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1.
Simen Gjelseth Antonsen Arne Joakim C. Bunkan Tomas Mikoviny Yngve Stenstrøm Armin Wisthaler 《Molecular physics》2020,118(15)
The kinetics of the O3, OH and NO3 radical reactions with diazomethane were studied in smog chamber experiments employing long-path FTIR and PTR-ToF-MS detection. The rate coefficients were determined to be k CH2NN+O3?=?(3.2?±?0.4)?×?10?17 and k CH2NN+OH?=?(1.68?±?0.12)?×?10?10 cm3 molecule?1 s?1 at 295?±?3?K and 1013?±?30 hPa, whereas the CH2NN?+?NO3 reaction was too fast to be determined in the static smog chamber experiments. Formaldehyde was the sole product observed in all the reactions. The experimental results are supported by CCSD(T*)-F12a/aug-cc-pVTZ//M062X/aug-cc-pVTZ calculations showing the reactions to proceed exclusively via addition to the carbon atom. The atmospheric fate of diazomethane is discussed. 相似文献
2.
3.
Arne Miller 《Radiation Physics and Chemistry》1993,42(4-6):581-584
The activities and services of the accredited Risø High Dose Reference Laboratory are described. The laboratory operates according to the European standard EN 45001 regarding Operation of Testing Laboratories, and it fulfills the requirements of being able to deliver traceable dose measurements for control of radiation sterilization. The accredited services include:
1. 1. Irradiation of dosimeters and test samples with cobalt-60 gamma rays.
2. 2. Irradiation of dosimeters and test samples with 10 MeV electrons.
3. 3. Issue of and measurement with calibrated dosimeters.
4. 4. Measurement of the dosimetric parameters of an irradiation facility.
5. 5. Measurement of absorbed dose distribution in irradiated products.
The paper describes these services and the procedures necessary for their execution. 相似文献
4.
Linear complexity and linear complexity profile are important characteristics of a sequence for applications in cryptography
and Monte-Carlo methods.
The nonlinear congruential method is an attractive alternative to the classical linear congruential method for pseudorandom
number generation.
Recently, a weak lower bound on the linear complexity profile of a general nonlinear congruential pseudorandom number generator
was proven by Gutierrez, Shparlinski and the first author. For most nonlinear generators a much stronger lower bound is expected.
Here, we obtain a much stronger lower bound on the linear complexity profile of nonlinear congruential pseudorandom number
generators with Dickson polynomials. 相似文献
5.
6.
Arne Barinka Stephan Dahlke Wolfgang Dahmen 《Advances in Computational Mathematics》2006,24(1-4):5-34
Recently adaptive wavelet methods have been developed which can be shown to exhibit an asymptotically optimal accuracy/work
balance for a wide class of variational problems including classical elliptic boundary value problems, boundary integral equations
as well as certain classes of noncoercive problems such as saddle point problems. A core ingredient of these schemes is the
approximate application of the involved operators in standard wavelet representation. Optimal computational complexity could
be shown under the assumption that the entries in properly compressed standard representations are known or computable in
average at unit cost. In this paper we propose concrete computational strategies and show under which circumstances this assumption
is justified in the context of elliptic boundary value problems.
Dedicated to Charles A. Micchelli on the occasion of his 60th birthday
Mathematics subject classifications (2000) 41A25, 41A46, 65F99, 65N12, 65N55.
This work has been supported in part by the Deutsche Forschungsgemeinschaft SFB 401, the first and third author are supported
in part by the European Community's Human Potential Programme under contract HPRN-CT-202-00286 (BREAKING COMPLEXITY). The
second author acknowledges the financial support provided through the European Union's Human Potential Programme, under contract
HPRN-CT-2002-00285 (HASSIP) and through DFG grant DA 360/4–1. 相似文献
7.
Richard P. Fischer Arne W. Fliflet 《International Journal of Infrared and Millimeter Waves》2002,23(9):1297-1313
This paper presents the design and test of asymmetric quasioptical resonators for gyrotron applications, where most of the diffraction output coupling comes from the smaller of two mirrors. A computer code based on scalar diffraction theory is used to calculate the resonator losses and the electric field near the mirrors. Resonators with mirror separations approaching confocal have reduced side lobes in the diffraction patterns, which should allow for better power transmission and focusing. Cold tests have been performed at 94 and 141 GHz to measure the quality factor of the asymmetric resonators as a function of mirror separation and mirror misalignment. Typical resonator parameters include 65 cm mirror separation, 1-3% output coupling and 85% of the losses from the small mirror. A half-symmetric resonator with one flat and one curved mirror has also been investigated. The calculated values of Q are in reasonably good agreement with the cold test measurements. 相似文献
8.
Arne Schirrmacher 《Physics in Perspective (PIP)》2003,5(1):4-20
David Hilbert (1862-1943) played an important role in establishing quantum physics in Göttingen. I analyze the ways in which his influence was decisive by comparison with Woldemar Voigt (1850-1919). Voigt was the leading Göttingen theoretical physicist before the arrival of Peter Debye (1884-1966), who was appointed to a new professorship in 1914 at Hilbert's instigation. I portray the Göttingen mathematicians, above all Hermann Minkowski (1864-1909) and David Hilbert, as planting the seeds for the blossoming of quantum physics under their student Max Born (1882-1970) in the 1920s. 相似文献
9.
10.
R. Klein R. Grieser L. Hoog G. Huber I. Klaft P. Merz T. Kühl S. Schröder M. Grieser D. Habs W. Petrich D. Schwalm 《Zeitschrift für Physik A Hadrons and Nuclei》1992,342(4):455-461
We have performed for the first time precision spectroscopy on a coasting fast7Li+ ion beam in a storage ring. The ion beam moving with 6.4% speed of light was first electron cooled and then merged with two counterpropagating laser beams acting on two different hyperfine transitions sharing a common upper level (λ-system). One laser was frequency locked to thea 3 127J2 hfs frequency component established as a secondary frequency standard at 514 nm. The second laser was tuned over theλ-resonance, which was recorded relative to127J2 hfs components. This experiment is sensitive to the time dilation in fast moving frames and will lead to new limits for the verification of special relatively. The present status of the experiment and perspectives in accuracy are discussed. 相似文献