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V Correcher J Garcia-Guinea FJ Valle-Fuentes 《Journal of Thermal Analysis and Calorimetry》2006,83(2):439-444
In
this paper, novel results on the blue thermally stimulated luminescence (TSL)
emission of ulexite (NaCaB5O6(OH)6·5H2O)
have been studied. The four maxima appearing at 60, 110, 200 and 240°C
on the TSL glow curves of this borate could be respectively associated to:
(i) the first dehydration (NaCaB5O6(OH)6·5H2O→NaCaB5O6(OH)6·3H2O),
(ii) the creation-annihilation of the three-hydrated
phase, (iii) the Na-coordinated chains
dehydroxylation and the starting point of the alkali self-diffusion through
the lattice and (iv) the amorphisation
of the lattice. These results are fairly well correlated with the differential
thermal analyses (DTA), in situ thermal observations under environmental scanning
electron microscope (TESEM) and thermal X-ray diffraction (TXRD) techniques. 相似文献
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S. Wenmackers D. E. P. Vanpoucke I. Douven 《The European Physical Journal B - Condensed Matter and Complex Systems》2012,85(1):44
We present a model for studying communities of epistemically interacting agents who
update their belief states by averaging (in a specified way) the belief states of other
agents in the community. The agents in our model have a rich belief state, involving
multiple independent issues which are interrelated in such a way that they form a theory
of the world. Our main goal is to calculate the probability for an agent to end up in an
inconsistent belief state due to updating (in the given way). To that end, an analytical
expression is given and evaluated numerically, both exactly and using statistical
sampling. It is shown that, under the assumptions of our model, an agent always has a
probability of less than 2% of ending up in an inconsistent belief state. Moreover, this
probability can be made arbitrarily small by increasing the number of independent issues
the agents have to judge or by increasing the group size. A real-world situation to which
this model applies is a group of experts participating in a Delphi-study. 相似文献
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A Flexible Photoactive Titanium Metal–Organic Framework Based on a [TiIV3(μ3‐O)(O)2(COO)6] Cluster
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Bart Bueken Dr. Frederik Vermoortele Dr. Danny E. P. Vanpoucke Dr. Helge Reinsch Dr. Chih‐Chin Tsou Dr. Pieterjan Valvekens Dr. Trees De Baerdemaeker Prof. Dr. Rob Ameloot Prof. Dr. Christine E. A. Kirschhock Prof. Dr. Veronique Van Speybroeck Prof. Dr. James M. Mayer Prof. Dr. Dirk De Vos 《Angewandte Chemie (International ed. in English)》2015,54(47):13912-13917
The synthesis of titanium–carboxylate metal–organic frameworks (MOFs) is hampered by the high reactivity of the commonly employed alkoxide precursors. Herein, we present an innovative approach to titanium‐based MOFs by the use of titanocene dichloride to synthesize COK‐69, the first breathing Ti MOF, which is built up from trans‐1,4‐cyclohexanedicarboxylate linkers and an unprecedented [TiIV3(μ3‐O)(O)2(COO)6] cluster. The photoactive properties of COK‐69 were investigated in depth by proton‐coupled electron‐transfer experiments, which revealed that up to one TiIV center per cluster can be photoreduced to TiIII while preserving the structural integrity of the framework. The electronic structure of COK‐69 was determined by molecular modeling, and a band gap of 3.77 eV was found. 相似文献
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Identification of the impedance model of an implanted cochlear prosthesis from intracochlear potential measurements 总被引:2,自引:0,他引:2
Vanpoucke FJ Zarowski AJ Peeters SA 《IEEE transactions on bio-medical engineering》2004,51(12):2174-2183
Those suffering from a severe to profound sensorineural hearing loss can obtain substantial benefit from a cochlear implant prosthesis. An electrode array implanted in the inner ear stimulates auditory nerve fibers by direct injection of electrical current. A major limitation of today's technology is the imprecise control of intracochlear current flow, particularly the relatively wide spread of neural excitation. A better understanding of the intracochlear electrical fields is, therefore, required. This paper analyzes the structure of intracochlear potential measurements in relation to both the subject's anatomy and to the properties of the electrode array. An electrically equivalent network is proposed, composed of small lumped circuits for the interface impedance and for the cochlear tissues. The numerical methods required to estimate the model parameters from high-quality electrical potential recordings are developed. Finally, some models are presented for subjects wearing a Clarion CII device with a HiFocus electrode and discussed in terms of model reliability. 相似文献
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Moonen M. Vanpoucke F.J. Deprettere E.F. 《Signal Processing, IEEE Transactions on》1994,42(9):2439-2448
Recently the new class of so-called subspace methods for high-resolution direction finding has received a great deal of attention in the literature. When a real-time implementation is aimed at, the computational complexity involved is known to represent a serious impediment. In this paper, an ESPRIT-type algorithm is developed, which is fully adaptive and therefore particularly suited for real-time processing. Furthermore, a systolic array is described, which allows the processing of incoming data at a rate which is independent of the problem size. The algorithm is based on orthogonal transformations only. Estimates are computed for the angles of arrival, as well as for the source signals. Our aim is not so much to develop yet another ESPRIT-type algorithm but rather to show that it is indeed possible to develop an algorithm that is fully parallel and adaptive. This is something that has not been done before 相似文献
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