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It is shown how the energy-positivity criterion enables us to localize the energy in various field theories. For this purpose the role of surface integrals in a canonical formalism is investigated. The same techniques are applied to linearized gravity, where the mixed Cauchy-boundary value problem in a finite volume is analyzed. Unconstrained degrees of freedom and boundary data which have to be controlled are found. This paper is part of a program to analyze the possibility of localization of gravitational energy in complete General Relativity. 相似文献
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Micha Kijak Anna Zieli ska Charles Chamchoumis Jerzy Herbich Randolph P. Thummel Jacek Waluk 《Chemical physics letters》2004,400(4-6):279-285
Depending on the polarity and protic abilities of the solvent, 2-(2′-pyridyl)pyrrole can exist in either syn or anti rotameric forms. In nonpolar solvents, intramolecular excited state single proton transfer is observed, manifested by the appearance of low-energy tautomeric emission. The solvent-assisted excited state double proton transfer reaction is also detected. DFT calculations confirm low barriers for both single and double proton transfer processes in the lowest excited singlet state and show different character of the tautomerization in both cases: in the intramolecular reaction, mutual approach of two nitrogen atoms plays an important role. 相似文献
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We prove that certain two-point Padé approximants occupying the diagonal of the Padé table form monotone sequences of lower and upper bounds uniformly converging to a Stieltjes function. The results can be applied to the theory of inhomogeneous media for the calculation of the bounds on the effective transport coefficients of heterogeneous materials. 相似文献
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Jerzy F. Plebański Maciej Przanowski 《International Journal of Theoretical Physics》1994,33(7):1535-1551
Electrodynamics admitting a duality transformation group is considered. For such an electrodynamics an extension of the classical Rainich-Misner-Wheeler theory is presented.On leave of absence from the University of Warsaw, Warsaw, Poland. 相似文献
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The paper is focused on the phenomena of various steady-state oscillations exhibited by the twin-well potential system. Regions of existence of different attractors in the system parameter domain are examined and a picture book of different steady states for fixed damping and forcing is presented: 20 different combinations of single or coexisting, small orbit or large orbit, periodic and chaotic attractors are displayed. Computer simulations are followed by an approximate analytical analysis: A study of various forms of instability of periodic solutions gives close form approximate criteria for occurrence of T-periodic small orbit and large orbit oscillations, and for cross-well chaos. 相似文献
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Commercially available 1,4-dioxane, even of spectroscopic grade, contains various impurities that arise mostly from reaction of the solvent with oxygen. Aspects relevant to the spectroscopy and photochemistry of the dioxane/oxygen system are discussed. Methods of purification and storage of the solvent are presented. 相似文献
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Exchange interactions in copper(II) complexes with tridentate Schiff bases: EPR and magnetic studies
Bogusława Jeżowska-Trzebiatowska Julia Jezierska Jerzy Baranowski 《Chemical physics letters》1977,52(3):590-594
The influence of the nature of ligands upon the magnetic and EPR properties was investigated for the series of polynuclear Cu(II) complexes with tridentate Schiff bases. A similar tendency of changes in the |J| and D parameters was found for binuclear Cu(II) complexes with ligands derived from condensation of 3-amino-1-propanol with 2-hydroxyaldehydes and acetylacetone as well as for Cu(II) complexes with condensation products of o-aminophenol and β-diketones. The Cu(II) complex with Schiff base of 1-amino-2-propanol and acetylacetone exhibits ferromagnetic behaviour suggesting tetrameric structure. 相似文献