides having different spatial modes. In addition, as an example for the verification of the fundamental operation, we demonstrate an interconnection between a photonic crystal fiber and a laser that have obviously different spatial modes. The polarization alignment system operates synergistically with a self-written waveguide formed with a double phaseconjugate mirror. This technique enables us to interconnect a photonic crystal fiber with a laser source without complicated and time-consuming optical alignment. In this method, although it is not necessary to perform an external control for interconnection, the waveguide most suitable for connection is formed autonomously in a Sn₂P₂S₆:Sb crystal developed for this purpose. There was a marked reduction in the polarization dependence of coupling efficiency, compared with that observed using a stand-alone double phase-conjugate mirror.     

Finite-size scaling and power law relations for dipole-quadrupole interaction on Blume-Emery-Griffiths model

The Blume-Emery-Griffiths model with the dipole-quadrupole interaction ($ \ell = \frac{I} {J} $ \ell = \frac{I} {J} ) has been simulated using a cellular automaton algorithm improved from the Creutz cellular automaton (CCA) on the face centered cubic (fcc) lattice. The finite-size scaling relations and the power laws of the order parameter (M) and the susceptibility (χ) are proposed for the dipole-quadrupole interaction (ℓ). The dipole-quadrupole critical exponent δ_χ has been estimated from the data of the order parameter (M) and the susceptibility (χ). The simulations have been done in the interval $ 0 \leqslant \ell = \frac{I} {J}0 \leqslant 0.01 $ 0 \leqslant \ell = \frac{I} {J}0 \leqslant 0.01 for $ d = \frac{D} {J} = 0,k = \frac{K} {J} = 0 $ d = \frac{D} {J} = 0,k = \frac{K} {J} = 0 and $ h = \frac{H} {J} = 0 $ h = \frac{H} {J} = 0 parameter values on a face centered cubic (fcc) lattice with periodic boundary conditions. The results indicate that the effect of the ℓ parameter is similar to the external magnetic field (h). The critical exponent δ_ℓ are in good agreement with the universal value (δ _h = 5) of the external magnetic field.     

The influence of geometry on the vibronic spectra of quantum aggregates

A study is presented of the localisation of excitonic states on extended molecular aggregates composed of identical monomers arising, not from disorder due to statistical energy shifts of the monomers, induced by environmental interactions (Anderson localisation), but rather simply due to changes in the orientation and geometrical arrangement of the transition dipoles. It is shown further that such small changes nevertheless can have a drastic effect on the shape of the vibronic spectrum of the aggregate. The vibronic spectra are calculated using the ‘coherent exciton scattering’ (CES) approximation whose derivation we generalise to be applicable to aggregates of arbitrary size and geometry.     

Superluminal Signal Velocity and Causality

A superluminal signal velocity (i.e. faster than light) is said to violate causality. However, superluminal signal velocities have been measured in tunneling experiments recently. The classical dipole interaction approach by Sommerfeld and Brillouin results in a complex refractive index with a finite real part. For the tunneling process with its purely imaginary refractive index this model obtaines a zero-time traversing of tunneling barriers in agreement with wave meechanics. The information of a signal is proportional to the product of its frequency band width and its time duration. The reasons that superluminal signal velocities do not violate causality are: (i) physical signals are frequency band limited and (ii) signals have a finite time duration.