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1.
[reaction: see text] Various ferrocene-based organosilanols have been synthesized in four steps starting from achiral ferrocene carboxylic acid. Applying these novel planar-chiral ferrocenes as catalysts in asymmetric phenyl transfer reactions to substituted benzaldehydes afforded products with high enantiomeric excesses. The best result (91% ee) was achieved in the addition to p-chlorobenzaldehyde with organosilanol 2b, which has a tert-butyl substituent on the oxazoline ring and an isopropyl group on the silanol fragment. 相似文献
2.
Muhammed Oz Namik Kemal Saritekin Cetin Bozkurt Erhan Budak Gurcan Yildirim 《Crystal Research and Technology》2016,51(12):708-717
This study is interested in the effect of lithium carbonate on the formation of hexagonal boron nitride (hBN) by means of the available experimental methods including TGA, XRD, FTIR, SEM and HR‐TEM. hBN samples were synthesized at the 1450 °C with different molar ratios of lithium carbonate by modified O'Connor routine. The crystalline hBN formation tended to improve with the increment of the Li2CO3 concentration level (especially after more 20 %). The dopant quantity decreased the residual stresses due to the presence of possible relaxation mechanisms along with the nanocrystal structure, even favored by XRD experimental findings regarding the enhancement of crystal plane alignments, crystallite sizes and lattice parameters. As for the FTIR surveys, the Li2CO3 foreign impurities strengthened more and more the covalent bonds between boron and nitrogen atoms. At the same time, the samples with 40 % lithium carbonate were annealed at the varied temperatures of 1000, 1150, 1300 and 1450 °C to determine the optimum annealing temperature. The XRD+FTIR investigations indicated that the degree of hexagonality improved with the increased annealing temperature. Similarly, the surface morphology confirmed not only the formation of regularity and flaky hexagonal BN structures, but also the strengthening of covalent bonds between the atoms. 相似文献
3.
We consider in the framework of the fluid-gravity correspondence the dynamics of hypersurfaces located in the holographic radial direction at r = r(0). We prove that these hypersurfaces evolve, to all orders in the derivative expansion and including all higher curvature corrections, according to the same hydrodynamics equations with identical transport coefficients. The analysis is carried out for normal fluids as well as for superfluids. Consequently, this proves the exactness of the bulk viscosity formula derived by us [J. High Energy Phys. 06 (2011) 007] via the null horizon dynamics. 相似文献
4.
Jasmin Oz 《Waves in Random and Complex Media》1997,7(1):107-117
The recently introduced modal expansion representation for the two-frequency mutual coherence function is applied here to the solution of a point-source field in a random medium. This approach reduces the solution for any structure function to an eigenvalue problem for an ordinary differential equation. For the initial point source it is shown here that the modal expansion yields a result similar to that for the initial plane wave, modified by a spherical free-space phase which contains a weighted coordinate that does not interact with the medium. Having established these general characteristics, special attention is paid to power-law media and, in particular, to a quadratic medium, for which a new exact solution is derived. Via a collective summation of this new modal solution, we rederive the alternative exact solution which exists in the literature. We also discuss the new parameterization implied by the new modal solution. 相似文献
5.
Huang C Lu W Zhou M Clayton CE Joshi C Mori WB Muggli P Deng S Oz E Katsouleas T Hogan MJ Blumenfeld I Decker FJ Ischebeck R Iverson RH Kirby NA Walz D 《Physical review letters》2007,99(25):255001
The electron hosing instability in the blow-out regime of plasma-wakefield acceleration is investigated using a linear perturbation theory about the electron blow-out trajectory in Lu et al. [in Phys. Rev. Lett. 96, 165002 (2006)10.1103/PhysRevLett.96.165002]. The growth of the instability is found to be affected by the beam parameters unlike in the standard theory Whittum et al. [Phys. Rev. Lett. 67, 991 (1991)10.1103/PhysRevLett.67.991] which is strictly valid for preformed channels. Particle-in-cell simulations agree with this new theory, which predicts less hosing growth than found by the hosing theory of Whittum et al. 相似文献
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9.
Oz E Deng S Katsouleas T Muggli P Barnes CD Blumenfeld I Decker FJ Emma P Hogan MJ Ischebeck R Iverson RH Kirby N Krejcik P O'Connell C Siemann RH Walz D Auerbach D Clayton CE Huang C Johnson DK Joshi C Lu W Marsh KA Mori WB Zhou M 《Physical review letters》2007,98(8):084801
The onset of trapping of electrons born inside a highly relativistic, 3D beam-driven plasma wake is investigated. Trapping occurs in the transition regions of a Li plasma confined by He gas. Li plasma electrons support the wake, and higher ionization potential He atoms are ionized as the beam is focused by Li ions and can be trapped. As the wake amplitude is increased, the onset of trapping is observed. Some electrons gain up to 7.6 GeV in a 30.5 cm plasma. The experimentally inferred trapping threshold is at a wake amplitude of 36 GV/m, in good agreement with an analytical model and PIC simulations. 相似文献
10.
In many generic combustion models, one finds that a combustionwave will develop with a specific wave speed. However, thereare possible initial temperature profiles which do not evolveinto such waves, but rather die out to the ambient temperature.There can exist, in some models, a clear distinction betweenthose initial conditions that do evolve into combustion wavesand those that do not; this is sometimes referred to as thewatershed initial condition. When fuel consumption is consideredto be negligible, analytical methods can be used to obtain theexact watershed. In this paper, we consider the problem of determiningpseudo-watersheds and ascertaining the relationship betweenthese pseudo-watersheds and the exact watersheds. In the processa novel weight-function approach for infinite spatial domainsis developed. 相似文献