Dual mode near-field scanning optical microscopy for near-field imaging of surface plasmon polariton

In this paper, we theoretically and experimentally demonstrate that metal coated apertured probes are efficient near-field probes on surfaces with high reflectivity for the scattering as well as for the collection mode near-field scanning optical microscopy (NSOM). We show that a blunt apertured metal coated tip is very effective in suppressing image dipoles which affect strongly the signals scattered from frequently used sharp metal tips or gold nanoparticle attached probes. By using a simultaneous collection and scattering mode (dual mode) NSOM we measure the near-field images of surface plasmon polariton (SPP) launched from a slit. The collection mode measures propagating SPP along lateral distance in a long scan range with high signal-to-noise ratio, and the scattering mode measures the polarization resolved near-field of SPP. Comparisons of the measured data obtained in the dual mode enable to easily characterize SPP and to separate the measured near-field into the propagating SPP and the directly transmitted light.     

Surface plasmon resonance (SPR) reflectance imaging: Far-field recognition of near-field phenomena

The surface plasmon resonance (SPR) reflectance imaging technique provides a label-free visualization tool to characterize the near-field fluidic transport properties within 100 nm from the solid surface. The key idea is that the SPR reflectance intensity varies with the near-field refractive index (RI) of the test fluid, which in turn depends on the micro- and nano-fluidic scalar properties such as concentrations, temperatures, and phase changes, occurring in the near-field. As essential knowledge to understand and implement the SPR reflectance imaging technique, this paper presents discussions on the basics of surface plasmon polaritons (SPPs), surface plasmon resonance (SPR), setup of the SPR reflectance imaging system, and the SPR reflectance imaging resolution. The second part of the paper elaborates the applications of the SPR imaging sensor technique in characterizing the near-field fingerprints of nanofluidic evaporative self-assembly.     

Faraday-rotation imaging by near-field optical microscopy

Scanning near-field optical microscopy with polarization modulation (PM-SNOM) has been applied to image the surface of a yttrium-iron-garnet (YIG) film. Lock-in detection of the phase of the transmitted light directly gives the magnitude of the Faraday rotation angle.     

Cloaked near-field scanning optical microscope tip for noninvasive near-field imaging

Near-field imaging is a well-established technique in biomedical measurements, since closer to the detail of interest it is possible to resolve subwavelength details otherwise unresolved by regular lenses. A near-field scanning optical microscope (NSOM) tip may indeed overcome the resolution limits of far-field optics, but its proximity inherently perturbs the measurement. Here, we apply the recent concept of a "cloaked sensor" to an NSOM device in collection mode, showing theoretically how a proper plasmonic cover applied to an NSOM tip may drastically improve its overall measurement capabilities.     

Surface plasmon polariton-based optical beam profiler

We describe a surface plasmon polariton- (SPP-) based device for measuring the intensity distribution of strongly focused light beams. A gold thin film configured as a sharp step is positioned in the focal region of a light beam, converting light into SPPs. The SPPs emit directional leakage radiation into the glass substrate beneath the thin film. The intensity of the leakage radiation is proportional to the intensity of the incident local light at the position of the step, allowing us to reconstruct the optical field profile by scanning the thin film's edge through the focal region.     

Surface plasmon polaritons based optical directional coupler

As a basic optical device, the optical directional coupler (ODC) is basically used as optical splitters, optic switches and so on. A novel ODC employing surface plasmon polaritons (SPPs) is proposed for high integration. The finite difference time domain (FDTD) method is adopted to simulate and analyze its properties. Results show that the ODC proposed here follows the general regulations of a conventional dielectric ODC, but its transverse size is of nanoscale, which improves the optical integration greatly. For 1550 nm and 1310 nm input wavelengths, when the coupling region length (L) equals half of its coupling length, the Excess Loss is respectively 0.57 dB and 0.56 dB, which is practical in applications. So the research on the present ODC is of some practical importance.     

Surface plasmon polariton assisted optical pulling force

We demonstrate both analytically and numerically the existence of optical pulling forces acting on particles located near plasmonic interfaces. Two main factors contribute to the appearance of this negative recoil force. The interference between the incident and reflected waves induces a rotating dipole with an asymmetric scattering pattern, while the directional excitation of surface plasmon polaritons (SPPs) enhances the linear momentum of scattered light. The strongly asymmetric SPP excitation is determined by spin–orbit coupling of the rotating dipole and surface plasmon polariton. As a result of the total momentum conservation, the force acting on the particle points in a direction opposite to the incident wave propagation. We derive analytical expressions for the force acting on dipolar particles placed in the proximity of plasmonic surfaces. Analytical expressions for this pulling force are derived within the dipole approximation and are in excellent agreement with results of electromagnetic numerical calculations. The forces acting on larger particles are analyzed numerically, beyond the dipole approximation.

