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Novel mixed valence states have been obtained by the treatment of cobaltous ferrocyanides (Co+2FeII) and ferricyanides (Co+2FeIII) in an ozone flow. The CN stretching bands occur at 2085 cm–1 for Co+2FeII and at 2160 cm–1 for Co+2FeIII. After the ozonization process of Co+2FeII, an intense band approximately at 2125 cm–1 is detected. This intermediate band must correspond to a mixed valence state of the type: FeII–CN–Co2+–NC–FeIII Mössbauer spectra recorded in situ during the ozonization of Co+2FeII show the presence of two components: a doublet with isomer shift and quadrupole splitting values close to the cobalti ferricyanide and a very broad line for the mixed valence state. From the Mössbauer and infrared spectra of the aged samples of the Co+2FeII after ozonization, a relaxation process to the initial state of the samples is observed but the mixed valence state is stable. 相似文献
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Abe K Ahrens LA Amako K Aronson SH Beier EW Callas JL Cutts D Diwan M Durkin LS Gibbard BG Heagy SM Hedin D Hoftun JS Hurley M Kabe S Kurihara Y Lanou RE Mann AK Marx MD Murtagh MJ Nagashima Y Newcomer FM Shinkawa T Stern E Suzuki Y Terada S White DH Williams HH Yamaguchi Y 《Physical review letters》1987,58(7):636-639
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Makins NC Ent R Chapman MS Hansen J Lee K Milner RG Nelson J Arnold RG Bosted PE Keppel CE Lung A Rock SE Spengos M Szalata ZM Tao LH White JL Coulter KP Geesaman DF Holt RJ Jackson HE Papavassiliou V Potterveld DH Zeidman B Arrington J Beise EJ Belz E Filippone BW Gao H Lorenzon W Mueller B McKeown RD O'Neill TG Epstein M Margaziotis DJ Napolitano J Kinney E Anthony PL van Bibber K Dietrich FS Gearhart RA Patratos GG Kuhn SE van den Brand JF Bulten H Jones CE 《Physical review letters》1994,72(13):1986-1989
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van den Brand JF Ent R Anthony PL Arnold RG Arrington J Beise EJ Belz JE Bosted PE Bulten H Chapman MS Coulter KP Dietrich FS Epstein M Filippone BW Gao H Gearhart RA Geesaman DF Hansen J Holt RJ Jackson HE Jones CE Keppel CE Kinney ER Kuhn S Lee K Lorenzon W Lung A Makins NC Margaziotis DJ McKeown RD Milner RG Mueller B Napolitano J Nelson J O'Neill TG Papavassiliou V Petratos GG Potterveld DH Rock SE Spengos M Szalata ZM Tao LH van Bibber K Wasson DA White JL Zeidman B 《Physical review D: Particles and fields》1995,52(9):4868-4871
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Summary We investigate the transition from two-frequency quasiperiodicity to chaotic behavior in a model for a quasiperiodically driven
magnetoelastic ribbon. The model system is a two-frequency parametrically driven Duffing oscillator. As a driving parameter
is increased, the route to chaos takes place in four distinct stages. The first stage is a torus-doubling bifurcation. The
second stage is a transition from the doubled torus to a strange nonchaotic attractor. The third stage is a transition from
the strange nonchaotic attractor to a geometrically similar chaotic attractor. The final stage is a hard transition to a much
larger chaotic attractor. This latter transition arises as the result of acrisis, the characterization of which is one of our primary concerns. Numerical evidence is given to indicate that the crisis arises
from the collision of the chaotic attractor with the stable manifold of a saddle torus. Intermittent bursting behavior is
present after the crisis with the mean time between bursts scaling as a power law in the distance from the critical control
parameter; τ ∼ (A-Ac)-α. The critical exponent is computed numerically, yielding the value α=1.03±0.01. Theoretical justification is given for the
computed critical exponent. Finally, a Melnikov analysis is performed, yielding an expression for transverse crossings of
the stable and unstable manifolds of the crisis-initiating saddle torus. 相似文献
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Tkaczyk S Tollefson K Tollestrup A Toyoda H Trischuk W de Troconiz JF Tseng J Turini N Ukegawa F Valls J Vejcik S Velev G Vidal R Vilar R Vologouev I Vucinic D Wagner RG Wagner RL Wahl J Wallace NB Walsh AM Wang C Wang CH Wang MJ Watanabe T Waters D 《Physical review letters》2000,84(6):1110-1115
We search for color singlet technirho and technipion production in p&pmacr; collisions at sqrt[s] = 1.8 TeV recorded with the Collider Detector at Fermilab. These exotic technimesons are present in a model of walking technicolor. The signatures studied are lepton plus two jets plus E(T) and multijet final states. No excess of events is seen in either final state. We set an upper limit on the technirho production cross section and exclude a region in the technipion mass versus technirho mass plane. 相似文献
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Toyoda H Trischuk W de Troconiz JF Tseng J Turini N Ukegawa F Vaiciulis T Valls J Vejcik S Velev G Vidal R Vilar R Volobouev I Vucinic D Wagner RG Wagner RL Wahl J Wallace NB Walsh AM Wang C Wang CH Wang MJ Watanabe T Waters D Watts T Webb R 《Physical review letters》2000,84(22):5043-5048
We report results from a study of events with a leading antiproton of beam momentum fraction 0.9057 GeV. Using the dijet events, we evaluate the diffractive structure function of the antiproton and compare it with expectations based on results obtained in diffractive deep inelastic scattering experiments at the DESY ep collider HERA. 相似文献