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A new scheme for controlling photodissociation through preparation of a variationally optimized linear superposition of field free vibrational eigenstates is applied for selective control of IBr and HI dissociation. The dependence of photodissociation on various field parameters and initial conditions is examined to investigate the mechanistic basis of selective control. The parametric equations of motion approach for determining vibrational dynamics as a function of field parameters without having to solve the time dependent Schrödinger equation explicitly for each field parameter separately is outlined and its use to identify field characteristics which will provide the requisite population mix represented by the optimal linear superposition of vibrational states is advocated. 相似文献
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Kenneth A. Caldwell Michael L. Gross 《Journal of the American Society for Mass Spectrometry》1994,5(2):72-91
Accurate mass measurements were used to assign elemental compositions and tandem mass spectrometry was used to characterize the peak-at-every-mass background ions produced by kiloelectron-volt-particle bombardment of neat fast-atom bombardment matrices. The majority of the background ions observed in the mass spectrum of neat glycerol was identified. On the basis of the experiments with glycerol, a theory for the formation of background ions is presented. Results are discussed according to the chemical and physical changes that ygoe;on-volt-particle bombardment produces in the matrix. 相似文献
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The purpose of this paper is to review the mechanisms and available theoretical methods for modeling the strength and failure of thin film/substrate systems 相似文献
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D. Gross 《Applied physics. B, Lasers and optics》2007,86(3):367-370
According to a classical result due to Hudson, the Wigner function of a pure, continuous-variable quantum state is non-negative
if and only if the state is Gaussian. We have proven an analogous statement for finite-dimensional quantum systems. In this
context, the role of Gaussian states is taken on by stabilizer states. The general results have been published in [1]. For
the case of systems of odd prime dimension, a different, greatly simplified method of proof can be employed which still exhibits
the main ideas. The present paper gives a self-contained account of these methods.
PACS 03.65.Fd; 03.65.Sq; 03.67.-a 相似文献
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[reaction: see text] Following the discovery that meso-substituted corroles are formed in solvent-free condensation of pyrrole with aldehydes, we demonstrate that a small variation in the methodology is suitable for facile synthesis of cobalt(III) corrole and hexaphyrin. These compounds, as well as three noncyclic products, were fully characterized by spectroscopy and X-ray crystallography. 相似文献