     

Apparent superresolution in near-field optical imaging of periodic gratings

A superresolution phenomenon in images of diffraction gratings obtained with a near-field optical microscope probe positioned at distances of the order of 1>mu;m from the surface was recently reported [Appl. Opt. 33, 876 (1994)]. This experiment was interpreted in terms of evanescent waves observed in the far field. We show that the effect observed in that experiment is a very well known far-field optical phenomenon called the Talbot effect. The existence of self-imaging Talbot planes for gratings with periods of the order of a few micrometers appears promising for many practical applications.     

Surface plasmon resonance polarizator for biosensing and imaging

A novel polarization-sensitive surface plasmon resonance (SPR) biosensing/imaging scheme is proposed. The scheme uses a periodical spatial phase modulation of the pumping beam of a mixed polarization in the Kretschmann–Raether geometry and takes advantage of SPR-based polarizing effect to drastically absorb p-polarized component changing the resulting polarization state of the beam. The scheme then uses Fourier Transformation to efficiently treat and filter spatially-modulated polarization-sensitive signals and thus to extract and process selected SPR-based response. This approach offers a much higher accuracy of measurements in SPR-based multi-sensing and remote sensing.     

THz near-field optical imaging by a local source

A new THz imaging system based on a local illumination by a near-field source is presented. Model object is imaged, and sub-wavelength spatial resolution is demonstrated for the first time to our knowledge with this configuration. The contrast and the resolution are confirmed by a theoretical study based on the diffraction in near-field zone.     

Surface plasmon optical tweezers: tunable optical manipulation in the femtonewton range

We present a quantitative analysis of 2D surface plasmon based optical tweezers able to trap microcolloids at a patterned metal surface under low laser intensity. Photonic force microscopy is used to assess the properties of surface plasmon traps, such as confinement and stiffness, revealing stable trapping with forces in the range of a few tens of femtonewtons. We also investigate the specificities of surface plasmon tweezers with respect to conventional 3D tweezers responsible for their selectivity to the trapped specimen's size. The accurate engineering of the trapping properties through the adjustment of the illumination parameters opens new perspectives in the realization of future optically driven on-a-chip devices.     

Three-dimensional modeling of amplitude-object imaging in scanning near-field optical microscopy

The imaging properties of the transmission-illumination mode of a scanning near-field optical microscope are investigated. Three-dimensional calculations of the power transmitted into classically allowed and forbidden regions for a nonsymmetrically positioned amplitude object are implemented by use of the finite-difference time-domain solution of Maxwell's equations. The evolution of the images with the distance from the object as well as the effect of the polarization of the illumination is shown. The computations show that for applications involving the imaging of an amplitude object, the use of the allowed light is preferred. Collection of light from both the allowed and the forbidden zones leads to degraded contrast and resolution.     

Surface plasmon resonance in near-field coupled gold cylinder arrays fabricated by EUV-interference lithography and hot embossing

Arrays of metal nanoparticles with nanometer-scale gaps between the particles is highly interesting for plasmonic field enhancement applications. We report a simple method to fabricate arrays of closely spaced Au particles with inter-particle separation down to 20 nm. We used extreme ultraviolet interference lithography (EUV-IL) and a mechanical press to fabricate two-dimensional arrays of Au nanoparticles. Lithographically produced particle arrays were modified by hot pressing in a nanoimprint machine and the gap was varied in a range from 50 nm to below 20 nm. Optical measurement shows two resonances at 520 nm and 620 nm, with the latter gaining strength as the gap is reduced. The experimental and theoretical investigations using a FDTD algorithm demonstrate that the low-energy resonance can be assigned to a collective surface plasmon resonance arising from the strong near-field coupling between the nanoparticles. Surface Enhanced Raman Spectroscopy (SERS) experiments performed on a model molecule (BPE) show a large gain in signal intensity as a result of the reduced gaps between the particles.     

