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1.
Use of ab initio pseudopotentials for the assignment of boundary conditions of clusters modeling MgO
V. A. Nasluzov G. L. Gutsev V. V. Rivanenkov K. M. Neiman A. G. Anshits 《Journal of Structural Chemistry》1992,33(2):157-161
Conclusions The work reported in this article was aimed at determining the feasibility and desirability of using ab initio core pseudopotential anionic centers and cluster models of ionic crystals of the type of a cluster implanted in a crystal. The results presented herein, from calculations of a number of clusters of magnesium oxide, demonstrate the promise of this approach for compensation of bond rupture effects. In particular, such a model offers a means for a substantial reduction of the artifact-introduced nonequivalence of the partial ionic densities and the effective charges. The comparatively high reliability of the cluster scheme proposed in this work is also supported by results from calculations of the geometric parameters of the crystal.Branch of Institute of Chemical Physics, Russian Academy of Sciences. Institute of Chemistry of Natural Organic Raw Materials, Siberian Branch, Russian Academy of Sciences. Translated from Zhurnal Strukturnoi Khimii, Vol. 33, No. 2, pp. 3–7, March–April, 1992. 相似文献
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I. L. Glazko O. P. Gur’yanova S. V. Levanova S. A. Kozlova N. S. Neiman 《Russian Journal of Applied Chemistry》2005,78(6):950-954
A procedure was developed for preparing a plasticizer for polyvinyl chloride compounds from the fraction of dioxane alcohols. The main physicochemical properties of the new plasticizer were determined. Items prepared from formulations containing the new plasticizer were fabricated and tested in laboratory.__________Translated from Zhurnal Prikladnoi Khimii, Vol. 78, No. 6, 2005, pp. 972–976.Original Russian Text Copyright © 2005 by Glazko, Gur’yanova, Levanova, Kozlova, Neiman. 相似文献
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6-Thiopurine and its N- or C-alkyl derivatives all form an [M – 1]-ion upon fragmentation. In the 7-alkyl derivatives, this ion represents the major component of the spectrum. This is ascribed to formation of a five-membered thiazoline-like ring. Similar ring formation stabilises the [M – 1]-ion in the 7-methyl derivatives of hypoxanthine, adenine and 6-selenopurine. 相似文献
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A. Ya. Neiman A. V. Karapetyan N. N. Pestereva 《Russian Journal of Electrochemistry》2014,50(1):58-69
Composites {Me2(WO4)3 ? xWO3} (Me = Sc, In) (x = 0.5–99%) are synthesized and characterized by XRD and electron microscopy methods and also by the density and specific surface measurements. Temperature dependences of the total conductivity of composites are measured. The contributions of σtot and σel are assessed by the $\sigma (a_{O_2 } )$ and EMF methods. The concentration dependences of conductivity and activation energy are plotted based on the σtot and σion data. It is shown that (a) in the interval x = 0–30 vol % WO3 (0–70 mol %), the conductivity is independent of composition and the ionic component prevails; (b) in the interval x = 60–94.5 vol % (90–99 mol %), the electron conductivity prevails and increases with the increase in x; (c) in the x interval of 30–60 vol % WO3 (70–90 mol %), the conductivity is mixed, i.e., electron(n-type)-ionic; the latter region represents the transition interval from ionic to electron conductivity as x increases. These data are compared with the results obtained earlier for MeWO4-WO3 composites (Me = Ca, Sr, Ba). As regards the structural topology, the {Me2(WO4)3 ? xWO3} composites pertain to the randomly distributed type. It is shown that in contrast to {MeIIWO4 · xWO3} composites, the composites under study do not form the nonautonomous interface phase with the high ionic conductivity. The possible reasons for the observed differences in the topology and the conduction type of composites based on MeWO4 and Me2(WO4)3 are analyzed. 相似文献
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Neiman A Schimansky-Geier L Moss F Shulgin B Collins JJ 《Physical review. E, Statistical physics, plasmas, fluids, and related interdisciplinary topics》1999,60(1):284-292
We study, in terms of synchronization, the nonlinear response of noisy bistable systems to a stochastic external signal, represented by Markovian dichotomic noise. We propose a general kinetic model which allows us to conduct a full analytical study of the nonlinear response, including the calculation of cross-correlation measures, the mean switching frequency, and synchronization regions. Theoretical results are compared with numerical simulations of a noisy overdamped bistable oscillator. We show that dichotomic noise can instantaneously synchronize the switching process of the system. We also show that synchronization is most pronounced at an optimal noise level-this effect connects this phenomenon with aperiodic stochastic resonance. Similar synchronization effects are observed for a stochastic neuron model stimulated by a stochastic spike train. 相似文献
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