Local magneto-optical Kerr effect imaging by scanning near-field optical microscope in reflection-mode

<正>A method for local magneto-optical Kerr effect imaging based on a home-made scanning near-field optical microscope working in reflection mode is presented.Shear force detection is carried out by using a symmetric piezoelectric bimorph sensor,which provides an easy way not only for probe-surface distance control but also for imaging.Polarization-preserving fiber probes used as a local optical detector are fabricated with a heating-pulling technique and the probes' polarization properties are measured.Shear force topographic and near-field magneto-optical images of magneto-optical disk taken with the proposed method are shown.     

Surface plasmon resonance sensors based on Ag-metalized nanolayer in microstructured optical fibers

Surface plasmon resonance sensors based on Ag-metalized nanolayer in microstructured optical fibers are theoretically analyzed by using finite element method (FEM). In our simulations we use Drude-Lorentz model to describe the metal dielectric constant. The numerical results show that the sensitivity of Ag-metalized SPR sensor could reach 1167 nm/RIU and corresponding resolution is 8.57×10⁻⁵ RIU. Compared to conventional Au-metalized SPR sensors the performance of our device is obviously better.     

Surface plasmon interferometric microscopy for three-dimensional imaging of dynamic processes

A method, which we named surface plasmon interferometric microscopy, for real-time displaying of the dynamic evolution of the refractive index (RI) of a sample in three-dimensions is demonstrated experimentally. The Fourier fringe analysis technique is employed to get the phase variations of the samples by demodulating the interference patterns captured by a CCD camera, and the 3D RI distribution can be obtained through numerical interpolation from the relation between the phase and the RI of the samples. Our method may provide an interesting way to monitor fast dynamics of physical, biological, and chemical processes in real time.     

光存储技术中超分辨近场结构研究进展

超分辨近场结构(Super-RENS)是近场光学存储中最具有潜力和应用前景的方案之一。介绍了Super-RENS从基本类型到第三代Super-RENS的发展历程,简述了掩膜材料的研究进展以及Super-RENS在不同记录系统中的应用。展望了它的发展前景。     

Quantum dot labeling based on near-field optical imaging of CD44 molecules

The lateral organization of membrane proteins and lipids domains has a direct impact on many cellular processes, but generally these domains are too small to be resolved by diffraction-limited resolution of fluorescence microscopy. Here, we use quantum dot (QD) labeling based on near-field optical imaging, to study the nanoscale organization of hyaluronan receptor CD44 molecules of fixed mesenchymal stem cells (MSCs) in air, with a optical resolution down to 50 nm. The photostability and high luminance of QD evidently improve the signal-to-noise ratio and reproducibility of near-field optical data. Importantly, the blinking-intensity analysis was proposed to identify single QD, providing a calibration to relate intensity to numbers of antibody for the first time. Additionally, the fluorescence-topographic imaging enables us to investigate the topographic location pattern. Our results demonstrate that CD44 molecules on MSCs are enriched into nanosized domain and they predominantly locate on the peak of the membrane protrusions, which may contribute to clarify the underlying mechanism of functions ascribed to these molecules.     

Surface plasmon polaritons mediated by surface modes in a metal-based photonic crystal complex structure

A hybrid metal–organic–photonic crystal (PC), a gold film with a SU8 film on its top followed by a three-dimensional (3D) PC, was designed to exercise additional control upon the photon behaviors. Attenuated total reflection measurements demonstrate that the 3D PC plays a crucial role in the formation of significant optical properties of the metal-based hybrid and the reflectivity minimum in its reflectivity curve is, mostly, a result of synergetic action of the coupling of surface plasmon polaritons to surface modes and additional guided modes yielded in the resonant cavity composed of the gold film and the PC.     

Boundary-value problems in near-field optical microscopy and optical size resonances

We have solved a boundary-value problem for a ball probe interacting with a flat dielectric surface in an external optical radiation field. This interaction gives rise to the optical size resonance at frequencies significantly different from the natural frequencies of two-level atoms both in the medium and in the probe with allowance for the local field corrections. These resonances depend significantly on the distance from the probe center to the surface, on the ball probe size, on the concentration of two-level atoms in the probe and in the medium, on the spectral line width, and on the atomic inversion. The field strengths inside and outside the ball probe and a semiinfinite dielectric medium have been calculated in the near-field and wave zones. It is shown that the proposed electrodynamic theory of optical near-field microscopy agrees with the results of experimental measurements.